Spatio-spectral couplings in optical parametric amplifiers.

Optical parametric amplification (OPA) is a powerful tool for the generation of ultrashort light pulses. However, under certain circumstances, it develops spatio-spectral couplings, color dependent aberrations that degrade the pulse properties. In this work, we present a spatio-spectral coupling generated by a non-collimated pump beam and resulting in the change of direction of the amplified signal with respect to the input seed. We experimentally characterize the effect, introduce a theoretical model to explain it as well as reproduce it through numerical simulations. It affects high-gain non-collinear OPA configurations and becomes especially relevant in sequential optical parametric synthesizers. In collinear configuration, however, beyond the direction change, also angular and spatial chirp is produced. We obtain with a synthesizer about 40% decrease in peak intensity in the experiments and local elongation of the pulse duration by more than 25% within the spatial full width at half maximum at the focus. Finally, we present strategies to correct or mitigate the coupling and demonstrate them in two different systems. Our work is important for the development of OPA-based systems as well as few-cycle sequential synthesizers.

Saturation control of an optical parametric chirped-pulse amplifier.

Optical parametric chirped-pulse amplification (OPCPA) is a light amplification technique that provides the combination of broad spectral gain bandwidth and large energy, directly supporting few-cycle pulses with multi-terawatt (TW) peak powers. Saturation in an OPCPA increases the stability and conversion efficiency of the system. However, distinct spectral components experience different gain and do not saturate under the same conditions, which reduces performance. Here, we describe a simple and robust approach to control the saturation for all spectral components. The demonstrated optimal saturation increases the overall gain, conversion efficiency and spectral bandwidth. We experimentally obtain an improvement of the pulse energy by more than 18%. This technique is easily implemented in any existing OPCPA system with a pulse shaper to maximize its output.

Dispersion control for temporal contrast optimization.

We investigate the temporal contrast of the Light Wave Synthesizer 20 (LWS-20): a powerful, few-cycle source based on the optical parametric synthesizer principle. Saturation effects in the RF amplifier driving the acousto-optic programmable dispersive filter (AOPDF) were found to degrade the coherent contrast for non-monotonic group delay corrections. We subsequently present a new dispersion scheme and design a novel transmission grism-based stretcher optimized for LWS-20. The resulting temporal contrast of the amplified, compressed output pulses is improved by 2-4 orders of magnitude compared to the former design.