Mesoscopic Stacking Reconfigurations in Stacked van der Waals Film.

Mesoscopic-scale stacking reconfigurations are investigated when van der Waals (vdW) films are stacked. A method to visualize complicated stacking structures and mechanical distortions simultaneously in stacked atom-thick films using Raman spectroscopy is developed. In the rigid limit, it is found that the distortions originate from the transfer process, which can be understood through thin film mechanics with a large elastic property mismatch. In contrast, with atomic corrugations, the in-plane strain fields are more closely correlated with the stacking configuration, highlighting the impact of atomic reconstructions on the mesoscopic scale. It is discovered that the grain boundaries do not have a significant effect while the cracks are causing inhomogeneous strain in stacked polycrystalline films. This result contributes to understanding the local variation of emerging properties from moiré structures and advancing the reliability of stacked vdW material fabrication.

Highly efficient diode-pumped alkali-vapor amplification with near-extreme-limit gain.

We report high-efficiency optical amplification with near-extreme-limit gain from a diode-pumped Cs vapor cell. We used wavelength-division multiplexing to couple 852 nm pump and 895 nm seed lasers to achieve nearly overlapping spatial modes in the Cs vapor cell. We investigated the amplification factor as a function of the focal length of the lens focusing on the combined pump and seed signals and determined the optimal focal length under our experimental conditions. The small-signal amplification factor from the Cs vapor cell reached >30 dB at 240 mW pump power, and the optimal optical amplification factor per pump power was 4171/W.

Ultrafast Fiber Lasers with Low-Dimensional Saturable Absorbers: Status and Prospects.

Wide-spectral saturable absorption (SA) in low-dimensional (LD) nanomaterials such as zero-, one-, and two-dimensional materials has been proven experimentally with outstanding results, including low saturation intensity, deep modulation depth, and fast carrier recovery time. LD nanomaterials can therefore be used as SAs for mode-locking or Q-switching to generate ultrafast fiber laser pulses with a high repetition rate and short duration in the visible, near-infrared, and mid-infrared wavelength regions. Here, we review the recent development of emerging LD nanomaterials as SAs for ultrafast mode-locked fiber laser applications in different dispersion regimes such as anomalous and normal dispersion regimes of the laser cavity operating in the near-infrared region, especially at ~1550 nm. The preparation methods, nonlinear optical properties of LD SAs, and various integration schemes for incorporating LD SAs into fiber laser systems are introduced. In addition to these, externally (electrically or optically) controlled pulsed fiber laser behavior and other characteristics of various LD SAs are summarized. Finally, the perspectives and challenges facing LD SA-based mode-locked ultrafast fiber lasers are highlighted.

Robust, low-noise, polarization-maintaining mode-locked Er-fiber laser with a planar lightwave circuit (PLC) device as a multi-functional element.

We demonstrate a new planar lightwave circuit (PLC)-based device, integrated with a 980/1550 wavelength division multiplexer, an evanescent-field-interaction-based saturable absorber, and an output tap coupler, which can be employed as a multi-functional element in mode-locked fiber lasers. Using this multi-functional PLC device, we demonstrate a simple, robust, low-noise, and polarization-maintaining mode-locked Er-fiber laser. The measured full-width at half-maximum bandwidth is 6 nm centered at 1555 nm, corresponding to 217 fs transform-limited pulse duration. The measured RIN and timing jitter are 0.22% [10 Hz-10 MHz] and 6.6 fs [10 kHz-1 MHz], respectively. Our results show that the non-gain section of mode-locked fiber lasers can be easily implemented as a single PLC chip that can be manufactured by a wafer-scale fabrication process. The use of PLC processes in mode-locked lasers has the potential for higher manufacturability of low-cost and robust fiber and waveguide lasers.

Optically controlled in-line graphene saturable absorber for the manipulation of pulsed fiber laser operation.

We demonstrate an optically tunable graphene saturable absorber to manipulate the laser operation in pulsed fiber laser system. Owing to the strongly enhanced evanescent field interaction with monolayer graphene, we could realize an efficient control of modulation depth in the graphene saturable absorber by optical means through cross absorption modulation method. By integrating the tunable graphene saturable absorber into the fiber laser system, we could switch the laser operation from Q-switching through Q-switched mode-locking to continuous wave mode-locking by adjusting only the optical power of the control beam. In addition, we realized a hybrid Q-switching of fiber laser by periodical modulation of the absorption of the graphene saturable absorber, where we observed that the repetition rate of the Q-switched laser could be continuously tuned according to the modulation frequency of the applied external signal.

All-fiber Tm-doped soliton laser oscillator with 6 nJ pulse energy based on evanescent field interaction with monoloayer graphene saturable absorber.

We demonstrate an all-fiber Tm-doped soliton laser with high power by using a monolayer graphene saturable absorber (SA). Large area, uniform monolayer graphene was transferred to the surface of the side-polished fiber (SPF) to realize an in-line graphene SA that operates around 2 µm wavelength. To increase the nonlinear interaction with graphene, we applied an over-cladding onto the SPF, where enhanced optical absorption at monolayer graphene was observed. All-fiber Tm-doped mode-locked laser was built including our in-line graphene SA, which stably delivered the soliton pulses with 773 fs pulse duration. The measured 3-dB spectral bandwidth was 5.14 nm at the wavelength of 1910 nm. We obtained the maximum average output power of 115 mW at a repetition rate of 19.31 MHz. Corresponding pulse energy was estimated to be 6 nJ, which is the highest value among all-fiber Tm-doped soliton oscillators using carbon-material-based SAs.

Q-switched operation of a femtosecond-laser-inscribed Yb:YAG channel waveguide laser using carbon nanotubes.

We demonstrate a diode-pumped femtosecond-laser-inscribed Yb:YAG channel waveguide laser, Q-switched by using single-walled carbon nanotubes (SWCNTs) near 1029 nm. We used saturable absorber mirrors (SAMs) fabricated by depositing SWCNTs on three different output couplers. Best performance of the 9.3-mm-long ultra-compact Q-switched waveguide laser is obtained with an output coupling transmission of 20%. In this case, a maximum average output power of 60 mW with a corresponding pulse energy of 37.7 nJ and a pulse duration of 88 ns at 1.59-MHz repetition rate were achieved. The highest pulse energy of 39.2 nJ and the shortest pulse duration of 78 ns were obtained with 30% and 10% output couplers, respectively.

Monolayer graphene saturable absorbers with strongly enhanced evanescent-field interaction for ultrafast fiber laser mode-locking.

We demonstrate an efficient all-fiber saturable absorber (SA) that evanescently interacts with a graphene monolayer. Strong nonlinear interaction between the graphene sheet and evanescent wave was realized in both experiments and numerical calculations by employing an over-cladding structure on high-quality monolayer graphene that uniformly covered the side-polished fiber. A passively mode-locked Er-doped fiber laser was built, including our in-line graphene SA, which stably generated ultrashort pulses with pulse duration of 377 fs at a repetition rate of 37.7 MHz. The corresponding 3-dB spectral bandwidth of the laser was measured to be 8.6 nm at the central wavelength of 1607.7 nm. We also experimentally observed that the spectral bandwidth and pulse duration of the laser output could be controlled by proper selection of the refractive index of the over-cladding material on the monolayer-graphene SA.

300-MHz-repetition-rate, all-fiber, femtosecond laser mode-locked by planar lightwave circuit-based saturable absorber.

We show the implementation of fiber-pigtailed, evanescent-field-interacting, single-walled carbon nanotube (CNT)-based saturable absorbers (SAs) using standard planar lightwave circuit (PLC) fabrication processes. The implemented PLC-CNT-SA device is employed to realize self-starting, high-repetition-rate, all-fiber ring oscillators at telecommunication wavelength. We demonstrate all-fiber Er ring lasers operating at 303-MHz (soliton regime) and 274-MHz (stretched-pulse regime) repetition-rates. The 303-MHz (274-MHz) laser centered at 1555 nm (1550 nm) provides 7.5 nm (19 nm) spectral bandwidth. After extra-cavity amplilfication, the amplified pulse train of the 303-MHz (274-MHz) laser delivers 209 fs (178 fs) pulses. To our knowledge, this corresponds to the highest repetition-rates achieved for femtosecond lasers employing evanescent-field-interacting SAs. The demonstrated SA fabrication method, which is based on well-established PLC processes, also shows a potential way for mass-producible and lower-cost waveguide-type SA devices suitable for all-fiber and waveguide lasers.

Broadband supercontinuum generation using a hollow optical fiber filled with copper-ion-modified DNA.

We experimentally demonstrated supercontinuum generation through a hollow core photonic bandgap fiber (HC-PBGF) filled with DNA nanocrystals modified by copper ions in a solution. Both double-crossover nano DNA structure and copper-ion-modified structure provided a sufficiently high optical nonlinearity within a short length of hollow optical fiber. Adding a higher concentration of copper ion into the DNA nanocrystals, the bandwidth of supercontinuum output was monotonically increased. Finally, we achieved the bandwidth expansion of about 1000 nm to be sufficient for broadband multi-spectrum applications.

Mode-locking of Er-doped fiber laser using a multilayer MoS2 thin film as a saturable absorber in both anomalous and normal dispersion regimes.

Application of a multilayer Molybdenum Disulfide (MoS2) thin film as a saturable absorber was experimentally demonstrated by realizing a stable and robust passive mode-locked fiber laser via the evanescent field interaction between the light and the film. The MoS2 film was grown by chemical vapor deposition, and was then transferred to a side polished fiber by a lift-off method. Intensity-dependent optical transmission through the MoS2 thin film on side polished fiber was experimentally observed showing efficient saturable absorption characteristics. Using erbium doped fiber as an optical gain medium, we built an all-fiber ring cavity, where the MoS2 film on the side polished fiber was inserted as a saturable absorber. Stable dissipative soliton pulse trains were successfully generated in the normal dispersion regime with a spectral bandwidth of 23.2 nm and the pulse width of 4.98 ps. By adjusting the total dispersion in the cavity, we also obtained soliton pulses with a width of 637 fs in the anomalous dispersion regime near the lasing wavelength λ = 1.55 µm. Detailed and systematic experimental comparisons were made for stable mode locking of an all-fiber laser cavity in both the normal and anomalous regimes.

All-fiber mode-locked laser oscillator with pulse energy of 34 nJ using a single-walled carbon nanotube saturable absorber.

We demonstrate a dissipative soliton fiber laser with high pulse energy (>30 nJ) based on a single-walled carbon nanotube saturable absorber (SWCNT-SA). In-line SA that evanescently interacts with the high quality SWCNT/polymer composite film was fabricated under optimized conditions, increasing the damage threshold of the saturation fluence of the SA to 97 mJ/cm(2). An Er-doped mode-locked all-fiber laser operating at net normal intra-cavity dispersion was built including the fabricated in-line SA. The laser stably delivers linearly chirped pulses with a pulse duration of 12.7 ps, and exhibits a spectral bandwidth of 12.1 nm at the central wavelength of 1563 nm. Average power of the laser output is measured as 335 mW at an applied pump power of 1.27 W. The corresponding pulse energy is estimated to be 34 nJ at the fundamental repetition rate of 9.80 MHz; this is the highest value, to our knowledge, reported in all-fiber Er-doped mode-locked laser using an SWCNT-SA.

Carbon nanostructure-based saturable absorber mirror for a diode-pumped 500-MHz femtosecond Yb:KLu(WO4)2 laser.

We report a diode-pumped Yb:KLu(WO(4))(2) (Yb:KLuW) laser passively mode-locked by employing a carbon nanostructure-based multi-functional saturable absorber mirror. Two types of carbon nanostructures, single-walled carbon nanotubes (SWCNTs) and graphene, were deposited on a single dielectric mirror and applied both for stable mode-locking of the Yb:KLuW laser near 1050 nm in a compact cavity configuration. The carbon nanostructure mode-locked laser delivers 157-fs pulses with output powers of up to 85 mW at a repetition rate of 500 MHz.

Pulse width shaping of passively mode-locked soliton fiber laser via polarization control in carbon nanotube saturable absorber.

We report the continuous control of the pulse width of a passively mode-locked fiber laser via polarization state adjustment in a single-walled carbon nanotube saturable absorber (SWCNT-SA). The SWCNT, coated on the side-polished fiber, was fabricated with optimized conditions and used for stable mode-locking of the fiber laser without Q-switching instabilities for any polarization state of the laser intra-cavity. The 3-dB spectral bandwidth of the mode-locked pulses can be continuously tuned from 1.8 nm to 8.5 nm with the polarization control for a given laser cavity length and applied pump power. A pulse duration varying from 470 fs to 1.6 ps was also observed with a change in the spectral bandwidth. The linear and the nonlinear transmission properties of the SA were analyzed, and found to exhibit different modulation depths depending on the input polarization state in the SA. The largest modulation depth of the SA was observed at the polarization state of the transverse electric mode that delivers shortest pulses at the laser output.

Yb:KYW planar waveguide laser Q-switched by evanescent-field interaction with carbon nanotubes.

We report Q-switched operation of a planar waveguide laser by evanescent-field interaction with single-walled carbon nanotubes deposited on top of the waveguide. The saturable-absorber-integrated gain medium, which operates based on evanescent-field interaction, enables the realization of a diode-pumped 2.5-cm-long Q-switched Yb:KYW waveguide laser emitting at 1030 nm. With such a compact cavity design, we achieve maximum output powers of up to 30 mW, corresponding to a single-pulse energy of 124 nJ, at 241 kHz repetition rate. The shortest pulse duration of 433 ns is generated at a repetition rate of 231 kHz.

Highly nonlinear optic nucleic acid thin-solid film to generate short pulse laser.

Using aqueous precursors, we report successfully fabricating thin-solid films of two nucleic acids, ribonucleic acid (RNA) and deoxyribonucleic acid (DNA). We investigated the potential of these films deposited on a fiber optic platform as all-fiber integrated saturable absorbers (SAs) for ultrafast nonlinear optics. RNA-SA performances were comparable to those of DNA-SA in terms of its nonlinear transmission, modulation depth, and saturation intensity. Upon insertion of these devices into an Erbium-doped fiber ring-laser cavity, both RNA and DNA SAs enabled efficient passive Q-switching operation. RNA-SA application further facilitated robust mode-locking and generated a transform-limited soliton pulse, exhibiting a pulse duration of 633 femtoseconds. A detailed analysis of these pulsed laser characteristics compared RNA and DNA fiber optic SAs with other nonlinear optic materials. The findings of this research establish the feasibility of utilizing RNA as a saturable absorber in ultrafast laser systems with an equal or higher potential as DNA, which presents novel possibilities for the nonlinear photonic applications of nucleic acid thin solid films.

175 fs Tm:Lu2O3 laser at 2.07 µm mode-locked using single-walled carbon nanotubes.

Single-walled carbon nanotube saturable absorbers were designed and fabricated for passive mode-locking of bulk lasers operating in the 2 µm spectral range. Mode-locked lasers based on Tm:Lu2O3 single crystals containing different Tm3+-doping concentrations were studied. Nearly transform-limited pulses as short as 175 fs at 2070 nm were generated at 88 MHz repetition rate.

Graphene-filled hollow optical fiber saturable absorber for efficient soliton fiber laser mode-locking.

We demonstrate a novel in-line saturable absorber based on hollow optical fiber (HOF) filled with graphene composite for high power operation of mode-locked fiber laser. Evanescent field of guided mode propagating in few centimeter-long HOF interacts with the graphene/polyvinyl acetate (PVAc) composite, which enables robust and efficient nonlinear absorption leading to stable passive mode-locking. The mode-locked fiber laser generates soliton pulses with 5.9-nm spectral bandwidth and its maximum output power is measured up to 80 mW. We also observe passive harmonic mode-locking of soliton laser delivering stable pulses with a repetition rate of 506.9 MHz at 33rd harmonics.

Toward higher-order passive harmonic mode-locking of a soliton fiber laser.

We report >13 MHz/mW pump power efficiency in increasing the repetition rate of passive harmonic mode-locking by engineering the soliton pulse energy in Er fiber lasers incorporating carbon nanotube saturable absorber. Stable pulses with a ∼5 GHz repetition rate and 40 dB of super-mode suppression are demonstrated with only ∼400 mW pump power in a single-clad fiber laser.

Low noise GHz passive harmonic mode-locking of soliton fiber laser using evanescent wave interaction with carbon nanotubes.

Passive harmonic mode-locking in soliton fiber laser is presented with excellent noise characteristics by employing a single-walled carbon nanotubes saturable absorber designed to interact with evanescent wave of the laser field. The 34(th) harmonic mode-locking pulses at 943.16 MHz repetition rate were stably generated with 18 mW output power, >50 dB side-mode suppression and -140 dB/Hz relative intensity noise. Soliton energy control with polarization controller further increased the harmonic order to 61st, 1.692 GHz, but with compromised performance. Scaling to higher-order harmonic mode-locking is discussed for practical application in optical communication system.