Thermodynamic evidence of fractional Chern insulator in moiré MoTe2.

Chern insulators, which are the lattice analogues of the quantum Hall states, can potentially manifest high-temperature topological orders at zero magnetic field to enable next-generation topological quantum devices1-3. Until now, integer Chern insulators have been experimentally demonstrated in several systems at zero magnetic field3-8, whereas fractional Chern insulators have been reported in only graphene-based systems under a finite magnetic field9,10. The emergence of semiconductor moiré materials11, which support tunable topological flat bands12,13, provides an opportunity to realize fractional Chern insulators13-16. Here we report thermodynamic evidence of both integer and fractional Chern insulators at zero magnetic field in small-angle twisted bilayer MoTe2 by combining the local electronic compressibility and magneto-optical measurements. At hole filling factor ν = 1 and 2/3, the system is incompressible and spontaneously breaks time-reversal symmetry. We show that they are integer and fractional Chern insulators, respectively, from the dispersion of the state in the filling factor with an applied magnetic field. We further demonstrate electric-field-tuned topological phase transitions involving the Chern insulators. Our findings pave the way for the demonstration of quantized fractional Hall conductance and anyonic excitation and braiding17 in semiconductor moiré materials.

Remote imprinting of moiré lattices.

Two-dimensional moiré materials are formed by overlaying two layered crystals with small differences in orientation or/and lattice constant, where their direct coupling generates moiré potentials. Moiré materials have emerged as a platform for the discovery of new physics and device concepts, but while moiré materials are highly tunable, once formed, moiré lattices cannot be easily altered. Here we demonstrate the electrostatic imprinting of moiré lattices onto a target monolayer semiconductor. The moiré potential-created by a lattice of electrons that is supported by a Mott insulator state in a remote MoSe2/WS2 moiré bilayer-imprints a moiré potential that generates flat bands and correlated insulating states in the target monolayer and can be turned on/off by gate tuning the doping density of the moiré bilayer. Additionally, we studied the interplay between the electrostatic and structural relaxation contributions to moiré imprinting. Our results demonstrate a pathway towards gate control of moiré lattices.

Nonlinear optics in the fractional quantum Hall regime.

Engineering strong interactions between optical photons is a challenge for quantum science. Polaritonics, which is based on the strong coupling of photons to atomic or electronic excitations in an optical resonator, has emerged as a promising approach to address this challenge, paving the way for applications such as photonic gates for quantum information processing1 and photonic quantum materials for the investigation of strongly correlated driven-dissipative systems2,3. Recent experiments have demonstrated the onset of quantum correlations in exciton-polariton systems4,5, showing that strong polariton blockade6-the prevention of resonant injection of additional polaritons in a well delimited region by the presence of a single polariton-could be achieved if interactions were an order of magnitude stronger. Here we report time-resolved four-wave-mixing experiments on a two-dimensional electron system embedded in an optical cavity7, demonstrating that polariton-polariton interactions are strongly enhanced when the electrons are initially in the fractional quantum Hall regime. Our experiments indicate that, in addition to strong correlations in the electronic ground state, exciton-electron interactions leading to the formation of polaron-polaritons8-11 have a key role in enhancing the nonlinear optical response of the system. Our findings could facilitate the realization of strongly interacting photonic systems, and suggest that nonlinear optical measurements could provide information about fractional quantum Hall states that is not accessible through their linear optical response.

Polaron Polaritons in the Integer and Fractional Quantum Hall Regimes.

Elementary quasiparticles in a two-dimensional electron system can be described as exciton polarons since electron-exciton interactions ensures dressing of excitons by Fermi-sea electron-hole pair excitations. A relevant open question is the modification of this description when the electrons occupy flat bands and electron-electron interactions become prominent. Here, we perform cavity spectroscopy of a two-dimensional electron system in the strong coupling regime, where polariton resonances carry signatures of strongly correlated quantum Hall phases. By measuring the evolution of the polariton splitting under an external magnetic field, we demonstrate the modification of polaron dressing that we associate with filling factor dependent electron-exciton interactions.