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Binary Solvent Regulated Architecture of Ultra-Microporous Hydrogen-Bonded Organic Frameworks with Tunable Polarization for Highly-Selective Gas Separation.
Ding, Xiaojun; Liu, Zeyu; Zhang, Yusheng; Ye, Gang; Jia, Jianfeng; Chen, Jing.
  • Ding X; Collaborative Innovation Center of Advanced Nuclear Energy Technology, Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing, 100084, China.
  • Liu Z; Collaborative Innovation Center of Advanced Nuclear Energy Technology, Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing, 100084, China.
  • Zhang Y; Collaborative Innovation Center of Advanced Nuclear Energy Technology, Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing, 100084, China.
  • Ye G; Collaborative Innovation Center of Advanced Nuclear Energy Technology, Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing, 100084, China.
  • Jia J; Collaborative Innovation Center of Advanced Nuclear Energy Technology, Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing, 100084, China.
  • Chen J; Collaborative Innovation Center of Advanced Nuclear Energy Technology, Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing, 100084, China.
Angew Chem Int Ed Engl ; 61(13): e202116483, 2022 Mar 21.
Article en En | MEDLINE | ID: mdl-35023611
A binary solvent synthetic strategy is proposed for the construction of C2 -symmetric molecule-based hydrogen-bonded organic frameworks (HOFs) with permanent ultra-micropores and surface polarization derived from tunable coplanar open oxygen atoms. The activated HOFs BTBA-1 a and PTBA-1 a show highly selective separation of CO2 /N2 with a record high ideal adsorbed solution theory (IAST) selectivity >2000 under ambient temperature and pressure.
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Texto completo: 1 Banco de datos: MEDLINE Idioma: En Año: 2022 Tipo del documento: Article
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Texto completo: 1 Banco de datos: MEDLINE Idioma: En Año: 2022 Tipo del documento: Article