Quantum Phases from Competing Van der Waals and Dipole-Dipole Interactions of Rydberg Atoms.

Competing short- and long-range interactions represent distinguished ingredients for the formation of complex quantum many-body phases. Their study is hard to realize with conventional quantum simulators. In this regard, Rydberg atoms provide an exception as their excited manifold of states have both density-density and exchange interactions whose strength and range can vary considerably. Focusing on one-dimensional systems, we leverage the Van der Waals and dipole-dipole interactions of the Rydberg atoms to obtain the zero-temperature phase diagram for a uniform chain and a dimer model. For the uniform chain, we can influence the boundaries between ordered phases and a Luttinger liquid phase. For the dimerized case, a new type of bond-order-density-wave phase is identified. This demonstrates the versatility of the Rydberg platform in studying physics involving short- and long-ranged interactions simultaneously.

Synthetic Dimension-Induced Conical Intersections in Rydberg Molecules.

We observe a series of conical intersections in the potential energy curves governing both the collision between a Rydberg atom and a ground-state atom and the structure of Rydberg molecules. By employing the electronic energy of the Rydberg atom as a synthetic dimension we circumvent the von Neumann-Wigner theorem. These conical intersections can occur when the Rydberg atom's quantum defect is similar in size to the electron-ground-state atom scattering phase shift divided by π, a condition satisfied in several commonly studied atomic species. The conical intersections have an observable consequence in the rate of ultracold l-changing collisions of the type Rb(nf)+Rb(5s)→Rb(nl>3)+Rb(5s). In the vicinity of a conical intersection, this rate is strongly suppressed, and the Rydberg atom becomes nearly transparent to the ground-state atom.

Entangling Lattice-Trapped Bosons with a Free Impurity: Impact on Stationary and Dynamical Properties.

We address the interplay of few lattice trapped bosons interacting with an impurity atom in a box potential. For the ground state, a classification is performed based on the fidelity allowing to quantify the susceptibility of the composite system to structural changes due to the intercomponent coupling. We analyze the overall response at the many-body level and contrast it to the single-particle level. By inspecting different entropy measures we capture the degree of entanglement and intraspecies correlations for a wide range of intra- and intercomponent interactions and lattice depths. We also spatially resolve the imprint of the entanglement on the one- and two-body density distributions showcasing that it accelerates the phase separation process or acts against spatial localization for repulsive and attractive intercomponent interactions, respectively. The many-body effects on the tunneling dynamics of the individual components, resulting from their counterflow, are also discussed. The tunneling period of the impurity is very sensitive to the value of the impurity-medium coupling due to its effective dressing by the few-body medium. Our work provides implications for engineering localized structures in correlated impurity settings using species selective optical potentials.

Compact localized states of open scattering media: a graph decomposition approach for an ab initio design.

We study the compact localized scattering resonances of periodic and aperiodic chains of dipolar nanoparticles by combining the powerful equitable partition theorem (EPT) of a graph theory with the spectral dyadic Green's matrix formalism for the engineering of embedded quasi-modes in non-Hermitian open scattering systems in three spatial dimensions. We provide the analytical and numerical design of the spectral properties of compact localized states in electromagnetically coupled chains and establish a connection with the distinctive behavior of bound states in the continuum. Our results extend the concept of compact localization to the scattering resonances of open systems with an arbitrary aperiodic order beyond tight-binding models, and are relevant for the efficient design of novel photonic and plasmonic metamaterial architectures for enhanced light-matter interaction.

Effective Three-Body Interactions in Cs(6s)-Cs(nd) Rydberg Trimers.

Ultralong-range Rydberg trimer molecules are spectroscopically observed in an ultracold gas of Cs(nd_{3/2}) atoms. The anisotropy of the atomic Rydberg state allows for the formation of angular trimers, whose energies may not be obtained from integer multiples of dimer energies. These nonadditive trimers coexist with Rydberg dimers. The existence of such effective three-body interactions is confirmed with the observation of asymmetric line profiles and interpreted by a theoretical approach that includes relativistic spin interactions. Simulations of the observed spectra with and without angular trimer lines lend convincing support to the existence of effective three-body interactions.

Edge modes of scattering chains with aperiodic order.

We study the scattering resonances of one-dimensional deterministic aperiodic chains of electric dipoles using the vectorial Green's matrix method, which accounts for both short- and long-range electromagnetic interactions in open scattering systems. We discover the existence of edge-localized scattering states within fractal energy gaps with characteristic topological band structures. Notably, we report and characterize edge-localized modes in the classical wave analogues of the Su-Schrieffer-Heeger (SSH) dimer model, quasiperiodic Harper and Fibonacci crystals, as well as in more complex Thue-Morse aperiodic systems. Our study demonstrates that topological edge-modes with characteristic power-law envelope appear in open aperiodic systems and coexist with traditional exponentially localized ones. Our results extend the concept of topological states to the scattering resonances of complex open systems with aperiodic order, thus providing an important step towards the predictive design of topological optical metamaterials and devices beyond tight-binding models.

Simultaneous Control of Multispecies Particle Transport and Segregation in Driven Lattices.

We provide a generic scheme to separate the particles of a mixture by their physical properties like mass, friction, or size. The scheme employs a periodically shaken two-dimensional dissipative lattice and hinges on a simultaneous transport of particles in species-specific directions. This selective transport is achieved by controlling the late-time nonlinear particle dynamics, via the attractors embedded in the phase space and their bifurcations. To illustrate the spectrum of possible applications of the scheme, we exemplarily demonstrate the separation of polydisperse colloids and mixtures of cold thermal alkali atoms in optical lattices.

Highly excited electronic image states of metallic nanorings.

We study electronic image states around a metallic nanoring and show that the interplay between the attractive polarization force and a repulsive centrifugal force gives rise to Rydberg-like image states trapped several nanometers away from the surface. The nanoring is modeled as a perfectly conducting isolated torus whose classical electrostatic image potential is derived analytically. The image states are computed via a two-dimensional finite-difference scheme as solutions of the effective Schrödinger equation describing the outer electron subject to this image potential. These findings demonstrate not only the existence of detached image states around nanorings but allow us also to provide general criteria on the ring geometry, i.e., the aspect ratio of the torus, that need to be fulfilled in order to support such states.

Diffusion and transport in locally disordered driven lattices.

We study the effect of disorder on the particle density evolution in a classical Hamiltonian driven lattice setup. If the disorder is localized within a finite sub-domain of the lattice, the emergence of strong tails in the density distribution which even increases towards larger positions is shown, thus yielding a highly non-Gaussian particle density evolution. As the key underlying mechanism, we identify the conversion between different components of the unperturbed systems mixed phase space which is induced by the disorder. Based on the introduction of individual conversion rates between chaotic and regular components, a theoretical model is developed which correctly predicts the scaling of the particle density. The effect of disorder on the transport properties is studied where a significant enhancement of the transport for cases of localized disorder is shown, thereby contrasting strongly the merely weak modification of the transport for global disorder.

Spatiotemporal oscillation patterns in the collective relaxation dynamics of interacting particles in periodic potentials.

We demonstrate the emergence of self-organized structures in the course of the relaxation of an initially excited, dissipative, and finite chain of interacting particles in a periodic potential towards its many particle equilibrium configuration. Specifically, we observe a transition from an in phase correlated motion via phase randomized oscillations towards oscillations with a phase difference π between adjacent particles thereby yielding the growth of long time transient spatiotemporal oscillation patterns. Parameter modifications allow for designing these patterns, including steady states and even states that combine in phase and correlated out of phase oscillations along the chain. The complex relaxation dynamics is based on finite size effects together with an evolution running from the nonlinear to the linear regime, thereby providing a highly unbalanced population of the center-of-mass and relative motion.

Disorder induced regular dynamics in oscillating lattices.

We explore the impact of weak disorder on the dynamics of classical particles in a periodically oscillating lattice. It is demonstrated that the disorder induces a hopping process from diffusive to regular motion; i.e., we observe the counterintuitive phenomenon that disorder leads to regular behavior. If the disorder is localized in a finite-sized part of the lattice, the described hopping causes initially diffusive particles to even accumulate in regular structures of the corresponding phase space. A hallmark of this accumulation is the emergence of pronounced peaks in the velocity distribution of particles that should be detectable in state of the art experiments, e.g., with cold atoms in optical lattices.

Equilibria and dynamics of two coupled chains of interacting dipoles.

We explore the energy transfer dynamics in an array of two chains of identical rigid interacting dipoles. Varying the distance b between the two chains of the array, a crossover between two different ground-state (GS) equilibrium configurations is observed. Linearizing around the GS configurations, we verify that interactions up to third nearest neighbors should be accounted to accurately describe the resulting dynamics. Starting with one of the GS, we excite the system by supplying it with an excess energy ΔK located initially on one of the dipoles. We study the time evolution of the array for different values of the system parameters b and ΔK. Our focus is hereby on two features of the energy propagation: the redistribution of the excess energy ΔK among the two chains and the energy localization along each chain. For typical parameter values, the array of dipoles reaches both the equipartition between the chains and the thermal equilibrium from the early stages of the time evolution. Nevertheless, there is a region in parameter space (b,ΔK) where even up to the long computation time of this study, the array does neither reach energy equipartition nor thermalization between chains. This fact is due to the existence of persistent chaotic breathers.

The multi-layer multi-configuration time-dependent Hartree method for bosons: theory, implementation, and applications.

We develop the multi-layer multi-configuration time-dependent Hartree method for bosons (ML-MCTDHB), a variational numerically exact ab initio method for studying the quantum dynamics and stationary properties of general bosonic systems. ML-MCTDHB takes advantage of the permutation symmetry of identical bosons, which allows for investigations of the quantum dynamics from few to many-body systems. Moreover, the multi-layer feature enables ML-MCTDHB to describe mixed bosonic systems consisting of arbitrary many species. Multi-dimensional as well as mixed-dimensional systems can be accurately and efficiently simulated via the multi-layer expansion scheme. We provide a detailed account of the underlying theory and the corresponding implementation. We also demonstrate the superior performance by applying the method to the tunneling dynamics of bosonic ensembles in a one-dimensional double well potential, where a single-species bosonic ensemble of various correlation strengths and a weakly interacting two-species bosonic ensemble are considered.

Evolution of discrete symmetries.

Symmetries are known to dictate important physical properties and can be used as a design principle in particular in wave physics, including wave structures and the resulting propagation dynamics. Local symmetries, in the sense of a symmetry that holds only in a finite domain of space, can be either the result of a self-organization process or a structural ingredient into a synthetically prepared physical system. Applying local symmetry operations to extend a given finite chain we show that the resulting one-dimensional lattice consists of a transient followed by a subsequent periodic behavior. Due to the fact that, by construction, the implanted local symmetries strongly overlap the resulting lattice possesses a dense skeleton of such symmetries. We proof this behavior on the basis of a class of local symmetry operations allowing us to conclude upon the "asymptotic" properties such as the final period, decomposition of the unit cell and the length and appearance of the transient. As an example case, we explore the corresponding tight-binding Hamiltonians. Their energy eigenvalue spectra and eigenstates are analyzed in some detail, showing in particular the strong variability of the localization properties of the eigenstates due to the presence of a plethora of local symmetries.

Characterizing a transition from limited to unlimited diffusion in energy for a time-dependent stochastic billiard.

We explore Fermi acceleration in a stochastic oval billiard which shows unlimited to limited diffusion in energy when passing from the free to the dissipative case. We provide evidence for a transition from limited to unlimited energy growth taking place while detuning the corresponding restitution coefficient responsible for the degree of dissipation. A corresponding order parameter is suggested, and its susceptibility is shown to diverge at the critical point. We show that this order parameter is also be applicable to the periodically driven oval billiard and discuss the elementary excitation of the controlled diffusion process.

Construction of analytical many-body wave functions for correlated bosons in a harmonic trap.

We develop an analytical many-body wave function to accurately describe the crossover of a one-dimensional bosonic system from weak to strong interactions in a harmonic trap. The explicit wave function, which is based on the exact two-body states, consists of symmetric multiple products of the corresponding parabolic cylinder functions and respects the analytically known limits of zero and infinite repulsion for arbitrary number of particles. For intermediate interaction strengths we demonstrate that the energies, as well as the reduced densities of first and second order, are in excellent agreement with large scale numerical calculations.

Chaos and thermalization in a classical chain of dipoles.

We explore the connection between chaos, thermalization, and ergodicity in a linear chain of N interacting dipoles. Starting from the ground state, and considering chains of different numbers of dipoles, we introduce single site excitations with excess energy ΔK. The time evolution of the chaoticity of the system and the energy localization along the chain is analyzed by computing, up to a very long time, the statistical average of the finite-time Lyapunov exponent λ(t) and the participation ratio Π(t). For small ΔK, the evolution of λ(t) and Π(t) indicates that the system becomes chaotic at approximately the same time as Π(t) reaches a steady state. For the largest considered values of ΔK the system becomes chaotic at an extremely early stage in comparison with the energy relaxation times. We find that this fact is due to the presence of chaotic breathers that keep the system far from equipartition and ergodicity. Finally, we show numerically and analytically that the asymptotic values attained by the participation ratio Π(t) fairly correspond to thermal equilibrium.

External-field-induced dynamics of a charged particle on a closed helix.

We investigate the dynamics of a charged particle confined to move on a toroidal helix while being driven by an external time-dependent electric field. The underlying phase space is analyzed for linearly and circularly polarized fields. For small driving amplitudes and a linearly polarized field, we find a split up of the chaotic part of the phase space, which prevents the particle from inverting its direction of motion. This allows for a nonzero average velocity of chaotic trajectories without breaking the well-known symmetries commonly responsible for directed transport. Within our chosen normalized units, the resulting average transport velocity is constant and does not change significantly with the driving amplitude. A very similar effect is found in case of the circularly polarized field and low driving amplitudes. Furthermore, when driving with a circularly polarized field, we unravel a second mechanism of the split up of the chaotic phase space region for very large driving amplitudes. There exists a wide range of parameter values for which trajectories may travel between the two chaotic regions by crossing a permeable cantorus. The limitations of these phenomena, as well as their implication on manipulating directed transport in helical geometries are discussed.

Confinement-induced resonances in low-dimensional quantum systems.

We report on the observation of confinement-induced resonances in strongly interacting quantum-gas systems with tunable interactions for one- and two-dimensional geometry. Atom-atom scattering is substantially modified when the s-wave scattering length approaches the length scale associated with the tight transversal confinement, leading to characteristic loss and heating signatures. Upon introducing an anisotropy for the transversal confinement we observe a splitting of the confinement-induced resonance. With increasing anisotropy additional resonances appear. In the limit of a two-dimensional system we find that one resonance persists.

Tunable order of helically confined charges.

We investigate a system of equally charged Coulomb-interacting particles confined to a toroidal helix in the presence of an external electric field. Due to the confinement, the particles experience an effective interaction that oscillates with the particle distance and allows for the existence of stable bound states, despite the purely repulsive character of the Coulomb interaction. We design an order parameter to classify these bound states and use it to identify a structural crossover of the particle order, occurring when the electric field strength is varied. Amorphous particle configurations for a vanishing electric field and crystalline order in the regime of a strong electric field are observed. We study the impact of parameter variations on the particle order and conclude that the crossover occurs for a wide range of parameter values and even holds for different helical systems.