Toroidal Droplets: Growth Rates, Dispersion Relations, and Behavior in the Thick-Torus Limit.

ABSTRACT

Toroidal droplets in a viscous liquid are unstable and transform into single or multiple spherical droplets. For thin tori, this can happen via the Rayleigh-Plateau instability causing the breakup of cylindrical jets. In contrast, for thick tori, this can happpen via the shrinking of the "hole". In this work, we use the thin-torus limit to directly measure the growth rate associated with capillary disturbances. In the case of toroidal droplets inside a much more viscous liquid, we even obtain the full dispersion relation, which is in agreement with theoretical results for cylindrical jets. For thick tori, we employ particle image velocimetry to determine the flow field of a sinking toroidal drop inside another viscous liquid. We find that the presence of the "hole" greatly suppresses one of the circulation loops expected for sinking cylinders. Finally, using the flow field of a shrinking toroidal droplet and the time-reversal symmetry of the Stokes equations, we theoretically predict the expected shape deformation of an expanding torus and confirm the result experimentally using charged toroidal droplets.