CH3NH3SnxPb1-xBr3 hybrid perovskite solid solution: synthesis, structure, and optical properties.

We report the synthesis and characterization of a MASnxPb1-xBr3 (MA = methylammonium; nominal x = 0, 0.2, 0.4, 0.5, 0.6, 0.8, 1) solid solution. The original synthetic method developed allowed one to obtain single-phase materials with homogeneous Sn/Pb distribution. All of the samples prepared are cubic, and the unit cell linearly decreases with increasing x value. The optical response indicates a linear trend (Vegard's law) of the band gap with increasing Sn content from 2.20 eV (x = 0) to 1.33 eV (x = 1), thus extending light absorption into the near-IR.

Low-power continuous-wave generation of visible harmonics in silicon photonic crystal nanocavities.

We present the first demonstration of frequency conversion by simultaneous second- and third-harmonic generation in a silicon photonic crystal nanocavity using continuous-wave optical excitation. We observe a bright dual wavelength emission in the blue/green (450-525 nm) and red (675-790 nm) visible windows with pump powers as low as few microwatts in the telecom bands, with conversion efficiencies of ∼ 10 (-5) /W and ∼ 10/ W(2) for the second- and third-harmonic, respectively. Scaling behaviors as a function of pump power and cavity quality-factor are demonstrated for both second- and third order processes. Successful comparison of measured and calculated emission patterns indicates that third-harmonic is a bulk effect while second-harmonic is a surface-related effect at the sidewall holes boundaries. Our results are promising for obtaining practical low-power, continuous-wave and widely tunable multiple harmonic generation on a silicon chip.

All-optical switching in silicon-on-insulator photonic wire nano-cavities.

We report on experimental demonstration of all-optical switching in a silicon-on-insulator photonic wire nanocavity operating at telecom wavelengths. The switching is performed with a control pulse energy as low as approximately 0.1 pJ on a cavity device that presents very high signal transmission, an ultra-high quality-factor, almost diffraction-limited modal volume and a footprint of only 5 microm(2). High-speed modulation of the cavity mode is achieved by means of optical injection of free carriers using a nanosecond pulsed laser. Experimental results are interpreted by means of finite-difference time-domain simulations. The possibility of using this device as a logic gate is also demonstrated.

Direct measurement of refractive-index dispersion of transparent media by white-light interferometry.

We report on a technique for measuring the refractive indices of nonabsorbing media over a broad spectral range from 0.5 to 5 microm. White-light interferometry based on a double-interferometer system consisting of a fixed Mach-Zehnder interferometer and a Fourier-transform spectrometer is used for direct measurement of the absolute rotation-dependent phase shift induced by an optical element. Refractive index n(lambda) over the whole investigated spectral range is thus obtained directly to an accuracy of 10(-4) without the need for any specific assumption about dispersion. Results for synthetic fused silica are presented and discussed.