Laguerre-Gaussian laser filamentation for the control of electric discharges in air.

We study the use of Laguerre-Gaussian (LG) femtosecond laser filament with multi GW peak power to guide electric sparks in the atmosphere. We demonstrate that an LG beam with a vortex phase or with 6 azimuthal phase steps generates a filamentation regime, where a longer and more uniform energy deposition is produced compared to a normal beam with a flat phase. Such filaments can guide electric discharges over much longer distances. This technique could significantly extend the guiding range of laser filaments for lightning control and other long-range atmospheric experiments involving filamentation.

Spectral splitting of the lasing emission of nitrogen ions pumped by 800-nm femtosecond laser pulses.

We report on a spectral splitting effect of the cavity-less lasing emission of nitrogen ions at 391.4 nm pumped by 800-nm femtosecond laser pulses. It was found that with the increase of the nitrogen gas pressure and pump pulse energy, both R and P branches experience spectral splitting. With an external injected seeding pulse, a similar split spectral line is observed for the amplified emission. In contrast, for the fluorescence radiation, no such spectral splitting phenomenon is observed with much more abundant R branch structures. Our theoretical model considers gas ionization by the pump pulse, the competition of excitation of all relevant electronic and vibrational states, and an amplification of the seeding pulse in the plasma with a population inversion. Our simulation reproduces this spectral splitting effect, which is attributed to the gain saturation resulting in the oscillation of the amplitude of the amplified signal.

Quantum and quasi-classical effects in the strong field ionization and subsequent excitation of nitrogen molecules.

The processes leading to the N2 + lasing are rather complex and even the population distribution after the pump laser excitation is unknown. In this paper, we study the population distribution at electronic and vibrational levels in N2 + driven by ultra-short laser pulse at the wavelengths of 800 nm and 400 nm by using the quantum-mechanical time-domain incoherent superposition model based on the time-dependent Schrödinger equation and the quasi-classical model assuming instantaneous ionization injection described by density matrix. It is shown that while both models provide qualitatively similar results, the quasi-classical instantaneous ionization injection model underestimates the population inversions corresponding to the optical transitions at 391 nm, 423 nm and 428 nm due to the assumption of quantum mixed states at the ionization time. A fast and accurate correction to this error is proposed. This work solidifies the theoretical models for population at vibrational states in N2 + and paves the way to uncover the mechanism of the N2 + lasing.

Femtosecond filamentation of optical vortices for the generation of optical air waveguides.

We study the filamentation in air of multi-millijoule optical vortices and compare them with the classical filamentation regime. The femtosecond vortex beam generates multiple plasma filaments organized in a cylindrical geometry. This plasma configuration evolves into a meter-scale tubular neutral gas column that can be used as a waveguide for nanosecond laser pulses at 532 nm. It appears that optical vortices produce a more uniform heating along the propagation axis, when compared with Gaussian or super-Gaussian beams, and that the resulting low-density channel is poorly sensitive to the laser input power thanks to the combination of filamentation intensity clamping and phase vorticity.

Time-resolved study of laser emission in nitrogen gas pumped by two near IR femtosecond laser pulses.

The time profile of a lasing signal at 391.4 nm emitted by a weakly ionized gas of nitrogen molecules at low pressure is measured under double excitation with intense femtosecond laser pulses at 800 nm. An abrupt decrease in emission occurs at the time of arrival of the second pulse. It is explained by a transfer of population from ground to first excited ionic level and by a disruption of coherence, terminating the conditions for lasing in a V-scheme without population inversion.

Quantum erasing of laser emission in N2.

Cavity-free lasing of N2+ induced by a femtosecond laser pulse at 800 nm is nearly totally suppressed by a delayed twin control pulse. We explain this surprising effect within the V-scheme of lasing without population inversion. A fast transfer of population between nitrogen ionic states X2Σg+ and A2Πu, induced by the second pulse, terminates the conditions for amplification in the system. The appearance of short lasing bursts at delays corresponding to revivals of rotational wave packets is explained along the same lines.

HV discharges triggered by dual- and triple-frequency laser filaments.

We study the use of frequency upconversion schemes of near-IR picosecond laser pulses and compare their ability to guide and trigger electric discharges through filamentation in air. Upconversion, such as Second Harmonic Generation, is favorable for triggering electric discharges for given amount of available laser energy, even taking into account the losses inherent to frequency conversion. We focus on the practical question of optimizing the use of energy from a given available laser system and the potential advantage to use frequency conversion schemes.

Formation Dynamics of Excited Neutral Nitrogen Molecules inside Femtosecond Laser Filaments.

Nitrogen molecules are promoted to excited neutral states during femtosecond laser pulse filamentary propagation in atmosphere, leading to a characteristic UV fluorescence. Using a laser-induced fluorescence depletion technique, we measure the formation dynamics of these excited neutral nitrogen molecules with femtosecond time resolution. We find that the excited neutral molecules are formed in an unexpected ultrafast timescale of ∼4 ps at 1 bar and ∼120 ps at 30 mbar pressure. From this observation we deduce that the excitation of neutral N_{2} occurs via multiple collisions with hot free electrons. Numerical simulations based on rate equations reproduce well this ultrafast formation time and its dependence on gas pressure, and thus support this interpretation.

Unexpected Sensitivity of Nitrogen Ions Superradiant Emission on Pump Laser Wavelength and Duration.

Nitrogen molecules in ambient air exposed to an intense near-infrared femtosecond laser pulse give rise to cavity-free superradiant emission at 391.4 and 427.8 nm. An unexpected pulse duration-dependent cyclic variation of the superradiance intensity is observed when the central wavelength of the femtosecond pump laser pulse is finely tuned between 780 and 820 nm, and no signal occurs at the resonant wavelength of 782.8 nm (2ω_{782.8 nm}=ω_{391.4 nm}). On the basis of a semiclassical recollision model, we show that an interference of dipolar moments of excited ions created by electron recollisions explains this behavior.

Energy deposition from focused terawatt laser pulses in air undergoing multifilamentation.

Laser filamentation is responsible for the deposition of a significant part of the laser pulse energy in the propagation medium. We found that using terawatt laser pulses and moderately strong focusing conditions in air, more than 60 % of the pulses energy is transferred to the medium, eventually degrading into heat. This results in a strong hydrodynamic reaction of air with the generation of shock waves and associated underdense channels for each of the generated multiple filaments. In the focal zone, where filaments are close to each other, these discrete channels eventually merge to form a single cylindrical low-density tube over a ~ 1 µs timescale. We measured the maximum lineic deposited energy to be more than 1 J·m-1.

Recollision-Induced Superradiance of Ionized Nitrogen Molecules.

We propose a new mechanism to explain the origin of optical gain in the transitions between the excited and ground states of the ionized nitrogen molecule following irradiation of neutral nitrogen molecules with an intense ultrashort laser pulse. An efficient transfer of population to the excited state is achieved via field-induced multiple recollisions. We show that the proposed excitation mechanism must lead to a superradiant emission, a feature that we confirm experimentally.

Plasma luminescence from femtosecond filaments in air: evidence for impact excitation with circularly polarized light pulses.

Filaments produced in air by intense femtosecond laser pulses emit UV luminescence from excited N(2) and N(2)(+) molecules. We report on a strong dependence at high intensities (I≥1.4×10(14) W/cm(2)) of this luminescence with the polarization state of the incident laser pulses. We attribute this effect to the onset of new impact excitation channels from energetic electrons produced with circularly polarized laser pulses above a threshold laser intensity.

Underwater acoustic signals induced by intense ultrashort laser pulse.

Acoustic signals generated in water by terawatt (TW) laser pulses undergoing filamentation are studied. The acoustic signal has a very broad spectrum, spanning from 0.1 to 10 MHz and is confined in the plane perpendicular to the laser direction. Such a source appears to be promising for the development of remote laser based acoustic applications.

Backward stimulated radiation from filaments in nitrogen gas and air pumped by circularly polarized 800 nm femtosecond laser pulses.

We report on strong backward stimulated emission at 337 nm in nitrogen gas pumped by circularly polarized femtosecond laser pulses at 800 nm. A distinct dependence of the backward UV spectrum on pump laser polarization and intensity is observed, pointing to the occurrence of backward amplified spontaneous emission inside filaments. We attribute the population inversion to inelastic collision between the free electrons produced by the pump laser and neutral N2 molecules. The addition of oxygen molecules is detrimental for the gain, reducing it to near threshold at atmospheric concentration.

Backward Lasing of Air plasma pumped by Circularly polarized femtosecond pulses for the saKe of remote sensing (BLACK).

Recently, S. Mitryukovskiy et al. presented experimental evidence showing that backward Amplified Spontaneous Emission (ASE) at 337 nm can be obtained from plasma filaments in nitrogen gas pumped by circularly polarized 800 nm femtosecond pulses (Opt. Express, 22, 12750 (2014)). Here, we report that a seed pulse injected in the backward direction can be amplified by ~200 times inside this plasma amplifier. The amplified 337 nm radiation can be either linearly or circularly polarized, dictated by the seeding pulse, which is distinct from the non-polarized nature of the ASE. We performed comprehensive measurements of the spatial profile, optical gain dynamics, and seed pulse energy dependence of this amplification process. These measurements allow us to deduce the pulse duration of the ASE and the amplified 337 nm radiation as well as the corresponding laser intensity inside the plasma amplifier. It indicates that the amplification is largely in the unsaturated regime and that further improvement of laser energy is possible. Moreover, we observed optical gain in plasma created in ambient air. This represents an important step towards future applications exploiting backward lasing for remote atmospheric sensing.

Lasing of ambient air with microjoule pulse energy pumped by a multi-terawatt infrared femtosecond laser.

We report on the lasing action of atmospheric air pumped by an 800 nm femtosecond laser pulse with peak power up to 4 TW. Lasing emission at 428 nm increases rapidly over a small range of pump laser power, followed by saturation above ∼1.5 TW. The maximum lasing pulse energy is measured at 2.6 µJ corresponding to an emission power in the MW range, while a maximum conversion efficiency of 3.5×10(-5) is measured at moderate pump pulse energy. The optical gain inside the filament plasma is estimated to be in excess of 0.7/cm. Lasing emission shows a doughnut profile, reflecting the spatial distribution of the pump-generated white-light continuum that acts as a seed for the lasing. We attribute the pronounced saturation to the defocusing of the seed in the plasma amplifying region and to the saturation of the seed intensity.

Superfilamentation in air.

The interaction between a large number of laser filaments brought together using weak external focusing leads to the emergence of few filamentary structures reminiscent of standard filaments, but carrying a higher intensity. The resulting plasma is measured to be 1 order of magnitude denser than for short-scale filaments. This new propagation regime is dubbed superfilamentation. Numerical simulations of a nonlinear envelope equation provide good agreement with experiments.

Self-seeded lasing in ionized air pumped by 800 nm femtosecond laser pulses.

We report on the lasing in air and pure nitrogen gas pumped by a single 800 nm femtosecond laser pulse. Depending on gas pressure, incident laser power and beam convergence, different lasing lines are observed in the forward direction with rapid change of their relative intensities. The lines are attributed to transitions between vibrational and rotational levels of the first negative band of the singly charged nitrogen molecule-ion. We show that self-seeding plays an important role in the observed intensity changes.

Kilometer range filamentation.

We demonstrate for the first time the possibility to generate long plasma channels up to a distance of 1 km, using the terawatt femtosecond T&T laser facility. The plasma density was optimized by adjusting the chirp, the focusing and beam diameter. The interaction of filaments with transparent and opaque targets was studied.

Ciliary white light: optical aspect of ultrashort laser ablation on transparent dielectrics.

We report on a novel nonlinear optical phenomenon, coined as ciliary white light, during laser ablation of transparent dielectrics. It is observed in 14 different transparent materials including glasses, crystals, and polymers. This phenomenon is also universal with respect to laser polarization, pulse duration, and focusing geometry. We interpret its formation in terms of the nonlinear diffraction of the laser generated white light by the ablation crater covered by nanostructures. It carries rich information on the damage profile and morphology dynamics of the ablated surface, providing a real time in situ observation of the laser ablation process.