Heteroepitaxial Growth of Black Phosphorus on Tin Monosulfide.
Nano Lett
; 24(1): 479-485, 2024 Jan 10.
Article
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| MEDLINE
| ID: mdl-38147351
ABSTRACT
Black phosphorus (Black P), a layered semiconductor with a layer-dependent bandgap and high carrier mobility, is a promising candidate for next-generation electronics and optoelectronics. However, the synthesis of large-area, layer-precise, single crystalline Black P films remains a challenge due to their high nucleation energy. Here, we report the molecular beam heteroepitaxy of single crystalline Black P films on a tin monosulfide (SnS) buffer layer grown on Au(100). The layer-by-layer growth mode enables the preparation of monolayer to trilayer films, with band gaps that reflect layer-dependent quantum confinement.
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