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Dynamical heterogeneity in active glasses is inherently different from its equilibrium behavior.
Paul, Kallol; Mutneja, Anoop; Nandi, Saroj Kumar; Karmakar, Smarajit.
Afiliação
  • Paul K; Tata Institute of Fundamental Research Center for Interdisciplinary Science, Hyderabad 500046, Telangana, India.
  • Mutneja A; Tata Institute of Fundamental Research Center for Interdisciplinary Science, Hyderabad 500046, Telangana, India.
  • Nandi SK; Tata Institute of Fundamental Research Center for Interdisciplinary Science, Hyderabad 500046, Telangana, India.
  • Karmakar S; Tata Institute of Fundamental Research Center for Interdisciplinary Science, Hyderabad 500046, Telangana, India.
Proc Natl Acad Sci U S A ; 120(34): e2217073120, 2023 Aug 22.
Article em En | MEDLINE | ID: mdl-37585467
ABSTRACT
Activity-driven glassy dynamics, while ubiquitous in collective cell migration, intracellular transport, dynamics in bacterial and ant colonies, etc., also extends the scope and extent of the as-yet mysterious physics of glass transition. Active glasses are hitherto assumed to be qualitatively similar to their equilibrium counterparts at an effective temperature, [Formula see text]. Here, we combine large-scale simulations and an analytical mode-coupling theory (MCT) for such systems and show that, in fact, an active glass is inherently different from an equilibrium glass. Although the relaxation dynamics can be equilibrium-like at a [Formula see text], effects of activity on the dynamic heterogeneity (DH), which is a hallmark of glassy dynamics, are quite nontrivial and complex. With no preexisting data, we employ four distinct methods for reliable estimates of the DH length scales. Our work shows that active glasses exhibit dramatic growth of DH and systems with similar relaxation times, and thus, [Formula see text] can have widely varying DH. To theoretically study DH, we extend active MCT and find good qualitative agreement between the theory and simulation results. Our results pave avenues for understanding the role of DH in glassy dynamics and can have fundamental significance even in equilibrium.
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Texto completo: 1 Base de dados: MEDLINE Tipo de estudo: Qualitative_research Idioma: En Ano de publicação: 2023 Tipo de documento: Article

Texto completo: 1 Base de dados: MEDLINE Tipo de estudo: Qualitative_research Idioma: En Ano de publicação: 2023 Tipo de documento: Article