Experimental method of transfer function linewidth determination for laser amplifiers using FM-to-AM conversion.

We propose an experimental method for the determination of the transfer function linewidth of a laser amplifier. This technique is based on a transfer function scan using frequency modulation to amplitude modulation (FM-to-AM) temporal modulation measurement as a function of wavelength. Using this method, we show that the output spectrum of a laser amplifier in Q-switch mode is not representative of the transfer function of the amplifier.

Second-order nonlinear optical coefficients of the monoclinic crystal BaGa4Se7.

We characterize the magnitude and relative signs of the second-order nonlinear optical coefficients of the biaxial crystal BaGa4Se7 (BGSe) combining measurements of phase-matched and non-phase-matched second-harmonic generation at different wavelengths using slabs and a sphere.

Impact of the Kerr effect on FM-to-AM conversion in high-power lasers.

In order to smooth the focal spot of high-power energetic lasers, pulses are phase-modulated. However, due to propagation impairments, phase modulation is partly converted into power modulation. This is called frequency modulation to amplitude modulation (FM-to-AM conversion). This effect may increase laser damage and thus increase operating costs. For the first time, to the best of our knowledge, we have studied the impact of the Kerr effect in this process. We have shown that when the Kerr effect is followed by a dispersive transfer function, a dramatic increase of FM-to-AM conversion may occur for a particular kind of FM-to-AM conversion that we have named "anomalous." Hence, we should remove or compensate for one of the items of the sequence: phase modulation, anomalous FM-to-AM conversion, Kerr effect, or the dispersive function. We have assessed all these solutions, and we have found an efficient inspection method to avoid anomalous FM-to-AM conversion.

Study of middle infrared difference frequency generation using a femtosecond laser source in LGT.

We demonstrate phase-matched difference frequency generation in the emerging nonlinear crystal La3Ga5.5Ta0.5O14. Tunable wavelengths between 1.4 and 4.7 µm are generated by using femtosecond sources. We also report on the measurements of the optical damage threshold in the femtosecond regime and on the nonlinear refractive index n2.

Phase-matching directions and refined Sellmeier equations of the monoclinic acentric crystal BaGa4Se7.

We directly measured the phase-matching directions of second-harmonic and difference frequency generation in the principal planes of the biaxial BaGa4Se7 (BGSe) crystal using the sphere method. The simultaneous fit of the data allowed us to refine the Sellmeier equations of the three principal refractive indices of BGSe, and to calculate the tuning curves for infrared optical parametric generation.

Angle noncritical phase-matched second-harmonic generation in the monoclinic crystal BaGa4Se7.

We performed a complete study of angle noncritical phase-matched second-harmonic generation in BaGa4Se7 in the mid-infrared region. We measured the dielectric frame orientation and showed that it does not rotate as a function of wavelength. We determined the phase-matching wavelengths and the associated spectral and angular acceptances along the x and y axes of the dielectric frame. We also estimated the magnitude of the nonlinear coefficients involved.

Phase-matching directions, refined Sellmeier equations, and second-order nonlinear coefficient of the infrared Langatate crystal La3Ga(5.5)Ta(0.5)O14.

We directly measured phase-matching directions of second harmonic, sum, and difference frequency generations in the Langatate La3Ga(5.5)Ta(0.5)O14 (LGT) uniaxial crystal. The simultaneous fit of the data enabled us to refine the Sellmeier equations of the ordinary and extraordinary principal refractive indices over the entire transparency range of the crystal, and to calculate the phase-matching curves and efficiencies of LGT for infrared optical parametric generation.

Dual-wavelength source from 5%MgO:PPLN cylinders for the characterization of nonlinear infrared crystals.

We conceived a unique fully parametric source based on two independent cylindrical OPOs simultaneously pumped by the same Nd:YAG laser. Each OPO delivers more than 2 mJ and is continuously tunable between 1.41 µm and 4.3 µm. This source is of particular interest for the study of the generation of infrared parametric light in nonlinear crystals. It was validated by performing difference frequency generation experiments in CdSe crystals with output in the range 8 - 10 µm.