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Employing a second-quantization of the electromagnetic field in the presence of media with both gain and loss, we investigate the propagation of the squeezed coherent state of light through a dispersive non-Hermitian multilayered structure, in particular at a discrete set of frequencies for which this structure is PT-symmetric. We detail and generalize this study to cover various angles of incidence and s- and p-polarizations to reveal how dispersion, gain/loss-induced noises in such multilayered structures affect nonclassical properties of the incident light, such as squeezing and sub-Poissonian statistics. Varying the loss layers' coefficient, we demonstrate a squeezed coherent state, when transmits through the structure whose gain and loss layers have unidentical bulk permittivities, retains its nonclassical features to some extent. Our results show by increasing the number of unit cells and incident angle, the quantum features of the transmitted state for both polarizations degrade.
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The presence of species other than the target biomolecules in the fluidic analyte used in the refractive index biosensor based on the surface plasmon resonances (SPRs) can lead to measurement ambiguity. Using graphene-based acousto-plasmonic biosensors, we propose two methods to eliminate any possible ambiguity in interpreting the measured results. First, we take advantage of the dynamic tunability of graphene SPRs in the acousto-plasmonic biosensor with a surface acoustic wave (SAW) induced uniform grating, performing measurements at different applied voltages. Second, a single measurement employing a similar biosensor but with SAW-induced dual-segment gratings. The numerical results show the capability of both methods in decoupling the effect of the target analyte from the other species in the fluid, enabling interpreting the measurement results with no ambiguity. We also report the results of our numerical investigation on the effect of measuring parameters like the target layer effective refractive index and thickness, and the fluid effective refractive index, in addition to the controlling parameters of the proposed acousto-plasmonic biosensor, including graphene Fermi energy and electrical signaling on the sensing characteristics. Both types of proposed biosensors show promising features for developing the next generation lab-on-a-chip biosensors with minimal cross-sensitivities to non-target biomolecules.
Assuntos
Técnicas Biossensoriais , Grafite , Técnicas Biossensoriais/métodos , Meios de Cultura , Refratometria , Ressonância de Plasmônio de SuperfícieRESUMO
We propose investigating the electro-optical properties of photodetectors based on mono- and bilayer graphene quantum dots or nanodots (GNDs). These photodetectors consist of dissimilar metals (gold, silver and titanium) that are in contact with the GNDs. To obtain photoelectrical characteristics, we employed density functional theory to solve the non-equilibrium Green's function. Photo-responsivities and quantum efficiencies obtained for these nanostructures were far better than those for structures based on graphene nanoribbons. Among the proposed photodetectors, the best performance belonged to the bilayer structures illuminated by in-plane polarized incident light. The proposed photodetectors operate without a need for externally applied voltage and are suitable for parallel light propagation using directional couplers based on the evanescent field of incident light; hence, they have applications in optical integrated circuits.
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Taking advantage of highly confined evanescent fields to overcome the free-space diffraction limit, we show plasmonic tweezers enable efficient trapping and manipulation of nanometric particles by low optical powers. In typical plasmonic tweezers, trapping/releasing particles is carried out by turning the laser power on and off, which cannot be achieved quickly and repeatedly during the experiment. We introduce hybrid gold-graphene plasmonic tweezers in which the trap stiffness is varied electrostatically by applying suitable voltages to a graphene layer. We show how the graphene layer absorbs the plasmonic field around the gold nanostructures in particular chemical potentials, allowing us to modulate the plasmonic force components and the trapping potential. We show graphene monolayer (bilayer) with excellent thermal properties enables more efficient heat transfer throughout the plasmonic tweezers, reducing the magnitude of thermophoretic force by about 23 (36) times. This thermophoresis suppression eliminates the risk of photothermal damage to the target sample. Our proposed plasmonic tweezers open up possibilities to develop tunable plasmonic tweezers with high-speed and versatile force-switching functionality and more efficient thermal performance.
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Intrinsic optical phonons and extrinsic polar optical phonons (POPs) strongly affect the graphene surface plasmons. Specifically, extraneous POPs present on the surface of an underlying substrate change the behavior of the graphene's surface plasmons sharply due to the plasmon-phonon hybridization. Here, we report modeling of exact dispersion relations for graphene's surface plasmons affected by intrinsic optical phonons and extrinsic POPs of the surface of polar dielectric substrates with one or more vibrational frequencies. In doing so, we have employed random phase approximation with modified two-dimensional polarizability (2D-Π0). The adapted Π0 addresses limitations of the previously derived plasmons dispersion, obtained using classical two-dimensional polarizability. We show the new model overcomes the unsatisfying behavior of the plasmonic dispersion relation obtained by the classical 2D-Π0 at high-wavenumbers and its inability to indicate the starting point of the mode damping. Our new simple model eliminates the complexity of the other presented models in describing the surface plasmons' behavior, specifically at high wavenumbers. Besides, we use our dispersion model to learn about the plasmon content of the hybrid modes, which is a vital value to compute output current in plasmonic graphene-based devices. The coupled-mode lifetime due to the hybrid nature depends on both plasmon and phonon lifetimes. We capture this value here. There is an excellent agreement between our theoretical results and the experimental data reported earlier. They pave the way for the exact modeling of graphene plasmons on common polar substrates and bring in the closeness of the theoretical approaches and experimental results.
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Using a plasmonic graphene ring resonator of resonant frequency 10.38 THz coupled to a plasmonic graphene waveguide, we design a lab-on-a-chip optophoresis system that can function as an efficient plasmonic force switch. Finite difference time domain numerical simulations reveal that an appropriate choice of chemical potentials of the waveguide and ring resonator keeps the proposed structure in on-resonance condition, enabling the system to selectively trap a nanoparticle. Moreover, a change of 250 meV in the ring chemical potential (i.e., equivalent to 2.029 V change in the corresponding applied bias) switches the structure to a nearly perfect off-resonance condition, releasing the trapped particle. The equivalent plasmonic switch ON/OFF ratio at the waveguide output is -15.519 dB. The designed system has the capability of trapping, sorting, controlling, and separating PS nanoparticles of diameters ≥30 nm with a THz source intensity of 14.78 mW/µm2 and ≥22 nm with 29.33 mW/µm2.
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We present theoretical and experimental studies of the plasmonic properties of hexagonal arrays of gold triangles, fabricated by angle-resolved nanosphere lithography method. Our numerical and experimental results both show that a change in the angle of gold deposition affects the size and the distance between the triangles, leading to a controlled shift in their absorption and scattering spectra. We calculate the force exerted on the polystyrene particles of 650 nm radii numerically while passing above the hexagonal arrays. Simulation results show that the presented hexagonal arrays of gold triangles can operate as efficient plasmonic tweezers with a controllable operating wavelength and high trap strength, owing to the additive interaction of the neighboring triangles. Moreover, we apply the realized plasmonic nanostructures in a conventional optical tweezers configuration and show that the optical tweezers stiffness can be effectively modulated by the plasmonic forces, at the IR wavelength of 1064 nm.
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Unique properties of lead chalcogenides have enabled multiple exciton generation (MEG) in their nanocrystals that can be beneficial in enhancing the efficiency of third-generation solar cells. Although the intrinsic electric field plays an imperative role in a solar cell, its effect on the multiple exciton generation (MEG) has been overlooked, so far. Using EOM-CCSD as a many-body approach, we show that any electric field can affect the absorptivity spectra of the lead chalcogenide nanocrystals (Pb4 Te4 , Pb4 Se4 , and Pb4 S4 ). The same electric field, however, has insignificant effects on the MEG quantum probabilities and the thresholds in these nanocrystals. Furthermore, simulations show that Pb4 Te4 , among the aforementioned nanocrystals, has the lowest MEG threshold and the strongest absorptivity peak that is located in the multi-excitation window, irrespective of the field strength, making it the most suitable candidate for MEG applications. Simulations also demonstrate that an electric field affects the MEG characteristics in the Pb4 Te4 nanocrystal, in general, less than it perturbs MEG characteristics in Pb4 Se4 and Pb4 S4 nanocrystals. Our results can have a great impact in designing optoelectronic devices whose performance can be significantly influenced by MEG.
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We numerically investigate and design a compact electrically pumped edge-emitting photonic crystal waveguide (PCW) quantum dot (QD) laser operating at room temperature. Use of a narrowband folded directional coupler as the output mirror has made the proposed structure an edge-emitting single-mode laser. Moreover, we propose a set of rate equations to model the performance of the PCW-QD laser. In the proposed model, we take the effects of the homogeneous and inhomogeneous broadenings and the slow-light effects on the modal gain and loss coefficient into account. Simulations show that threshold current as low as â¼26 µA can be achieved for the PCW-QD laser with a 50-µm-long cavity and output power in the range of micro-watts. The proposed low-threshold edge-emitting PCW-QD laser is a promising light source for the off-chip and on-chip photonic network applications.
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A new generation unbiased antennaless CW terahertz (THz) photomixer emitters array made of asymmetric metal-semiconductor-metal (MSM) gratings with a subwavelength pitch, operating in the optical near-field regime, is proposed. We take advantage of size effects in near-field optics and electrostatics to demonstrate the possibility of enhancing the THz power by 4 orders of magnitude, compared to a similar unbiased antennaless array of the same size that operates in the far-field regime. We show that, with the appropriate choice of grating parameters in such THz sources, the first plasmonic resonant cavity mode in the nanoslit between two adjacent MSMs can enhance the optical near-field absorption and, hence, the generation of photocarriers under the slit in the active medium. These photocarriers, on the other hand, are accelerated by the large built-in electric field sustained under the nanoslits by two dissimilar Schottky barriers to create the desired large THz power that is mainly radiated downward. The proposed structure can be tuned in a broadband frequency range of 0.1-3 THz, with output power increasing with frequency.
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We are introducing a new bias free CW terahertz photomixer emitter array. Each emitter consists of an asymmetric metal-semiconductor-metal (MSM) that is made of two side by side dis-similar Schottky contacts, on a thin layer of low temperature grown (LTG) GaAs, with barrier heights of difference (ΔΦ(B)) and a finite lateral spacing (s). Simulations show that when an appropriately designed structure is irradiated by two coherent optical beams of different center wavelengths, whose frequency difference (∆f) falls in a desired THz band, the built-in field between the two dis-similar potential barriers can accelerate the photogenerated carriers that are modulated by ∆ω, making each pitch in the array to act as a CW THz emitter, effectively. We also show the permissible values of s and ΔΦ(B) pairs, for which the strengths of the built-in electric field maxima fall below that of the critical of 50 V/µm- i.e., the breakdown limit for the LTG-GaAs layer. Moreover, we calculate the THz radiation power per emitter in an array. Among many potential applications for these bias free THz emitters their use in endoscopic imaging without a need for hazardous external biasing circuitry that reduces the patient health risk, could be the most important one. A hybrid numerical simulation method is used to design an optimum emitter pitch, radiating at 0.5 THz.
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We propose a nanostructured hyperbolic metamaterial (HMM) that can make the transition between elliptic and hyperbolic regimes in the near infrared (IR) frequency range. This switchable HMM is a slab made of a periodic stack of metal/Al(2)O(3)/graphene/Al(2)O(3)/metal nano-layers. By tuning the graphene conductivity via tuning its chemical potential, through a variable external bias, the response of this highly anisotropic medium to a monochromatic TM incident light can be switched between a positive/negative refraction regime and a negative refraction/no-transmission regime. The proposed structure is suitable for applications such as beam splitters, modulators, four-port devices, and optical gates.
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Using numerical analysis, we compare the results of optofluidic and rod filling techniques for the broadening of supercontinuum spectra generated by As2Se3 chalcogenide photonic crystal fibers (PCFs). The numerical results show that when air-holes constituting the innermost ring in a PCF made of As2Se3-based chalcogenide glass are filled with rods of As2Se3-based chalcogenide glass, over a wide range of mid-IR wavelengths, an ultra-flattened near-zero dispersion can be obtained, while the total loss is negligible and the PCF nonlinearity is very high. The simulations also show that when a 50 fs input optical pulse of 10 kW peak power and center wavelength of 4.6 µm is launched into a 50 mm long rod-filled chalcogenide PCF, a ripple-free spectral broadening as wide as 3.86 µm can be obtained.
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To examine the second-order coherence of light propagation of quantum states in arbitrary directions through dispersive non-Hermitian optical media, we considered two sets of non-Hermitian periodic structures that consist of gain/loss unit cells. We show that each batch can satisfy the parity-time symmetry conditions at a distinct frequency. We then varied the gain/loss strength in the stable electromagnetic regime to evaluate the transmittance of N-photon number states through each structure. The results show both sets preserve their antibunching characteristics under specific incident light conditions. Furthermore, s(p)-polarized light exhibits higher (lower) second-order coherence at larger incident angles. In addition, the antibunching features of the transmitted states degrade with an increase in the number of unit cells in multilayered structures for both polarizations.
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We propose a photodetector (PD) based on the internal photoemission effect over a Schottky barrier on a CMOS-compatible Si microring resonator for 1.55 µm. To analyze the device, we model the microring waveguide partially covered by a metal/silicide nanolayer, using the Z-transform method. The proposed structure benefits from the resonant-cavity-enhanced (RCE) waveguide PDs enjoying high efficiency and wavelength selectivity. Simulations show that the maximum value of the bandwidth-efficiency product for the proposed structure is in the order of 10 GHz, which is much higher than those reported for other RCE-based PDs.
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We present the design procedure for an ultracompact low-power all-optical modulator based on a dispersion-engineered slow-light regime in a photonic crystal Mach-Zehnder interferometer (PhC MZI), selectively infiltrated by nonlinear optical fluids. The dispersionless slow-light regime enhancing the nonlinearities enabled a 22 µm long PhC MZI to operate as a modulator with an input power as low as 3 mW/µm. Simulations reveal that the switching threshold can be controlled by varying the optofluidic infiltration.
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We propose a metasurface THz modulator based on split-ring resonators (SRRs) formed by four interconnected horizontal Si-Au Schottky diodes. The equivalent junction capacitance of each SRR in the proposed modulator is much smaller than that of the previously reported metasurface counterparts with vertical Schottky junctions, leading to a higher modulation speed. To modulate a THz incident signal by the proposed metasurface, we vary the bias voltage externally applied to the Schottky junctions. Applying a reverse bias of VA = - 5 V to the Au gate, two LC resonances at 0.48 THz, and 0.95 THz are excited in the metasurface. Switching the applied voltage to VA = + 0.49 V, we diminish the oscillator strengths of the LC resonances, creating one dipole resonance at 0.73 THz in the transmission spectrum of the metasurface modulator. The modulation depths at these resonances are more than 45%, reaching 87% at 0.95 THz. The phase modulation for this THz modulator is about 1.12 rad at 0.86 THz. Furthermore, due to the particular design of the meta-atoms, the modulation speed of this device is estimated up to approximately several hundred GHz, which makes this device an appropriate candidate for high-speed applications in wireless communications systems based on external modulators.
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All-optical communication systems are under continuous development to address different core elements of inconvenience. Here, we numerically investigate an all-optical modulator, realizing a highly efficient modulation depth of 22 dB and a low insertion loss of 0.32 dB. The tunable optical element of the proposed modulator is a layer of Al-doped Zinc Oxide (AZO), also known as an epsilon-near-zero transparent conductive oxide. Sandwiching the AZO layer between a carefully designed distributed Bragg reflector and a dielectric metasurface-i.e., composed of a two-dimensional periodic array of cubic Si-provides a guided-mode resonance at the OFF state of the modulator, preventing the incident signal reflection at λ = 1310 nm. We demonstrate the required pump fluence for switching between the ON/OFF states of the designed modulator is about a few milli-Joules per cm2. The unique properties of the AZO layer, along with the engineered dielectric metasurface above it, change the reflection from 1 to 93%, helping design better experimental configurations for the next-generation all-optical communication systems.
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Surface plasmons in graphene have mainly been affected by intrinsic optical phonons due to the vibrations of the carbon atoms and surface polar optical phonons (S-POPs) of the underlying dielectric surface. This plasmon hybridization dramatically changes the features of the plasmonic devices. However, a complete theoretical model for the graphene impedance to consider the optical phonons effects is yet remained to be developed. Here, we show how to derive a model for graphene impedance to include such impacts on graphene surface plasmons. Earlier models suffer from two limitations-i.e., the inability to show (i) the transformation of a single pure plasmonic mode into multiple hybrid plasmon-phonon excitations and (ii) the damping effect for energies beyond that of the intrinsic optical phonons due to the phonon emission. Our new model overcomes these two limitations. Then, we calculate the extinction spectra for a one-dimensional periodic array of graphene ribbons obtained through the impedance boundary condition method, addressing these obstacles. These spectra are directly related to graphene impedance, modeled using the dielectric function we developed in our earlier work. The extinction spectra show the presented model overcoming the limitations, firmly fitting the experimental data reported by others. Furthermore, we introduce our developed model for graphene to the CST Studio software to verify the accuracy of our extinction relation and impedance model. This study can be a step forward correctly predicting the behavior of graphene-based plasmonic devices.