An optical NMR spectrometer for Larmor-beat detection and high-resolution POWER NMR.

Optical nuclear magnetic resonance (ONMR) is a powerful probe of electronic properties in III-V semiconductors. Larmor-beat detection (LBD) is a sensitivity optimized, time-domain NMR version of optical detection based on the Hanle effect. Combining LBD ONMR with the line-narrowing method of POWER (perturbations observed with enhanced resolution) NMR further enables atomically detailed views of local electronic features in III-Vs. POWER NMR spectra display the distribution of resonance shifts or line splittings introduced by a perturbation, such as optical excitation or application of an electric field, that is synchronized with a NMR multiple-pulse time-suspension sequence. Meanwhile, ONMR provides the requisite sensitivity and spatial selectivity to isolate local signals within macroscopic samples. Optical NMR, LBD, and the POWER method each introduce unique demands on instrumentation. Here, we detail the design and implementation of our system, including cryogenic, optical, and radio-frequency components. The result is a flexible, low-cost system with important applications in semiconductor electronics and spin physics. We also demonstrate the performance of our systems with high-resolution ONMR spectra of an epitaxial AlGaAs/GaAs heterojunction. NMR linewidths down to 4.1 Hz full width at half maximum were obtained, a 10(3)-fold resolution enhancement relative any previous optically detected NMR experiment.

Microscopic Evidence for Spatially Inhomogeneous Charge Trapping in Pentacene.

Charge traps in pentacene thin-film transistors (Figure, left) have been imaged using electric force microscopy. The Figure shows a map of the trap distribution just below (middle) and well above (right) the transistor threshold voltage. It is found that the long-lived charge traps in polycrystalline pentacene are distributed inhomogeneously and do not appear to be associated with grain boundaries, as is generally assumed.

Nanoscale Fourier-transform imaging with magnetic resonance force microscopy.

We present a versatile method for Fourier encoding the spatial distribution of spins detected by magnetic resonance force microscopy. Shuttling a magnetic particle in synchrony with an rf pulse sequence causes spins in a constant-field slice near the particle to precess at a rate proportional to their x or y coordinate. A two-dimensional spin-density map is recovered by a linear Fourier transform of a set of integrated force signals. Performance of the rf sequence is demonstrated experimentally and numerical simulations show that the method can achieve nanoscale resolution. Our approach offers a new route to manipulating spin wave functions down to the atomic scale.