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A highly stereoselective, modular route to (E)-vinylsulfones and to (Z)- and (E)-alkenes.
Braun, Marie-Gabrielle; Quiclet-Sire, Béatrice; Zard, Samir Z.
Afiliação
  • Braun MG; Laboratoire de Synthèse Organique, CNRS UMR 7652, Ecole Polytechnique, 91128 Palaiseau, France.
J Am Chem Soc ; 133(40): 15954-7, 2011 Oct 12.
Article em En | MEDLINE | ID: mdl-21923183
A recently discovered radical fragmentation of 2-fluoro-6-pyridinoxy derivatives allows a new highly stereoselective and convergent route to (E)-vinylsulfones from allylic alcohols. Reductive desulfonylation or nickel-catalyzed couplings furnish di- and trisubstituted (E)- and (Z)-alkenes.

Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2011 Tipo de documento: Article

Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2011 Tipo de documento: Article