A Cooperative Interface for Highly Efficient Lithium-Sulfur Batteries.
Adv Mater
; 28(43): 9551-9558, 2016 Nov.
Article
em En
| MEDLINE
| ID: mdl-27629655
ABSTRACT
A cooperative interface constructed by "lithiophilic" nitrogen-doped graphene frameworks and "sulfiphilic" nickel-iron layered double hydroxides (LDH@NG) is proposed to synergistically afford bifunctional Li and S binding to polysulfides, suppression of polysulfide shuttles, and electrocatalytic activity toward formation of lithium sulfides for high-performance lithium-sulfur batteries. LDH@NG enables high rate capability, long lifespan, and efficient stabilization of both sulfur and lithium electrodes.
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2016
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Article