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Characterization of the [3Fe-4S](0/1+) cluster from the D14C variant of Pyrococcus furiosus ferredoxin via combined NRVS and DFT analyses.
Lauterbach, Lars; Gee, Leland B; Pelmenschikov, Vladimir; Jenney, Francis E; Kamali, Saeed; Yoda, Yoshitaka; Adams, Michael W W; Cramer, Stephen P.
Afiliação
  • Lauterbach L; Department of Chemistry, University of California, Davis, CA 95616, USA and Institut für Chemie, Technische Universität Berlin, 10623 Berlin, Germany. lars.lauterbach@tu-berlin.de pelmentschikov@tu-berlin.de.
  • Gee LB; Department of Chemistry, University of California, Davis, CA 95616, USA.
  • Pelmenschikov V; Institut für Chemie, Technische Universität Berlin, 10623 Berlin, Germany. lars.lauterbach@tu-berlin.de pelmentschikov@tu-berlin.de.
  • Jenney FE; Georgia Campus, Philadelphia College of Osteopathic Medicine, Suwanee, GA 30024, USA.
  • Kamali S; Department of Chemistry, University of California, Davis, CA 95616, USA and Department of Mechanical, Aerospace and Biomedical Engineering, University of Tennessee Space Institute, Tullahoma, TN 37388, USA.
  • Yoda Y; JASRI, SPring-8, Sayo-gun, Hyogo 679-5198, Japan.
  • Adams MW; Department of Biochemistry & Molecular Biology, Life Sciences Building, University of Georgia, Athens, GA 30602, USA.
  • Cramer SP; Department of Chemistry, University of California, Davis, CA 95616, USA and Physical Biosciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.
Dalton Trans ; 45(17): 7215-9, 2016 04 25.
Article em En | MEDLINE | ID: mdl-27063792
ABSTRACT
The D14C variant of Pyrococcus furiosus ferredoxin provides an extraordinary framework to investigate a [3Fe-4S] cluster at two oxidation levels and compare the results to its physiologic [4Fe-4S] counterpart in the very same protein. Our spectroscopic and computational study reveals vibrational property changes related to the electronic and structural aspects of both Fe-S clusters.
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Assunto principal: Pyrococcus furiosus / Ferredoxinas Idioma: En Ano de publicação: 2016 Tipo de documento: Article
Texto completo
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PubMed Links
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Assunto principal: Pyrococcus furiosus / Ferredoxinas Idioma: En Ano de publicação: 2016 Tipo de documento: Article