Do dielectric nanostructures turn metallic in high-electric dc fields?
Nano Lett
; 14(11): 6066-72, 2014 Nov 12.
Article
em En
| MEDLINE
| ID: mdl-25271987
ABSTRACT
Three-dimensional dielectric nanostructures have been analyzed using field ion microscopy (FIM) to study the electric dc field penetration inside these structures. The field is proved to be screened within a few nanometers as theoretically calculated taking into account the high-field impact ionization process. Moreover, the strong dc field of the order of 0.1 V/Å at the surface inside a dielectric nanostructure modifies its band structure leading to a strong band gap shrinkage and thus to a strong metal-like optical absorption near the surface. This metal-like behavior was theoretically predicted using first-principle calculations and experimentally proved using laser-assisted atom probe tomography (APT). This work opens up interesting perspectives for the study of the performance of all field-effect nanodevices, such as nanotransistor or super capacitor, and for the understanding of the physical mechanisms of field evaporation of dielectric nanotips in APT.
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01-internacional
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MEDLINE
Idioma:
En
Ano de publicação:
2014
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Article