Optical extinction, refractive index, and multiple scattering for suspensions of interacting colloidal particles.

We provide a general microscopic theory of the scattering cross-section and of the refractive index for a system of interacting colloidal particles, exact at second order in the molecular polarizabilities. In particular: (a) we show that the structural features of the suspension are encoded into the forward scattered field by multiple scattering effects, whose contribution is essential for the so-called "optical theorem" to hold in the presence of interactions; (b) we investigate the role of radiation reaction on light extinction; (c) we discuss our results in the framework of effective medium theories, presenting a general result for the effective refractive index valid, whatever the structural properties of the suspension, in the limit of particles much larger than the wavelength; (d) by discussing strongly-interacting suspensions, we unravel subtle anomalous dispersion effects for the suspension refractive index.

Optical phase conjugation in phase-modulated transmission systems: experimental comparison of different nonlinearity-compensation methods.

We experimentally compare the effectiveness of three different optical-phase-conjugation-based nonlinearity-compensation strategies on a transmission system employing phase-modulated signals, and hence affected by the Gordon-Mollenauer effect. We demonstrate that it is possible to obtain significant nonlinearity compensation, but that no improvement is obtained using configurations specifically aimed at the compensation of the nonlinear phase noise.

Experimental energy-density flux characterization of ultrashort laser pulse filaments.

Visualization of the energy density flux gives a unique insight into the propagation properties of complex ultrashort pulses. This analysis, formerly relegated to numerical investigations, is here shown to be an invaluable experimental diagnostic tool. By retrieving the spatio-temporal amplitude and phase we experimentally obtain the energy density flux within complex ultrashort pulses generated by filamentation in a nonlinear Kerr medium.

Observation of nonlinear Airy-like beam evolution in lithium niobate.

We report the observation of Gaussian beam fragmentation into Airy-like waveforms during nonlinear propagation. The effect is supported by the high-intensity photovoltaic nonlinearity arising in unbiased pure congruent lithium niobate. The process is found to occur when the nonlinear response is dominated by the nonlocal effects associated with the charge-displacement process.

Linear and nonlinear optical properties of Hafnium-doped lithium-niobate crystals.

Measurements of birefringence, second-harmonic phase-matching conditions, and nonlinear coefficient d(31) are performed for a set of Hafnium-doped congruent lithium niobate (Hf:cLN) crystals as functions of dopant concentration. The data highlight that the threshold concentration, above which there is a change in the Hf incorporation mechanism, is slightly above 2mol% and that, up to this value of concentration, the efficiency of nonlinear processes is not affected by the dopant insertion. Combining these results with those already present in literature, Hf:cLN crystals appear to be very promising candidates for the development of photorefractivity-free wavelength converters working at room temperature.

Dispersive wave generation by solitons in microstructured optical fibers.

We study the nonlinear propagation of femtosecond pulses in the anomalous dispersion region of microstructured fibers, where soliton fission mechanisms play an important role. The experiment shows that the output spectrum contains, besides the infrared supercontinuum, a narrow-band 430-nm peak, carrying about one fourth of the input energy. By combining simulation and experiments, we explore the generation mechanism of the visible peak and describe its properties. The simulation demonstrates that the blue peak is generated only when the input pulse is so strongly compressed that the short-wavelength tail of the spectrum includes the wavelength predicted for the dispersive wave. In agreement with simulation, intensity-autocorrelation measurements show that the duration of the blue pulse is in the picosecond time range, and that, by increasing the input intensity, satellite pulses of lower intensity are generated.

Enhancement of stability and efficiency of a nonlinear mirror mode-locked Nd:YVO(4) oscillator by an active Q-switch.

The stability and the peak power of a nonlinear-mirror mode-locked Nd:YVO(4) laser are significantly increased by the insertion of an acousto-optic modulator inside the laser cavity. The repetition rate for reliable operation can be varied in the range 35 kHz - 50 kHz. The laser generates the most intense and stable mode-locked pulses of width 9 ps lying underneath a Q-switched envelope of width 110 ns with a Q-switch modulation frequency of 38 kHz. For 10 W of pump power, a 224 times enhancement of peak power over that of cw mode-locking is obtained under reliable Q-switched and mode-locked operation.

Measurement of the nonlinear phase shift induced by cascaded interactions in a periodically poled lithium niobate waveguide.

We report on the measurement of nonlinear phase shift phiNL induced by a strong pump at wavelength lamda p on a weak signal at lamda s through a cascade of two second-order interactions in a periodically poled lithium-niobate waveguide. The experiment is performed by use of an interferometric scheme especially designed to be insensitive to slow mechanical and thermal drift effects. The observed behavior of phiNL as a function of pump power and of wavelength difference lamda p - lamda s, is in good agreement with the theoretical predictions.

From X- to O-shaped spatiotemporal spectra of light filaments in water.

We show that the angle-wavelength spectra of light filaments excited by ultrashort pulses experience a transition from X- to O-like structures when their carrier wavelengths are switched from normal to anomalous dispersion. Calculations confirm that the O-shaped conical emission follows the elliptic geometry of the nonlinear Schrödinger equation with anomalous dispersion.