Upgraded Three-Wavelength Lidar for Real-Time Observations of Volcanic Aerosol Optical and Microphysical Properties at Etna (Italy): Calibration Procedures and Measurement Tests.

An innovative mobile lidar device, developed to monitor volcanic plumes during explosive eruptions at Mt. Etna (Italy) and to analyse the optical properties of volcanic particles, was upgraded in October 2023 with the aim of improving volcanic plume retrievals. The new configuration of the lidar allows it to obtain new data on both the optical and the microphysical properties of the atmospheric aerosol. In fact, after the upgrade, the lidar is able to measure three backscattering coefficients, two extinction coefficients and two depolarisation ratios in a configuration defined as "state-of-the-art lidar", where properties such as particle size distribution and the refractive index can be derived. During the lidar implementation, we were able to test the system's performance through specific calibration measurements. A comparison in an aerosol-free region (7.2-12 km) between lidar signals at 1064 nm, 532 nm and 355 nm and the corresponding pure molecular profiles showed a relative difference of <1% between them for all the wavelengths, highlighting the good dynamic of the signals. The overlap correction allowed us to reduce the underestimation of the backscattering coefficient from 50% to 10% below 450 m and 750 m at both 355 and 532 nm, respectively. The correct alignment between the laser beam and the receiver optical chain was tested using the signal received from the different quadrants of the telescope, and the relative differences between the four directions were comparable to zero, within the margin of error. Finally, the first measurement results are shown and compared with results obtained by other instruments, with the aim of proving the ability of the upgraded system to more precisely characterise aerosol optical and microphysical properties.

Dynamics of volcanic vortex rings.

Vortex rings can easily be generated in the laboratory or with homemade devices, but they have also been observed on volcanoes, since the eighteenth century. However, the physical conditions under which volcanic vortex rings form are still unknown. In order to better understand this phenomenon and provide clues on the dynamics of the volcanic vortex rings, we performed a series of finite element simulations to investigate which model configuration leads to the rings formation that best matches the field observations. Results show that the formation of volcanic vortex rings requires a combination of fast gas release from gas bubbles (slugs) at the top of the magma conduit and regularity in the shape of the emitting vent. Our findings offer important insights into the geometry of the uppermost portion of vortex-forming volcanic conduits. Volcanic vortex ring studies may form the basis for a cross-disciplinary assessment of the upper conduit dynamics of volcanic vents.

Assessment of eruption source parameters using infrasound and plume modelling: a case study from the 2021 eruption of Mt. Etna, Italy.

Atmospheric injection of volcanic ash during eruptions is a threat to aviation. Reliable forecast of airborne ash dispersal relies on empirical and numerical models. Key inputs into these models are so-called eruption source parameters such as the rate at which pyroclastic material is ejected from the vent and the maximum height of eruptive columns. Here, we use infrasound data recorded during eruptive activity in June 2021 at Mt. Etna, Italy, to demonstrate its potential for assessment of eruption rates in near-real time. We calculate a time series of flow velocity at the vent using data corrected for topographic scattering, and the effect of vent geometry on the acoustic source radiation. We obtain values of flow velocity of 50-125 m/s during a period of sustained, paroxysmal, activity. We use independent estimates from other ground-based remote sensing data to validate our results. Further, we use the infrasound-derived flow velocities as input into a 1D plume model to estimate the maximum height of the eruption column. Our results suggest that infrasound technology holds promise to assess eruption rates and inform modelling of volcanic plumes. We anticipate that implementation of real-time operational workflows based on infrasound data and plume modelling will impact decision-making and risk mitigation at active volcanoes.

Aeolus winds impact on volcanic ash early warning systems for aviation.

Forecasting volcanic ash atmospheric pathways is of utmost importance for aviation. Volcanic ash can interfere with aircraft navigational instruments and can damage engine parts. Early warning systems, activated after volcanic eruptions can alleviate the impacts on aviation by providing forecasts of the volcanic ash plume dispersion. The quality of these short-term forecasts is subject to the accuracy of the meteorological wind fields used for the initialization of regional models. Here, we use wind profiling data from the first high spectral resolution lidar in space, Aeolus, to examine the impact of measured wind fields on regional NWP and subsequent volcanic ash dispersion forecasts, focusing on the case of Etna's eruption on March 2021. The results from this case study demonstrate a significant improvement of the volcanic ash simulation when using Aeolus-assimilated meteorological fields, with differences in wind speed reaching up to 8 m/s when compared to the control run. When comparing the volcanic ash forecast profiles with downwind surface-based aerosol lidar observations, the modeled field is consistent with the measurements only when Aeolus winds are assimilated. This result clearly demonstrates the potential of Aeolus and highlights the necessity of future wind profiling satellite missions for improving volcanic ash forecasting and hence aviation safety.

Small-scale volcanic aerosols variability, processes and direct radiative impact at Mount Etna during the EPL-RADIO campaigns.

The aerosol properties of Mount Etna's passive degassing plume and its short-term processes and radiative impact were studied in detail during the EPL-RADIO campaigns (summer 2016-2017), using a synergistic combination of observations and radiative transfer modelling. Summit observations show extremely high particulate matter concentrations. Using portable photometers, the first mapping of small-scale (within [Formula: see text] from the degassing craters) spatial variability of the average size and coarse-to-fine burden proportion of volcanic aerosols is obtained. A substantial variability of the plume properties is found at these spatial scales, revealing that processes (e.g. new particle formation and/or coarse aerosols sedimentation) are at play, which are not represented with current regional scale modelling and satellite observations. Statistically significant progressively smaller particles and decreasing coarse-to-fine particles burden proportion are found along plume dispersion. Vertical structures of typical passive degassing plumes are also obtained using observations from a fixed LiDAR station constrained with quasi-simultaneous photometric observations. These observations are used as input to radiative transfer calculations, to obtain the shortwave top of the atmosphere (TOA) and surface radiative effect of the plume. For a plume with an ultraviolet aerosol optical depth of 0.12-0.14, daily average radiative forcings of [Formula: see text] and [Formula: see text], at TOA and surface, are found at a fixed location [Formula: see text] downwind the degassing craters. This is the first available estimation in the literature of the local radiative impact of a passive degassing volcanic plume.

Unravelling the links between seismo-acoustic signals and eruptive parameters: Etna lava fountain case study.

Deriving eruption source parameters from geophysical data is critical for volcano hazard mitigation, yet remains a challenging task in most volcanoes worldwide. In this work, we explored the temporal relationship between geophysical signals and eruptive parameters measured during six explosive episodes from the New South-East Crater of Mt. Etna (Italy). The quadratic reduced seismic velocity and pressure were calculated to track the temporal variation of volcanic elastic radiation, and the lava fountain height was estimated by thermal camera image processing. The temporal relationships between these geophysical and eruptive time series were studied. In particular, the first considered lava fountain exhibited a "clockwise hysteresis" pattern: higher seismic amplitude with respect to the fountain height during the waxing phase as compared to the waning phase. We also calculated the regression parameters for both linear and power laws, linking seismo-acoustic and eruptive time series. For the linear regressions, we found fairly constant values of the scaling factors in five out of six eruptive episodes, which can be considered as a promising step to derive eruption source parameters from geophysical data in real-time. Regarding power law regressions, a clear relationship was observed between the exponents determined for the power law linking quadratic reduced velocity and lava fountain height, and the time interval duration from the previous eruption. These results suggest that the condition of the uppermost part of the plumbing system (e.g. viscosity of residing magma and conduit conditions) play a key role in the seismic energy generation during the eruptions.

Quantification of ash sedimentation dynamics through depolarisation imaging with AshCam.

Even modest ash-rich volcanic eruptions can severely impact a range of human activities, especially air travel. The dispersal of ash in these eruptions depends critically on aggregation and sedimentation processes - however these are difficult to quantify in volcanic plumes. Here, we image ash dynamics from mild explosive activity at Santiaguito Volcano, Guatemala, by measuring the depolarisation of scattered sunlight by non-spherical ash particles, allowing the dynamics of diffuse ash plumes to be investigated with high temporal resolution (>1 Hz). We measure the ash settling velocity downwind from the main plume, and compare it directly with ground sampled ash particles, finding good agreement with a sedimentation model based on particle size. Our new, cost-effective technique leverages existing technology, opening a new frontier of integrated ash visualisation and ground collection studies which could test models of ash coagulation and sedimentation, leading to improved ash dispersion forecasts. This will provide risk managers with improved data quality on ash location, reducing the economic and societal impacts of future ash-rich eruptions.

Effect of particle volume fraction on the settling velocity of volcanic ash particles: insights from joint experimental and numerical simulations.

Most of the current ash transport and dispersion models neglect particle-fluid (two-way) and particle-fluid plus particle-particle (four-way) reciprocal interactions during particle fallout from volcanic plumes. These interactions, a function of particle concentration in the plume, could play an important role, explaining, for example, discrepancies between observed and modelled ash deposits. Aiming at a more accurate prediction of volcanic ash dispersal and sedimentation, the settling of ash particles at particle volume fractions (ϕp) ranging 10-7-10-3 was performed in laboratory experiments and reproduced by numerical simulations that take into account first the two-way and then the four-way coupling. Results show that the velocity of particles settling together can exceed the velocity of particles settling individually by up to 4 times for ϕp ~ 10-3. Comparisons between experimental and simulation results reveal that, during the sedimentation process, the settling velocity is largely enhanced by particle-fluid interactions but partly hindered by particle-particle interactions with increasing ϕp. Combining the experimental and numerical results, we provide an empirical model allowing correction of the settling velocity of particles of any size, density, and shape, as a function of ϕp. These corrections will impact volcanic plume modelling results as well as remote sensing retrieval techniques for plume parameters.

Balancing bulk gas accumulation and gas output before and during lava fountaining episodes at Mt. Etna.

We focus on a sequence of 9 lava fountains from Etna that occurred in 2011, separated by intervals of 5 to 10 days. Continuous measurements allowed to discover the occurrence of gravity decreases before the onset of most fountaining episodes. We propose that the gravity changes are due to the pre-fountaining accumulation of a foam layer at shallow levels in the plumbing system of the volcano. Relying on the relationship between amount of gas trapped in the foam and amount of gas emitted during each episode, we develop a conceptual model of the mechanism controlling the passage from Strombolian to lava fountaining activity. Gas leakage from the foam layer during the late stages of its accumulation increases the gas volume fraction at upper levels, thus inducing a decrease of the magma-static pressure in the trapping zone and a further growth of the foam. This feedback mechanism eventually leads to the collapse of the foam layer and to the onset of lava fountaining. The possibility to detect the development of a foam layer at depth and to set quantitative constraints on the amount of trapped gas is important because of the implications for forecasting explosive eruptions and predicting their intensity.