Compensating losses in polariton propagation with synthesized complex frequency excitation.

Surface plasmon polaritons and phonon polaritons offer a means of surpassing the diffraction limit of conventional optics and facilitate efficient energy storage, local field enhancement and highsensitivity sensing, benefiting from their subwavelength confinement of light. Unfortunately, losses severely limit the propagation decay length, thus restricting the practical use of polaritons. While optimizing the fabrication technique can help circumvent the scattering loss of imperfect structures, the intrinsic absorption channel leading to heat production cannot be eliminated. Here, we utilize synthetic optical excitation of complex frequency with virtual gain, synthesized by combining the measurements made at multiple real frequencies, to compensate losses in the propagations of phonon polaritons with dramatically enhanced propagation distance. The concept of synthetic complex frequency excitation represents a viable solution to the loss problem for various applications including photonic circuits, waveguiding and plasmonic/phononic structured illumination microscopy.

Gauge Field Induced Chiral Zero Mode in Five-Dimensional Yang Monopole Metamaterials.

Owing to the chirality of Weyl nodes characterized by the first Chern number, a Weyl system supports one-way chiral zero modes under a magnetic field, which underlies the celebrated chiral anomaly. As a generalization of Weyl nodes from three-dimensional to five-dimensional physical systems, Yang monopoles are topological singularities carrying nonzero second-order Chern numbers c_{2}=±1. Here, we couple a Yang monopole with an external gauge field using an inhomogeneous Yang monopole metamaterial and experimentally demonstrate the existence of a gapless chiral zero mode, where the judiciously designed metallic helical structures and the corresponding effective antisymmetric bianisotropic terms provide the means for controlling gauge fields in a synthetic five-dimensional space. This zeroth mode is found to originate from the coupling between the second Chern singularity and a generalized 4-form gauge field-the wedge product of the magnetic field with itself. This generalization reveals intrinsic connections between physical systems of different dimensions, while a higher-dimensional system exhibits much richer supersymmetric structures in Landau level degeneracy due to the internal degrees of freedom. Our study offers the possibility of controlling electromagnetic waves by leveraging the concept of higher-order and higher-dimensional topological phenomena.

Spin-orbit interactions in a nonlinear medium due to a nonlinear-induced geometric phase.

In general, a spin-polarized light beam cannot couple its spin angular momentum (SAM) with intrinsic orbital angular momentum (IOAM) without spin reversal. Here we find that nonlinear media can give the spin-polarized photon an IOAM, as they travel in the media due to the nonlinear susceptibility along the transmission direction, which does not require spin reversal. To characterize this SAM-to-IOAM conversion process, we establish an evolution ray equation for photons carrying IOAM by reference to the Schrödinger equation. We further reveal the inherent physics of such a phenomenon from a full-wave perspective and find that the vortex generation originates from the nonlinear-induced geometric phase.

Vortex generation in the spin-orbit interaction of a light beam propagating inside a uniaxial medium: origin and efficiency.

It has been known that an optical vortex with a topological charge ±2 can be generated as a circularly polarized (CP) light beam propagates in a bulk uniaxial crystal, but its physical origin remains obscure which also hinders its practical applications. Here, through a rigorous full-wave analyses on the problem, we show that, as a CP beam possessing a particular spin (handedness) propagates inside a uniaxial crystal, two beams with opposite spins can be generated caused by the unique spin-sensitive light-matter interactions in the anisotropic medium. Flipping the spin can offer the light beam an vortex phase with a topological charge of ±2 owing to the Pancharatnam-Berry mechanism, with efficiency dictated by the material properties of the uniaxial medium and the topological structure of the beam itself. With its physical origin fully uncovered, we finally discuss how to improve the efficiency of such effect, and compare the mechanisms of vortex generations in different systems. Our findings not only provide deeper understandings on such an intriguing effect, but also shed light on other spin-orbit-interaction-induced effects.

Broadband and high-efficiency spin-polarized wave engineering with PB metasurfaces.

Manipulating circularly polarized (CP) light waves at will are highly important for photonic researches and applications. Recently, while Pancharatnam-Berry (PB) metasurfaces have shown unprecedented capabilities to control CP light, meta-devices constructed so far always suffer from the limitations of low-efficiency and narrow bandwidth. Here, we propose a scheme to construct PB metasurfaces with these two issues well addressed. To verify our idea, two PB meta-devices are designed and fabricated for achieving high-efficiency and broadband photonic spin Hall effect and focusing effect, respectively. Experimental results, in good agreement with full wave simulations, demonstrate the desired functionalities with efficiencies reaching 80% within an ultra-wide frequency band (8.2-17.3GHz). The proposed design scheme is generic and can be extended to high-frequency regimes. Our work can stimulate the realizations of high-performance and broadband PB meta-devices with diversified functionalities.

Magneto-optical chiral metasurfaces for achieving polarization-independent nonreciprocal transmission.

Nonreciprocal transmission, resulting from the breaking of Lorentz reciprocity, plays a pivotal role in nonreciprocal communication systems by enabling asymmetric forward and backward propagations. Metasurfaces endowed with nonreciprocity represent a compact and facile platform for manipulating electromagnetic waves in an unprecedented manner. However, most passive metasurfaces that achieve nonreciprocal transmissions are polarization dependent. While incorporation of active elements or nonlinear materials can achieve polarization-independent nonreciprocal metasurfaces, the complicated configurations limit their practical applications. To address this issue, we propose and demonstrate a passive and linear metasurface that combines magneto-optical and chiral effects, enabling polarization-independent isolation. The designed metasurface achieves a transmittance of up to 80%, with a high contrast between forward and backward propagations. Our work introduces a novel mechanism for nonreciprocal transmission and lays the foundation for the development of compact, polarization-insensitive nonreciprocal devices.

Prediction of nonlayered oxide monolayers as flexible high-κ dielectrics with negative Poisson's ratios.

During the last two decades, two-dimensional (2D) materials have been the focus of condensed matter physics and material science due to their promising fundamental properties and (opto-)electronic applications. However, high-κ 2D dielectrics that can be integrated within 2D devices are often missing. Here, we propose nonlayered oxide monolayers with calculated exfoliation energy as low as 0.39 J/m2 stemming from the ionic feature of the metal oxide bonds. We predict 51 easily or potentially exfoliable oxide monolayers, including metals and insulators/semiconductors, with intriguing physical properties such as ultra-high κ values, negative Poisson's ratios and large valley spin splitting. Among them, the most promising dielectric, GeO2, exhibits an auxetic effect, a κ value of 99, and forms type-I heterostructures with MoSe2 and HfSe2, with a band offset of ~1 eV. Our study opens the way for designing nonlayered 2D oxides, offering a platform for studying the rich physics in ultra-thin oxides and their potential applications in future information technologies.

Overcoming losses in superlenses with synthetic waves of complex frequency.

Superlenses made of plasmonic materials and metamaterials can image features at the subdiffraction scale. However, intrinsic losses impose a serious restriction on imaging resolution, a problem that has hindered widespread applications of superlenses. Optical waves of complex frequency that exhibit a temporally attenuating behavior have been proposed to offset the intrinsic losses in superlenses through the introduction of virtual gain, but experimental realization has been lacking because of the difficulty of imaging measurements with temporal decay. In this work, we present a multifrequency approach to constructing synthetic excitation waves of complex frequency based on measurements at real frequencies. This approach allows us to implement virtual gain experimentally and observe deep-subwavelength images. Our work offers a practical solution to overcome the intrinsic losses of plasmonic systems for imaging and sensing applications.

Transmission/reflection behaviors of surface plasmons at an interface between two plasmonic systems.

Although surface plasmon polaritons (SPPs) have been intensively studied in past years, the transmission/reflection properties of SPPs at an interface between two plasmonic media are still not fully understood. In this article, we employ a mode expansion method (MEM) to systematically study such a problem based on a model system jointing two superlattices, each consisting of a periodic stacking of dielectric and plasmonic slabs with different material properties. Such a generic model can represent two widely used plasmonic structures (i.e. interfaces between two single dielectric/metal systems or between two metal-insulator-metal waveguides) under certain conditions. Our MEM calculations, in excellent agreement with full-wave simulations, uncover the rich physics behind the SPP reflections at generic plasmonic interfaces. In particular, we successfully derive from the MEM several analytical formulas that can quantitatively describe the SPP reflections at different plasmonic interfaces, and show that our formulas exhibit wider applicable regions than previously proposed empirical ones.