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1.
Sensors (Basel) ; 23(1)2022 Dec 28.
Artigo em Inglês | MEDLINE | ID: mdl-36616925

RESUMO

In the optical system for reconstructing speech signals based on laser speckle images, the resonance between the sound source and nearby objects leads to frequency response problem, which seriously affects the accuracy of reconstructed speech. In this paper, we propose a speech enhancement algorithm to reduce the frequency response. The results show that after using the speech enhancement algorithm, the frequency spectrum correlation coefficient between the reconstructed sinusoidal signal and the original sinusoidal signal is improved by up to 82.45%, and the real speech signal is improved by up to 56.40%. This proves that the speech enhancement algorithm is a valuable tool for solving the frequency response problem and improving the accuracy of reconstructed speech.


Assuntos
Dispositivos Ópticos , Fala , Algoritmos , Lasers
2.
Angew Chem Int Ed Engl ; 61(23): e202117698, 2022 Jun 07.
Artigo em Inglês | MEDLINE | ID: mdl-35315956

RESUMO

High-silica zeolite Y (FAU) plays a vital role in (petro)chemical industries. However, the slow nucleation and growth kinetics of the high-silica FAU framework limit its direct synthesis and the improvement of framework SiO2 /Al2 O3 ratio (SAR). Here, a facile strategy is developed to realize the fast crystallization of high-silica zeolite Y, which involves the combination of high crystallization temperature, ultra-stable Y (USY) seeds and efficient organic-structure directing agent (OSDA). The synthesis can be finished in 5-16 h at 160 °C and with tunable SAR up to 18.2, and the key factors affecting crystallization kinetics and phase purity are elucidated. Moreover, the crystallization process was monitored to reveal the fast crystal growth mechanism. The high-silica products possess high (hydro)thermal stability and abundant strong acid sites, which endow them excellent catalytic cracking performance, obviously superior to commercial USY.

3.
Micromachines (Basel) ; 15(6)2024 May 21.
Artigo em Inglês | MEDLINE | ID: mdl-38930639

RESUMO

With the continuous development of wireless communication technology, the frequency band of 6G communication systems is moving towards higher frequencies such as millimeter waves and terahertz. In such high-frequency situations, wireless transmission requires antenna modules to be provided with characteristics of miniaturization, high integration, and high gain, which presents new challenges to the development of antenna technology. In this article, a 4 × 4 antenna array using multilayered low-temperature co-fired ceramic is proposed, operating in W-band, with a feeding network based on substrate-integrated waveguide, and an antenna element formed through the combination of a substrate-integrated cavity and surface parasitic patches, which guaranteed the array to possess the advantages of high integration and high gain. Combined with the substrate-integrated waveguide to a rectangular waveguide transition structure designed in the early stage, a physical array with a standard metal rectangular waveguide interface was fabricated and tested. The test results show that the gain of the antenna array is higher than 18 dBi from 88 to 98 GHz, with a maximum of 20.4 dBi.

4.
Chem Commun (Camb) ; 57(40): 4898-4901, 2021 May 18.
Artigo em Inglês | MEDLINE | ID: mdl-33870354

RESUMO

Na+-free Cu-SSZ-13 zeolites have been rationally synthesized via a cooperative strategy, which has the advantages of rapid crystallization (9-48 h), high yield (86-94%) and adjustable Cu content. The NH3-SCR catalytic performance and hydrothermal stability of the calcined materials were studied and correlated with their physicochemical properties.

5.
Adv Mater ; 32(26): e2000272, 2020 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-32430991

RESUMO

High-silica zeolite Y is a desired catalytic material for oil refining and the petrochemical industry. However, its direct synthesis remains a symbolic challenge in the field of zeolite synthesis, with a limited improvement of the framework SiO2 /Al2 O3 ratio (SAR) from ≈5 to 9 over the past 60 years. Here, the synthesis of highly siliceous zeolite Y with tunable SAR up to 15.6 through a cooperative strategy is reported, which involves the use of FAU nuclei, a bulky organic structure-directing agent (OSDA), and a gel system with low alkalinity (named NOA-co strategy). A series of quaternary alkylammonium ions is discovered as effective OSDAs based on the NOA-co strategy, and the relevant crystallization mechanism is elucidated. Moreover, the high-silica products are demonstrated to have greatly improved (hydro)thermal stability, high concentration of strong acid sites, and uniform acid distribution, which lead to superior catalytic performance in the cracking of bulky hydrocarbons. It is anticipated that this synthetic strategy will benefit the synthesis and development of zeolitic catalysts in a wide range of reaction processes.

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