Coulomb-driven energy boost of heavy ions for laser-plasma acceleration.

An unprecedented increase of kinetic energy of laser accelerated heavy ions is demonstrated. Ultrathin gold foils have been irradiated by an ultrashort laser pulse at a peak intensity of 8×10^{19} W/ cm^{2}. Highly charged gold ions with kinetic energies up to >200 MeV and a bandwidth limited energy distribution have been reached by using 1.3 J laser energy on target. 1D and 2D particle in cell simulations show how a spatial dependence on the ion's ionization leads to an enhancement of the accelerating electrical field. Our theoretical model considers a spatial distribution of the ionization inside the thin target, leading to a field enhancement for the heavy ions by Coulomb explosion. It is capable of explaining the energy boost of highly charged ions, enabling a higher efficiency for the laser-driven heavy ion acceleration.

Acceleration of neutral atoms in strong short-pulse laser fields.

A charged particle exposed to an oscillating electric field experiences a force proportional to the cycle-averaged intensity gradient. This so-called ponderomotive force plays a major part in a variety of physical situations such as Paul traps for charged particles, electron diffraction in strong (standing) laser fields (the Kapitza-Dirac effect) and laser-based particle acceleration. Comparably weak forces on neutral atoms in inhomogeneous light fields may arise from the dynamical polarization of an atom; these are physically similar to the cycle-averaged forces. Here we observe previously unconsidered extremely strong kinematic forces on neutral atoms in short-pulse laser fields. We identify the ponderomotive force on electrons as the driving mechanism, leading to ultrastrong acceleration of neutral atoms with a magnitude as high as approximately 10(14) times the Earth's gravitational acceleration, g. To our knowledge, this is by far the highest observed acceleration on neutral atoms in external fields and may lead to new applications in both fundamental and applied physics.

Observing Rydberg atoms to survive intense laser fields.

The idea of atoms defying ionization in ultrastrong laser fields has fascinated physicists for the last three decades. In contrast to extensive theoretical work on atoms stabilized in strong fields only few experiments limited to intermediate intensities have been performed. In this work we show exceptional stability of Rydberg atoms in strong laser fields extending the range of observation to much higher intensities. Corresponding field amplitudes of more than 1 GV/cm exceed the thresholds for static field ionization by more than 6 orders of magnitude. Most importantly, however, is our finding that a surviving atom is tagged with a measure of the laser intensity it has interacted with. Reading out this information removes uncertainty about whether the surviving atom has really seen the high intensity. The experimental results allow for an extension of the investigations on the stabilization and interaction of a quasifree electron with a strong field into the relativistic regime.

Frustrated tunnel ionization of noble gas dimers with Rydberg-electron shakeoff by electron charge oscillation.

Strong field single ionization of homo- and heteronuclear noble gas dimers with ultrashort infrared laser pulses is experimentally investigated. A pronounced photoelectron yield maximum is found for dimers in the momentum range |p|≤0.1 a.u. which is absent for the corresponding monomer. This yield enhancement can be attributed to a new two-step strong field ionization mechanism active only in the dimers. In the first step, frustrated tunnel ionization at one of the atomic centers populates Rydberg states, which then become ionized in a second step through charge oscillation within the dimer ion core.

Enhanced proton acceleration by an ultrashort laser interaction with structured dynamic plasma targets.

We experimentally demonstrate a notably enhanced acceleration of protons to high energy by relatively modest ultrashort laser pulses and structured dynamical plasma targets. Realized by special deposition of snow targets on sapphire substrates and using carefully planned prepulses, high proton yields emitted in a narrow solid angle with energy above 21 MeV were detected from a 5 TW laser. Our simulations predict that using the proposed scheme protons can be accelerated to energies above 150 MeV by 100 TW laser systems.

Compact x-ray microscope for the water window based on a high brightness laser plasma source.

We present a laser plasma based x-ray microscope for the water window employing a high-average power laser system for plasma generation. At 90 W laser power a brightness of 7.4 x 10(11) photons/(s x sr x µm(2)) was measured for the nitrogen Lyα line emission at 2.478 nm. Using a multilayer condenser mirror with 0.3 % reflectivity 10(6) photons/(µm(2) x s) were obtained in the object plane. Microscopy performed at a laser power of 60 W resolves 40 nm lines with an exposure time of 60 s. The exposure time can be further reduced to 20 s by the use of new multilayer condenser optics and operating the laser at its full power of 130 W.

Radiation-pressure acceleration of ion beams driven by circularly polarized laser pulses.

We present experimental studies on ion acceleration from ultrathin diamondlike carbon foils irradiated by ultrahigh contrast laser pulses of energy 0.7 J focused to peak intensities of 5x10(19) W/cm2. A reduction in electron heating is observed when the laser polarization is changed from linear to circular, leading to a pronounced peak in the fully ionized carbon spectrum at the optimum foil thickness of 5.3 nm. Two-dimensional particle-in-cell simulations reveal that those C6+ ions are for the first time dominantly accelerated in a phase-stable way by the laser radiation pressure.

Proton acceleration in the electrostatic sheaths of hot electrons governed by strongly relativistic laser-absorption processes.

Two different laser energy absorption mechanisms at the front side of a laser-irradiated foil have been found to occur, such that two distinct relativistic electron beams with different properties are produced. One beam arises from the ponderomotively driven electrons propagating in the laser propagation direction, and the other is the result of electrons driven by resonance absorption normal to the target surface. These properties become evident at the rear surface of the target, where they give rise to two spatially separated sources of ions with distinguishable characteristics when ultrashort (40fs) high-intensity laser pulses irradiate a foil at 45 degrees incidence. The laser pulse intensity and the contrast ratio are crucial. One can establish conditions such that one or the other of the laser energy absorption mechanisms is dominant, and thereby one can control the ion acceleration scenarios. The observations are confirmed by particle-in-cell (PIC) simulations.

The Thomson deflectometer: a novel use of the Thomson spectrometer as a transient field and plasma diagnostic.

Laser accelerated proton beams have been used for field characterization in expanding plasmas. The Thomson parabola spectrometer, as a charged particles analyzer, also allows precise measurement of the charged particles' trajectories. The proton's deflections by fast changing plasma fields can be measured with the new design of the Thomson parabola spectrometer and, therefore, it can be applied for proton deflectometry. It is shown that from resulting spectrograms the plasma field dynamics can be reconstructed with high temporal resolution. In a proof-of-principle experiment, a weakly relativistic plasma expansion is studied as an example.

Characterization of a nonlinear filter for the front-end of a high contrast double-CPA Ti:sapphire laser.

A nonlinear filter using rotation of the polarization ellipse in air is investigated. Scheme to enhance the temporal contrast is developed for a double-CPA multi-terawatt Ti:sapphire laser. It supports an energy level of millijoule and has a high efficiency. The method allows suppression of the ASE pedestal, pre- and post-pulses by 3 orders of magnitude and also steepens the pulse front. For the physical interpretation of the results, numerical simulation of the filtering is performed.

Non-sequential double ionization of Ne in intense laser pulses: a coincidence experiment.

The dynamics of Neon double ionization by 25 fs, 1.0 PW/cm 2 laser pulses at 795 nm has been studied in a many particle coincidence experiment. The momentum vectors of all ejected atomic fragments (electrons and ions) have been measured using combined electron and recoil-ion momentum spectroscopy. Electron emission spectra for double and single ionization will be discussed. In both processes the mean electron energies differ considerably and high energetic electrons with energies of more than 120 eV have been observed for double ionization. The experimental results are in qualitative agreement with the rescattering model.

Routes to nonsequential double ionization

A method is proposed for the calculation of the S matrix for many-electron processes in intense-laser atom physics, in close analogy to the strong-field approximation for one-electron processes. Given a scenario of how some process evolves, corresponding approximations to the classical action are made which allow for the evaluation of the quantum-mechanical S matrix. The method is applied to the distribution of the total electronic momentum in nonsequential double ionization, and the results are compared to recent measurements. Good agreement is obtained for neon for a rescattering scenario. There is no comparable agreement for helium and argon, and possible alternative scenarios are discussed.

Collective multielectron tunneling ionization in strong fields

We investigate the quantum mechanical process of two-electron tunneling in strong external electric fields. Numerical solution of a two-electron s-wave model reveals the existence of collective tunneling ionization in a mode where both electrons stay at equal distance from the nucleus. Otherwise the lagging electron is immediately recaptured. The corresponding double ionization rate fails to explain nonsequential multiple ionization in strong-field laser experiments. However, an empirically modified version of the analytical one-electron tunneling rate of Ammosov, Delone, and Krainov agrees with the experiments to a surprising accuracy. The reason for this agreement is presently unknown.

Momentum distributions of ne(n+) ions created by an intense ultrashort laser pulse

Vector momentum distributions of Ne(n+) (n = 1,2,3) ions created by 30 fs, approximately 1 PW/cm(2) laser pulses at 795 nm have been measured using recoil-ion momentum spectroscopy. Distinct maxima along the light polarization axis are observed at 4.0 and 7.5 a.u. for Ne2+ and Ne3+ production, respectively. Hence, mechanisms based on an instantaneous release of two (or more) electrons can be ruled out as a dominant contribution to nonsequential strong-field multiple ionization. The positions of the maxima are in accord with kinematical constraints set by the classical "rescattering model."

First observation of self-amplified spontaneous emission in a free-electron laser at 109 nm wavelength

We present the first observation of self-amplified spontaneous emission (SASE) in a free-electron laser (FEL) in the vacuum ultraviolet regime at 109 nm wavelength (11 eV). The observed free-electron laser gain (approximately 3000) and the radiation characteristics, such as dependency on bunch charge, angular distribution, spectral width, and intensity fluctuations, are all consistent with the present models for SASE FELs.

Towards time-resolved, coupled structure-function information on carotenoid excited state processes: X-ray and optical short-pulse double resonance spectroscopy.

A novel soft X-ray and optical short-pulse double resonance spectroscopic technique tailor-made to elucidate processes involving the optically forbidden S1 (2(1)A(g)) state of carotenoids in native biological samples (e.g., photosynthetic antenna complexes) is described. The principle relies on probing the near carbon K-edge absorption of the optically excited sample with soft X-rays generated by a laser-induced plasma. A first application concerns location of the 2(1)A(g) state of beta-carotene in vitro. Further applications are proposed.

Neutron energy spectra from the laser-induced Dd,n3He reaction.

Detailed neutron energy spectra were measured for the D(d,n)3He reaction induced in solid (CD2)(n) targets by irradiation with 50-fs 2 x 10(18) W/cm(2) light pulses from a 10-TW Ti:Sapphire laser. The neutrons were observed at two angles 5 degrees and 112 degrees relative to the incident laser beam. The neutron spectra at the two angles are characterized by peaks with large widths of about 700 keV full width at half maximum and a shift of 300 keV between them. Neutron energies of up to about 4 MeV were observed indicating that deuterons are accelerated up to an energy of 1 MeV in the laser produced plasma. Simulation calculations can describe qualitatively the neutron spectra by assuming isotropic deuteron acceleration and a reduction of the reaction probability by a factor of 1/3 for deuterons emitted from the front of the target. These calculations indicate in particular that it is necessary to assume deuterons moving both into and out of the front of the target in order to describe the neutron energy spectra at the two angles. The highest recorded mean neutron yield was about 10(4) neutrons per pulse. The neutron yield increases with the number of electrons emitted from the front of the target and with the intensity of the prompt gamma flash induced by the bremsstrahlung of energetic electrons.

Explosion characteristics of intense femtosecond-laser-driven water droplets.

An efficient acceleration of energetic ions is observed when small heavy-water droplets of approximately 20 microm diameter are exposed to ultrafast (approximately 40 fs) Ti:sapphire laser pulses of up to 10(19) W/cm2 intensity. Quantitative measurements of deuteron and neutron spectra were done, allowing one to analyze the outward and inward directed deuteron acceleration from the droplet. Neutron spectroscopy based on the D (d,n) fusion reaction was accomplished in four different spatial directions. The energy shifts of those fusion neutrons produced inside the exploding droplet reflect a remaining deuteron acceleration inside the irradiated droplet along the axis of the incident laser beam. The overall neutron yield of the microdroplets is relatively small as a result of the dominant outward directed acceleration of the deuterons with 1200 neutrons/shot. Relying on the "explosion-like" acceleration of such spherical droplet targets we have developed a spray target consisting of heavy-water microspheres with diameters of 150 nm . Both the high deuteron energies of up to 1 MeV resulting from the irradiation intensity of approximately 10(19) W/cm2 as well as the collisions between the deuterons and the surrounding spray delivered about one order of magnitude more neutrons than the single-droplet system. The approximately 6 x 10(3) neutrons per laser pulse from the spray can be attributed to an efficient deuteron release from a significantly smaller laser excited volume as from deuterium-cluster targets.

Absolute extreme ultraviolet yield from femtosecond-laser-excited Xe clusters.

Large Xe clusters (10(5)-10(6) atoms per cluster) have been irradiated with ultrashort (50 fs) and high-intensity ( approximately 2 x 10(18) W/cm(2)) pulses from a Ti:sapphire multi-TW laser at 800 nm wavelength. Scaling and absolute yield measurements of extreme ultraviolet (EUV) emission in a wavelength range between 7 and 15 nm in combination with cluster target characterization have been used for yield optimization. Maximum emission as a function of the backing pressure and a spatial emission anisotropy covering a factor of two at optimized yields is discussed with a simple model of the source geometry and EUV-radiation absorption. Circularly polarized laser light instead of linear polarization results in a factor of 2.5 higher emission in the 11 to 15 nm wavelength range. This indicates the initial influence of optical-field ionization for the interaction parameter range used and contrasts to collisional heating that seems to influence preferentially higher ionization. Absolute emission efficiency at 13.4 nm of up to 0.5% in 2pi sr and 2.2% bandwidth has been obtained.

Note: Thickness determination of freestanding ultra-thin foils using a table top laboratory extreme ultraviolet source.

We present a versatile and handy method allowing a thickness determination of freestanding thin plastic foils by its transmission characteristics in the extreme ultraviolet (EUV) spectrum. The method is based on a laser induced plasma source, emitting light in the EUV region, a compact double-mirror EUV monochromator operating at a fixed wavelength of 18.9 nm, and a CCD camera. The measurement delivers transmission values with a standard deviation of ΔT = 0.005 enabling foils thickness characterization with nm-accuracy at a given foil density and stoichiometric composition. Well characterized freestanding ultra-thin foils can be directly implemented in, e.g., high intensity laser matter experiments without further manipulation.