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Surface Immobilization of Transition Metal Ions on Nitrogen-Doped Graphene Realizing High-Efficient and Selective CO2 Reduction.
Bi, Wentuan; Li, Xiaogang; You, Rui; Chen, Minglong; Yuan, Ruilin; Huang, Weixin; Wu, Xiaojun; Chu, Wangsheng; Wu, Changzheng; Xie, Yi.
Afiliação
  • Bi W; Hefei National Laboratory for Physical Sciences at the Microscale, iChEM (Collaborative Innovation Center of Chemistry for Energy Materials), and CAS Key Laboratory of Mechanical Behavior and Design of Materials, University of Science and Technology of China, Hefei, 230026, China.
  • Li X; Hefei National Laboratory for Physical Sciences at the Microscale, iChEM (Collaborative Innovation Center of Chemistry for Energy Materials), and CAS Key Laboratory of Mechanical Behavior and Design of Materials, University of Science and Technology of China, Hefei, 230026, China.
  • You R; Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion and Department of Chemical Physics, University of Science and Technology of China, Hefei, 230026, China.
  • Chen M; CAS Key Laboratory of Materials for Energy Conversion, Synergetic Innovation of Quantum information and Quantum Technology and Department of Materials Science and Engineering, University of Science and Technology of China, Hefei, 230026, China.
  • Yuan R; Hefei National Laboratory for Physical Sciences at the Microscale, iChEM (Collaborative Innovation Center of Chemistry for Energy Materials), and CAS Key Laboratory of Mechanical Behavior and Design of Materials, University of Science and Technology of China, Hefei, 230026, China.
  • Huang W; Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion and Department of Chemical Physics, University of Science and Technology of China, Hefei, 230026, China.
  • Wu X; CAS Key Laboratory of Materials for Energy Conversion, Synergetic Innovation of Quantum information and Quantum Technology and Department of Materials Science and Engineering, University of Science and Technology of China, Hefei, 230026, China.
  • Chu W; National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui, 230026, China.
  • Wu C; Hefei National Laboratory for Physical Sciences at the Microscale, iChEM (Collaborative Innovation Center of Chemistry for Energy Materials), and CAS Key Laboratory of Mechanical Behavior and Design of Materials, University of Science and Technology of China, Hefei, 230026, China.
  • Xie Y; Hefei National Laboratory for Physical Sciences at the Microscale, iChEM (Collaborative Innovation Center of Chemistry for Energy Materials), and CAS Key Laboratory of Mechanical Behavior and Design of Materials, University of Science and Technology of China, Hefei, 230026, China.
Adv Mater ; 30(18): e1706617, 2018 May.
Article em En | MEDLINE | ID: mdl-29575274
ABSTRACT
Electrochemical conversion of CO2 to value-added chemicals using renewable electricity provides a promising way to mitigate both global warming and the energy crisis. Here, a facile ion-adsorption strategy is reported to construct highly active graphene-based catalysts for CO2 reduction to CO. The isolated transition metal cyclam-like moieties formed upon ion adsorption are found to contribute to the observed improvements. Free from the conventional harsh pyrolysis and acid-leaching procedures, this solution-chemistry strategy is easy to scale up and of general applicability, thus paving a rational avenue for the design of high-efficiency catalysts for CO2 reduction and beyond.
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2018 Tipo de documento: Article
Texto completo
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PubMed Links
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2018 Tipo de documento: Article