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We study the manifestation of the Nernst effect in the Corbino disk subjected to the normal external magnetic field and to the radial temperature gradient. The Corbino geometry offers a precious opportunity for the direct measurement of the magnetization currents that are masked by kinetic contributions to the Nernst current in the conventional geometry. The magnetization currents, also referred to as the edge currents, are independent on the conductivity of the sample which is why they can be conveniently described within the thermodynamic approach. They can be related to the Landau thermodynamic potential for an infinite system. We demonstrate that the observable manifestation of this, purely thermodynamic, Nernst effect consists in the strong oscillations of the magnetic field measured in the center of the disk as a function of the external field. The oscillations depend on the temperature difference at the edges of the disk. Dirac fermions and 2D electrons with a parabolic spectrum are characterized by oscillations of different phase and frequency. We predict qualitatively different power dependencies of the magnitude of the Nernst signal on the chemical potential for normal and Dirac carriers.
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We resolve single-shot polariton condensate polarization dynamics, revealing a high degree of circular polarization persistent up to T=170 K. The statistical analysis of pulse-to-pulse polariton condensate polarization elucidates the stochastic nature of the polarization pinning process, which is strongly dependent on the pump laser intensity and polarization. Our experiments show that by spatial trapping and isolating condensates from their noisy environment it is possible to form strongly spin-polarized polariton condensates at high temperatures, offering a promising route to the realization of polariton spin lattices for quantum simulations.
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It is well known that electrically neutral excitons can still be affected by crossed electric and magnetic fields that make them move in a direction perpendicular to both fields. We show that a similar effect appears in the absence of external electric fields, in the case of scattering of an exciton flow by charged impurities in the presence of the external magnetic field. As a result, the exciton flow changes the direction of its propagation that may be described in terms of the Hall conductivity for excitons. We develop a theory of this effect, which we refer to as the anomalous exciton Hall effect, to distinguish it from the exciton Hall effect that arises due to the valley selective exciton transport in transition metal dichalcogenides. According to our estimations, the effect is relatively weak for optically active or bright excitons in conventional GaAs quantum wells, but it becomes significant for optically inactive or dark excitons, because of the difference of the lifetimes. This makes the proposed effect a convenient tool for spatial separation of dark and bright excitons.
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We extend the thermodynamic approach for the description of the thermal Hall effect in two-dimensional superconductors above the critical temperature, where fluctuation Cooper pairs contribute to the conductivity, as well as in disordered normal metals where the particle-particle channel is important. We express the Hall heat conductivity in terms of the product of temperature derivatives of the chemical potential and of the magnetization of the system. Based on this general expression, we derive the analytical formalism that qualitatively reproduces the superlinear increase of the thermal Hall conductivity with the decrease of temperature observed in a large variety of experimentally studied systems [Grissonnanche et al., Nature (London) 571, 376 (2019)NATUAS0028-083610.1038/s41586-019-1375-0]. We also predict a nonmonotonic behavior of the thermal Hall conductivity in the regime of quantum fluctuations, in the vicinity of the second critical field and at very low temperatures.
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Dark excitons are of fundamental importance for a wide variety of processes in semiconductors but are difficult to investigate using optical techniques due to their weak interaction with light fields. We reveal and characterize dark excitons nonresonantly injected into a semiconductor microcavity structure containing InGaAs/GaAs quantum wells by a gated train of eight 100 fs pulses separated by 13 ns by monitoring their interactions with the bright lower polariton mode. We find a surprisingly long dark exciton lifetime of more than 20 ns, which is longer than the time delay between two consecutive pulses. This creates a memory effect that we clearly observe through the variation of the time-resolved transmission signal. We propose a rate equation model that provides a quantitative agreement with the experimental data.
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We report on the experimental evidence for a nanosecond timescale spin memory based on nonradiative excitons with large in-plane wave vector. The effect manifests itself in magnetic-field-induced oscillations of the energy of the optically active (radiative) excitons. The oscillations detected by a spectrally resolved pump-probe technique applied to a GaAs/AlGaAs quantum well structure in a transverse magnetic field persist over a timescale, which is orders of magnitude longer than the characteristic decoherence time in the system. The effect is attributed to the spin-dependent electron-electron exchange interaction of the optically active and inactive excitons. The spin relaxation time of the electrons belonging to nonradiative excitons appears to be much longer than the hole spin relaxation time.
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Bosonic cascade lasers are terahertz (THz) lasers based on stimulated radiative transitions between bosonic condensates of excitons or exciton-polaritons confined in a trap. We study the interaction of an incoming THz pulse resonant in frequency with the transitions between neighboring energy levels of the cascade. We show that at certain optical pump conditions the cascade becomes transparent to the incident pulse: it neither absorbs nor amplifies it in the mean-field approximation. The populations of intermediate levels of the bosonic cascade change as the THz pulse passes, nevertheless. In comparison, a fermionic cascade laser does not reveal any of these properties.
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We propose using the effective spin-orbit coupling of light in Bragg-modulated cylindrical waveguides for the efficient separation of spin-up and spin-down photons emitted by a single photon emitter. Because of the spin and directional dependence of photonic stop bands in the waveguides, spin-up (-down) photon propagation in the negative (positive) direction along the waveguide axis is blocked while the same photon freely propagates in the opposite direction. Frequency shifts of photonic band structures induced by the spin-orbit coupling are verified by finite-difference time-domain numerical simulations.
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We demonstrate the generation of chiral modes-vortex flows with fixed handedness in exciton-polariton quantum fluids. The chiral modes arise in the vicinity of exceptional points (non-Hermitian spectral degeneracies) in an optically induced resonator for exciton polaritons. In particular, a vortex is generated by driving two dipole modes of the non-Hermitian ring resonator into degeneracy. Transition through the exceptional point in the space of the system's parameters is enabled by precise manipulation of real and imaginary parts of the closed-wall potential forming the resonator. As the system is driven to the vicinity of the exceptional point, we observe the formation of a vortex state with a fixed orbital angular momentum (topological charge). This method can be extended to generate higher-order orbital angular momentum states through coalescence of multiple non-Hermitian spectral degeneracies. Our Letter demonstrates the possibility of exploiting nontrivial and counterintuitive properties of waves near exceptional points in macroscopic quantum systems.
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If bosonic particles are cooled down below the temperature of quantum degeneracy, they can spontaneously form a coherent state in which individual matter waves synchronize and combine. Spontaneous coherence of matter waves forms the basis of a number of fundamental phenomena in physics, including superconductivity, superfluidity and Bose-Einstein condensation. Spontaneous coherence is the key characteristic of condensation in momentum space. Excitons--bound pairs of electrons and holes--form a model system to explore the quantum physics of cold bosons in solids. Cold exciton gases can be realized in a system of indirect excitons, which can cool down below the temperature of quantum degeneracy owing to their long lifetimes. Here we report measurements of spontaneous coherence in a gas of indirect excitons. We found that spontaneous coherence of excitons emerges in the region of the macroscopically ordered exciton state and in the region of vortices of linear polarization. The coherence length in these regions is much larger than in a classical gas, indicating a coherent state with a much narrower than classical exciton distribution in momentum space, characteristic of a condensate. A pattern of extended spontaneous coherence is correlated with a pattern of spontaneous polarization, revealing the properties of a multicomponent coherent state. We also observed phase singularities in the coherent exciton gas. All these phenomena emerge when the exciton gas is cooled below a few kelvin.
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We predict spontaneous generation of superfluid polariton currents in planar microcavities with lateral periodic modulation of both the potential and decay rate. A spontaneous breaking of spatial inversion symmetry of a polariton condensate emerges at a critical pumping, and the current direction is stochastically chosen. We analyze the stability of the current with respect to the fluctuations of the condensate. A peculiar spatial current domain structure emerges, where the current direction is switched at the domain walls, and the characteristic domain size and lifetime scale with the pumping power.
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Angle-resolved second harmonic generation (SHG) spectra of ZnO microwires show characteristic Fano resonances in the spectral vicinity of exciton-polariton modes. We observe a resonant peak followed by a strong dip in SHG originating from the constructive and destructive interference of the nonresonant SHG and the resonant contribution of the polariton mode. It is demonstrated that the Fano line shape, and thus the Fano asymmetry parameter q, can be tuned by the phase shift of the two channels. We develop a model to calculate the phase-dependent q as a function of the radial angle in the microwire and achieve a good agreement with the experimental results. The deduced phase-to-q relation unveils the crucial information about the dynamics of the system and offers a tool for control on the line shape of the SHG spectra in the vicinity of exciton-polariton modes.
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We report the experimental investigation and theoretical modeling of a rotating polariton superfluid relying on an innovative method for the injection of angular momentum. This novel, multipump injection method uses four coherent lasers arranged in a square, resonantly creating four polariton populations propagating inwards. The control available over the direction of propagation of the superflows allows injecting a controllable nonquantized amount of optical angular momentum. When the density at the center is low enough to neglect polariton-polariton interactions, optical singularities, associated with an interference pattern, are visible in the phase. In the superfluid regime resulting from the strong nonlinear polariton-polariton interaction, the interference pattern disappears and only vortices with the same sign are persisting in the system. Remarkably, the number of vortices inside the superfluid region can be controlled by controlling the angular momentum injected by the pumps.
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We address, theoretically, the puzzling similarity observed in the thermodynamic behavior of independent clouds of cold dipolar excitons in coupled semiconductor quantum wells. We argue that the condensation of self-trapped exciton gas starts at the same critical temperature in all traps due to the specific scaling rule. As a consequence of the reduced dimensionality of the system, the scaling parameters appear to be insensitive to disorder.
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We propose a novel physical mechanism for the creation of long-lived macroscopic exciton-photon qubits in semiconductor microcavities with embedded quantum wells in the strong coupling regime. The polariton qubit is a superposition of lower branch and upper branch exciton-polariton states. We argue that the coherence time of Rabi oscillations can be dramatically enhanced due to their stimulated pumping from a permanent thermal reservoir of polaritons. We discuss applications of such qubits for quantum information processing, cloning, and storage purposes.
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We observe a strong variation of the Zeeman splitting of exciton polaritons in microcavities when switching between the linear regime, the polariton lasing, and photon lasing regimes. In the polariton lasing regime the sign of Zeeman splitting changes compared to the linear regime, while in the photon lasing regime the splitting vanishes. We additionally observe an increase of the diamagnetic shift in the polariton lasing regime. These effects are explained in terms of the nonequilibrium "spin Meissner effect."
Assuntos
Campos Eletromagnéticos , Modelos Teóricos , Óptica e Fotônica/métodos , Fótons , Teoria Quântica , SemicondutoresRESUMO
Dipolaritons are mixed light-matter quasiparticles formed in double quantum wells embedded in microcavities. Because of resonant coupling between direct and indirect excitons via electronic tunneling, dipolaritons possess large dipole moments. Resonant excitation of the cavity mode by a short pulse of light induces oscillations of the indirect exciton density with a characteristic frequency of Rabi flopping. This results in oscillations of a classical Hertz dipole array which generate supperradiant emission on a terahertz (THz) frequency. The resulting THz signal may be enhanced using the supplementary THz cavity in the weak coupling regime.
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We propose a concept of a quantum cascade laser based on transitions of bosonic quasiparticles (excitons) in a parabolic potential trap in a semiconductor microcavity. This laser would emit terahertz radiation due to bosonic stimulation of excitonic transitions. The dynamics of a bosonic cascade is strongly different from the dynamics of a conventional fermionic cascade laser. We show that populations of excitonic ladders are parity dependent and quantized if the laser operates without an external terahertz cavity.
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We report the observation of spin currents in a coherent gas of indirect excitons. The realized long-range spin currents originate from the formation of a coherent gas of bosonic pairs--a new mechanism to suppress the spin relaxation. The spin currents result in the appearance of a variety of polarization patterns, including helical patterns, four-leaf patterns, spiral patterns, bell patterns, and periodic patterns. We demonstrate control of the spin currents by a magnetic field. We also present a theory of coherent exciton spin transport that describes the observed exciton polarization patterns and indicates the trajectories of the spin currents.
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Vertical cavity surface emitting terahertz lasers can be realized in conventional semiconductor microcavities with embedded quantum wells in the strong coupling regime. The cavity is to be pumped optically at half the frequency of the 2p exciton state. Once a threshold population of 2p excitons is achieved, a stimulated terahertz transition populates the lower exciton-polariton branch, and the cavity starts emitting laser light both in the optical and terahertz ranges. The lasing threshold is sensitive to the statistics of photons of the pumping light.