Freezing and melting of 3D complex plasma structures under microgravity conditions driven by neutral gas pressure manipulation.

Freezing and melting of large three-dimensional complex plasmas under microgravity conditions is investigated. The neutral gas pressure is used as a control parameter to trigger the phase changes: Complex plasma freezes (melts) by decreasing (increasing) the pressure. The evolution of complex plasma structural properties upon pressure variation is studied. Theoretical estimates allow us to identify the main factors responsible for the observed behavior.

"Zyflex": Next generation plasma chamber for complex plasma research in space.

In this paper, we give a detailed description of a novel plasma chamber-the Zyflex chamber-that has been specifically designed for complex/dusty plasma research under reduced gravitational influence as realized during parabolic flight or aboard the International Space Station. The cylindrical, radio-frequency driven discharge device includes a variety of innovations that, for example, allow us to flexibly adjust plasma parameters and its volume via enhanced plasma generation control and a movable, multi-segmented electrode system. The new complex/dusty plasma research tool also supports, due to its overall increased size compared to former space based complex plasma experiments such as PKE-Nefedov or PK-3 Plus, much larger particle systems. Additionally, it can be operated at much lower neutral gas pressures, thus reducing the damping of particle motion considerably. Beyond the technical description and particle-in-cell simulation based characterization of the plasma vessel, we show sample results from experiments performed with this device in the laboratory as well as during parabolic flights, both of which clearly demonstrate the new quality of complex/dusty plasma research that becomes accessible with this new plasma device.

Long-term evolution of the three-dimensional structure of string-fluid complex plasmas in the PK-4 experiment.

Microparticle suspensions in a polarity-switched discharge plasma of the Plasmakristall-4 facility on board the International Space Station exhibit string-like order. As pointed out in [Phys. Rev. Research 2, 033314 (2020)2643-156410.1103/PhysRevResearch.2.033314], the string-order is subject to evolution on the timescale of minutes at constant gas pressure and constant parameters of polarity switching. We perform a detailed analysis of this evolution using the pair correlations and length spectrum of the string-like clusters (SLCs). Average exponential decay rate of the SLC length spectrum is used as a measure of string order. The analysis shows that the improvement of the string-like order is accompanied by the decrease of the thickness of the microparticle suspension, microparticle number density, and total amount of microparticles in the field of view. This suggests that the observed long-term evolution of the string-like order is caused by the redistribution of the microparticles, which significantly modifies the plasma conditions.

Kinetics of fluid demixing in complex plasmas: role of two-scale interactions.

Using experiments and combining theory and computer simulations, we show that binary complex plasmas are particularly good model systems to study the kinetics of fluid-fluid demixing at the "atomistic" (individual particle) level. The essential parameters of interparticle interactions in complex plasmas, such as the interaction range(s) and degree of nonadditivity, can be varied significantly, which allows systematic investigations of different demixing regimes. The critical role of competition between long-range and short-range interactions at the initial stage of the spinodal decomposition is discussed.

Dust coupling parameter of radio-frequency-discharge complex plasma under microgravity conditions.

Oscillation of particles in a dust crystal formed in a low-pressure radio-frequency gas discharge under microgravity conditions is studied. Analysis of experimental data obtained in our previous study shows that the oscillations are highly isotropic and nearly homogeneous in the bulk of a dust crystal; oscillations of the neighboring particles are significantly correlated. We demonstrate that the standard deviation of the particle radius vector along with the local particle number density fully define the coupling parameter of the particle subsystem. The latter proves to be of the order of 100, which is two orders of magnitude lower than the coupling parameter estimated for the Brownian diffusion of particles with the gas temperature. This means significant kinetic overheating of particles under stationary conditions. A theoretical interpretation of the large amplitude of oscillation implies the increase of particle charge fluctuations in the dust crystal. The theoretical estimates are based on the ionization equation of state for the complex plasma and the equation for the plasma perturbation evolution. They are shown to match the results of experimental data processing. Estimated order of magnitude of the coupling parameter accounts for the existence of the solid-liquid phase transition observed for similar systems in experiments.

Flame propagation in two-dimensional solids: Particle-resolved studies with complex plasmas.

Using two-dimensional (2D) complex plasmas as an experimental model system, particle-resolved studies of flame propagation in classical 2D solids are carried out. Combining experiments, theory, and molecular dynamics simulations, we demonstrate that the mode-coupling instability operating in 2D complex plasmas reveals all essential features of combustion, such as an activated heat release, two-zone structure of the self-similar temperature profile ("flame front"), as well as thermal expansion of the medium and temperature saturation behind the front. The presented results are of relevance for various fields ranging from combustion and thermochemistry, to chemical physics and synthesis of materials.

Density distribution of a dust cloud in three-dimensional complex plasmas.

We propose a method of determination of the dust particle spatial distribution in dust clouds that form in three-dimensional (3D) complex plasmas under microgravity conditions. The method utilizes the data obtained during the 3D scanning of a cloud, and it provides reasonably good accuracy. Based on this method, we investigate the particle density in a dust cloud realized in gas discharge plasma in the PK-3 Plus setup onboard the International Space Station. We find that the treated dust clouds are both anisotropic and inhomogeneous. One can isolate two regimes in which a stationary dust cloud can be observed. At low pressures, the particle density decreases monotonically with the increase of the distance from the discharge center; at higher pressures, the density distribution has a shallow minimum. Regardless of the regime, we detect a cusp of the distribution at the void boundary and a slowly varying density at larger distances (in the foot region). A theoretical interpretation of the obtained results is developed that leads to reasonable estimates of the densities for both the cusp and the foot. The modified ionization equation of state, which allows for violation of the local quasineutrality in the cusp region, predicts the spatial distributions of ion and electron densities to be measured in future experiments.

Plasmakristall-4: New complex (dusty) plasma laboratory on board the International Space Station.

New complex-plasma facility, Plasmakristall-4 (PK-4), has been recently commissioned on board the International Space Station. In complex plasmas, the subsystem of µm-sized microparticles immersed in low-pressure weakly ionized gas-discharge plasmas becomes strongly coupled due to the high (103-104 e) electric charge on the microparticle surface. The microparticle subsystem of complex plasmas is available for the observation at the kinetic level, which makes complex plasmas appropriate for particle-resolved modeling of classical condensed matter phenomena. The main purpose of PK-4 is the investigation of flowing complex plasmas. To generate plasma, PK-4 makes use of a classical dc discharge in a glass tube, whose polarity can be switched with the frequency of the order of 100 Hz. This frequency is high enough not to be felt by the relatively heavy microparticles. The duty cycle of the polarity switching can be also varied allowing to vary the drift velocity of the microparticles and (when necessary) to trap them. The facility is equipped with two videocameras and illumination laser for the microparticle imaging, kaleidoscopic plasma glow observation system and minispectrometer for plasma diagnostics and various microparticle manipulation devices (e.g., powerful manipulation laser). Scientific experiments are programmed in the form of scripts written with the help of specially developed C scripting language libraries. PK-4 is mainly operated from the ground (control center CADMOS in Toulouse, France) with the support of the space station crew. Data recorded during the experiments are later on delivered to the ground on the removable hard disk drives and distributed to participating scientists for the detailed analysis.

Force field inside the void in complex plasmas under microgravity conditions.

Observations of complex plasmas under microgravity conditions onboard the International Space Station performed with the Plasma-Kristall experiment-Nefedov facility are reported. A weak instability of the boundary between the central void (region free of microparticles) and the microparticle cloud is observed at low gas pressures. The instability leads to periodic injections of a relatively small number of particles into the void region (by analogy this effect is called the "trampoline effect"). The trajectories of injected particles are analyzed providing information on the force field inside the void. The experimental results are compared with theory which assumes that the most important forces inside the void are the electric and the ion drag forces. Good agreement is found clearly indicating that under conditions investigated the void formation is caused by the ion drag force.

Electrostatic modes in collisional complex plasmas under microgravity conditions.

A linear dispersion relation in a highly collisional complex plasma, including ion drift, was derived in the light of recent PKE-Nefedov wave experiment performed under microgravity conditions onboard the International Space Station. Two modifications of dust density waves with wave frequencies larger than the dust-neutral collision frequency were obtained. The relevance to the space observations was analyzed and a comparison of theory and observations was made for two different complex plasma domains formed by small and large microparticles. Good qualitative agreement is found between the measurements and the theoretical dispersion relations. This allows a determination of the basic complex plasma parameters.

Nonviscous motion of a slow particle in a dust crystal under microgravity conditions.

Subsonic motion of a large particle moving through the bulk of a dust crystal formed by negatively charged small particles is investigated using the PK-3 Plus laboratory onboard the International Space Station. Tracing the particle trajectories shows that the large particle moves almost freely through the bulk of the plasma crystal, while dust particles move along characteristic α-shaped pathways near the large particle. In the hydrodynamic approximation, we develop a theory of nonviscous dust particle motion about a large particle and calculate particle trajectories. Good agreement with experiment validates our approach.

Fluid-solid phase transitions in three-dimensional complex plasmas under microgravity conditions.

Phase behavior of large three-dimensional (3D) complex plasma systems under microgravity conditions onboard the International Space Station is investigated. The neutral gas pressure is used as a control parameter to trigger phase changes. Detailed analysis of structural properties and evaluation of three different melting-freezing indicators reveal that complex plasmas can exhibit melting by increasing the gas pressure. Theoretical estimates of complex plasma parameters allow us to identify main factors responsible for the observed behavior. The location of phase states of the investigated systems on a relevant equilibrium phase diagram is estimated. Important differences between the melting process of 3D complex plasmas under microgravity conditions and that of flat 2D complex plasma crystals in ground based experiments are discussed.

Dynamics of lane formation in driven binary complex plasmas.

The dynamical onset of lane formation is studied in experiments with binary complex plasmas under microgravity conditions. Small microparticles are driven and penetrate into a cloud of big particles, revealing a strong tendency towards lane formation. The observed time-resolved lane-formation process is in good agreement with computer simulations of a binary Yukawa model with Langevin dynamics. The laning is quantified in terms of the anisotropic scaling index, leading to a universal order parameter for driven systems.

First observation of electrorheological plasmas.

We report the experimental discovery of "electrorheological (ER) complex plasmas," where the control of the interparticle interaction by an externally applied electric field is due to distortion of the Debye spheres that surround microparticles (dust) in a plasma. We show that interactions in ER plasmas under weak ac fields are mathematically equivalent to those in conventional ER fluids. Microgravity experiments, as well as molecular dynamics simulations, show a phase transition from an isotropic to an anisotropic (string) plasma state as the electric field is increased.

Void Closure in Complex Plasmas under Microgravity Conditions.

We describe the first observation of a void closure in complex plasma experiments under microgravity conditions performed with the Plasma-Kristall (PKE-Nefedov) facility on board the International Space Station. The void--a grain-free region in the central part of the discharge where the complex plasma is generated--has been formed under most of the plasma conditions and thought to be an inevitable effect. However, we demonstrate in this Letter that an appropriate tune of the discharge parameters allows the void to close. This experimental achievement along with its theoretical interpretation opens new perspectives in engineering new experiments with large quasi-isotropic void-free complex plasma clouds in microgravity conditions.

Critical point in complex plasmas.

The occurrence of liquid-vapor phase transition and the possible existence of a critical point in complex plasmas--systems that consist of charged micrograins in a neutralizing plasma background--is investigated theoretically. An analysis based on the consideration of the intergrain interaction potential suggests that under certain conditions systems near and at the critical point should be observable. Measurements under microgravity conditions would appear to be required. The analysis aims at determining the plasma parameter regime most suitable for planned experimental investigations.

Application of a forward-angle-scattering transmissometer for simultaneous measurements of particle size and number density in an optically dense medium.

We consider the multiple-scattering and forward-scattering corrections to the transmission measurements in the case of a detector with a variable field of view. The transmission functions for predicting the angular distribution of forward-scattering transmittance are proposed. We present results of measurements of transmission functions for polystyrene spheres. Numerical estimations of the forward-multiple-scattering corrections are in good agreement with the experimental results.

Decharging of complex plasmas: first kinetic observations.

The first experiment on the decharging of a complex plasma in microgravity conditions was conducted. After switching off the rf power, in the afterglow plasma, ions and electrons rapidly recombine and leave a cloud of charged microparticles. Because of microgravity, the particles remain suspended in the experimental chamber for a sufficiently long time, allowing precise measurements of the rest particle charge. A simple theoretical model for the decharging is proposed which agrees quite well with the experiment results and predicts the rest charge at lower gas pressures.

Transport of microparticles in weakly ionized gas-discharge plasmas under microgravity conditions.

Measurements of effective structural (pair correlation function) and transport (diffusion constant) characteristics of the system of microparticles in dc and rf gas-discharge plasmas under microgravity conditions are reported. The comparison between these measurements and numerical simulations is used for complex plasma diagnostics.