Bright, coherent, ultrafast soft X-ray harmonics spanning the water window from a tabletop light source.

We demonstrate fully phase-matched high harmonic emission spanning the water window spectral region important for nano- and bioimaging and a breadth of materials and molecular dynamics studies. We also generate the broadest bright coherent bandwidth (≈300 eV) to date from any light source, small or large, that is consistent with a single subfemtosecond burst. The harmonic photon flux at 0.5 keV is 10³ higher than demonstrated previously. This work extends bright, spatially coherent, attosecond pulses into the soft x-ray region for the first time.

Spatially coherent, phase matched, high-order harmonic EUV beams at 50 kHz.

By focusing a high repetition rate (50 kHz), compact, femtosecond laser system with low pulse energy (25 muJ) using a tight-focusing geometry, we demonstrate fully phase matched high-order harmonic generation for the first time at very high repetition rates, resulting in EUV light with full spatial coherence. The result is a practical, single-box, coherent source useful for applications in metrology, ultrafast spectroscopy, imaging and microscopy. The soft x-ray flux can be improved further by increasing the laser pulse energy and/or repetition rate.

Enhanced high harmonic generation from multiply ionized argon above 500 eV through laser pulse self-compression.

By combining laser pulse self-compression and high harmonic generation within a single waveguide, we demonstrate high harmonic emission from multiply charged ions for the first time. This approach enhances the laser intensity and counteracts ionization-induced defocusing, extending the cutoff photon energy in argon above 500 eV for the first time, with higher spectral intensity and cutoff energy than He for the same input laser parameters. This Letter demonstrates a pathway for extending high harmonic emission to very high photon energies using large, multiply charged, ions with high ionization potentials.

Quasi-phase matching of high-order harmonic generation at high photon energies using counterpropagating pulses.

We extend all-optical quasi-phase matching of high-order harmonic generation into spectral regions where conventional phase matching is not possible. The high laser intensities required to generate harmonics at energy >130 eV, coupled with the resulting high level of ionization, preclude conventional phase matching in all nonlinear media. Selective enhancement factors between 40 and 150 in the flux of harmonics at photon energies around 140 eV are demonstrated using a train of two counterpropagating pulses.