Anomalous Optical Properties of KTN:Li Ferroelectric Supercrystals.

We report a spectroscopic investigation of potassium-lithium-tantalate-niobate (KTN:Li) across its room-temperature ferroelectric phase transition, when the sample manifests a supercrystal phase. Reflection and transmission results indicate an unexpected temperature-dependent enhancement of average index of refraction from 450 nm to 1100 nm, with no appreciable accompanying increase in absorption. Second-harmonic generation and phase-contrast imaging indicate that the enhancement is correlated to ferroelectric domains and highly localized at the supercrystal lattice sites. Implementing a two-component effective medium model, the response of each lattice site is found to be compatible with giant broadband refraction.

Practical two-photon-absorption cross sections and spectra of eosin and hematoxylin.

We experimentally investigate the two-photon absorption cross sections and spectra of eosin and hematoxylin for applications in nonlinear microscopy. The experiments are carried out on pure samples of the two dyes in DI-water solvent with different concentrations, in the typical range employed in standard staining procedures. Nonlinear fluorescence is excited by a line-shaped beam emitted by a Ti:Sapphire mode-locked laser in the wavelength range from 740 to 880 nm and is detected through a microscope setup. The two-photon absorption spectral response is systematically analyzed and discussed. Finally, the staining is applied on biological tissue samples, which are imaged by two-photon microscopy. Our results show that the employed dyes are fully suitable for applications in nonlinear imaging.

Spatiotemporal amplitude and phase retrieval of space-time coupled ultrashort pulses using the Shackled-FROG technique.

We demonstrate the validity of the Shackled-frequency-resolved-optical-gating technique for the complete characterization, both in space and in time, of ultrashort optical pulses that present strong angular dispersion. Combining a simple imaging grating with a Hartmann-Shack sensor and standard frequency-resolved-optical-gating detection at a single spatial position, we are able to retrieve the full spatiotemporal structure of a tilted pulse.

Dispersive wave generation by solitons in microstructured optical fibers.

We study the nonlinear propagation of femtosecond pulses in the anomalous dispersion region of microstructured fibers, where soliton fission mechanisms play an important role. The experiment shows that the output spectrum contains, besides the infrared supercontinuum, a narrow-band 430-nm peak, carrying about one fourth of the input energy. By combining simulation and experiments, we explore the generation mechanism of the visible peak and describe its properties. The simulation demonstrates that the blue peak is generated only when the input pulse is so strongly compressed that the short-wavelength tail of the spectrum includes the wavelength predicted for the dispersive wave. In agreement with simulation, intensity-autocorrelation measurements show that the duration of the blue pulse is in the picosecond time range, and that, by increasing the input intensity, satellite pulses of lower intensity are generated.

Enhancement of stability and efficiency of a nonlinear mirror mode-locked Nd:YVO(4) oscillator by an active Q-switch.

The stability and the peak power of a nonlinear-mirror mode-locked Nd:YVO(4) laser are significantly increased by the insertion of an acousto-optic modulator inside the laser cavity. The repetition rate for reliable operation can be varied in the range 35 kHz - 50 kHz. The laser generates the most intense and stable mode-locked pulses of width 9 ps lying underneath a Q-switched envelope of width 110 ns with a Q-switch modulation frequency of 38 kHz. For 10 W of pump power, a 224 times enhancement of peak power over that of cw mode-locking is obtained under reliable Q-switched and mode-locked operation.

Simple and versatile dual-signal wave optical parametric oscillator.

A synchronously pumped optical parametric oscillator that is able to deliver a signal pulse at two different wavelengths either simultaneously or even one at a time is presented. As the operation exploits the group-velocity mismatch between the interacting signal and pump pulses, just a cavity-length adjustment is required to switch between the three regimes. The widely tunable signal pulses are shown to be synchronous and near transform limited.