Electrically Driven Reprogrammable Vanadium Dioxide Metasurface Using Binary Control for Broadband Beam Steering.

Resonant optical phased arrays are a promising way to reach fully reconfigurable metasurfaces in the optical and near-infrared (NIR) regimes with low energy consumption, low footprint, and high reliability. Continuously tunable resonant structures suffer from inherent drawbacks such as low phase range, amplitude-phase correlation, or extreme sensitivity that makes precise control at the individual element level very challenging. We computationally investigate 1-bit (binary) control as a mechanism to bypass these issues. We consider a metasurface for beam steering using a nanoresonator antenna and explore the theoretical capabilities of such phased arrays. A thermally realistic structure based on vanadium dioxide sandwiched in a metal-insulator-metal structure is proposed and optimized using inverse design to enhance its performance at 1550 nm. Continuous beam steering over 90° range is successfully achieved using binary control, with excellent agreement with predictions based on the theoretical first-principles description of phased arrays. Furthermore, a broadband response from 1500 to 1700 nm is achieved. The robustness to the design manufacturing imperfections is also demonstrated. This simplified approach can be implemented to optimize tunable nanophotonic phased array metasurfaces based on other materials or phased shifting mechanisms for various functionalities.

Synergetic Transparent Electrode Architecture for Efficient Non-Fullerene Flexible Organic Solar Cells with >12% Efficiency.

Flexible organic solar cells (OSCs) are considered one key component in wearable, intelligent electronics due to the unique capacity for highly flexible renewable energy sources. However, it is urgently required to enhance their efficiency, as it is far inferior to that of their conventional, glass-based counterparts. To boost the performance of flexible OSCs on plastic substrates, we here present a synergetic transparent electrode structure, which combines electrically conductive silver nanowires, a sol-gel-derived ZnO planarization layer, and imprinted light-trapping nanostructures. This synergetic composite electrode exhibits good properties in terms of optical transparency, electrical conductivity, mechanical flexibility, and low-temperature processability. As a result, the single-junction non-fullerene-based flexible OSCs achieve a power conversion efficiency exceeding 12% due to the synergetic interplay between broadband light trapping and suppressed charge recombination loss. Moreover, these flexible OSCs are repeatedly bendable in both inward and outward bending directions, retaining over 60% of the initial efficiency after 1000 cycles of the bending test at a 3.0 mm radius. These results convey a clear depiction of the practicality of flexible OSCs in a variety of high-performance flexible applications.