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J Am Soc Mass Spectrom ; 35(9): 2230-2236, 2024 Sep 04.
Artigo em Inglês | MEDLINE | ID: mdl-39092830

RESUMO

The drug discovery process increasingly relies on high-throughput sample analysis to accelerate the identification of viable drug candidates. Recently, chromatographic-free high-throughput mass spectrometry (HT-MS) technologies have emerged, significantly increasing sample readout speed and enabling the analysis of large sample sets. These HT-MS platforms continuously acquire data from various samples into a single data file, presenting challenges in applying distinctive data acquisition methods to specific samples. This study introduces a novel approach that integrates real-time sample loading status to activate sample-specific MS/MS data acquisition methods on the high-throughput acoustic ejection mass spectrometry platform. Effective method switching and high signal reproducibility were demonstrated across different data acquisition window durations in multiple reaction monitoring (MRM), high-resolution MRM (MRMHR), and information-dependent acquisition modes. This advancement provides a user-friendly and robust solution to the method-setting challenges of HT-MS, expanding the implementation of HT-MS platforms in drug discovery and other high-throughput analytical applications.


Assuntos
Ensaios de Triagem em Larga Escala , Espectrometria de Massas em Tandem , Espectrometria de Massas em Tandem/métodos , Ensaios de Triagem em Larga Escala/métodos , Descoberta de Drogas/métodos , Reprodutibilidade dos Testes , Humanos
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