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Dual-Gated Transistor Platform for On-Site Detection of Lead Ions at Trace Levels.
Venkatesh, Shishir; Li, Tan; Wang, Xiang-Sheng; Yeung, Chi-Chung; Pei, Ke; Sun, Qi-Jun; Wu, Wei; Li, Robert K Y; Lam, Michael H W; Chan, Paddy K L; Wylie, Jonathan J; Roy, Vellaisamy A L.
Afiliação
  • Venkatesh S; State Key Laboratory for Millimeter Waves and Department of Material Science & Engineering , City University of Hong Kong , 83 Tat Chee Avenue , Kowloon , Hong Kong, S.A.R.
  • Li T; State Key Laboratory for Millimeter Waves and Department of Material Science & Engineering , City University of Hong Kong , 83 Tat Chee Avenue , Kowloon , Hong Kong, S.A.R.
  • Wang XS; Department of Mathematics , University of Louisiana at Lafayette , Lafayette , Louisiana 70503 , United States.
  • Yeung CC; Department of Chemistry , City University of Hong Kong , 83 Tat Chee Avenue , Kowloon , Hong Kong, S.A.R.
  • Pei K; Department of Mechanical Engineering , The University of Hong Kong , Pokfulam , Hong Kong, S.A.R.
  • Sun QJ; State Key Laboratory for Millimeter Waves and Department of Material Science & Engineering , City University of Hong Kong , 83 Tat Chee Avenue , Kowloon , Hong Kong, S.A.R.
  • Wu W; State Key Laboratory for Millimeter Waves and Department of Material Science & Engineering , City University of Hong Kong , 83 Tat Chee Avenue , Kowloon , Hong Kong, S.A.R.
  • Li RKY; State Key Laboratory for Millimeter Waves and Department of Material Science & Engineering , City University of Hong Kong , 83 Tat Chee Avenue , Kowloon , Hong Kong, S.A.R.
  • Lam MHW; Department of Chemistry , City University of Hong Kong , 83 Tat Chee Avenue , Kowloon , Hong Kong, S.A.R.
  • Chan PKL; Department of Mechanical Engineering , The University of Hong Kong , Pokfulam , Hong Kong, S.A.R.
  • Wylie JJ; Department of Mathematics , City University of Hong Kong , 83 Tat Chee Avenue , Kowloon , Hong Kong, S.A.R.
  • Roy VAL; State Key Laboratory for Millimeter Waves and Department of Material Science & Engineering , City University of Hong Kong , 83 Tat Chee Avenue , Kowloon , Hong Kong, S.A.R.
Anal Chem ; 90(12): 7399-7405, 2018 06 19.
Article em En | MEDLINE | ID: mdl-29812910
ABSTRACT
On-site monitoring of heavy metals in drinking water has become crucial because of several high profile instances of contamination. Presently, reliable techniques for trace level heavy metal detection are mostly laboratory based, while the detection limits of contemporary field-based methods are barely meeting the exposure limits set by regulatory bodies such as the World Health Organization (WHO). Here, we show an on-site deployable, Pb2+ sensor on a dual-gated transistor platform whose lower detection limit is 2 orders of magnitude better than the traditional sensor and 1 order of magnitude lower than the exposure limit set by WHO. The enhanced sensitivity of our design is verified by numerically solving PNP (Planck-Nernst-Poisson) model. We demonstrate that the enhanced sensitivity is due to the suppression of ionic flux. The simplicity and the robustness of the design make it applicable for on-site screening, thereby facilitating rapid response to contamination events.
Assuntos

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Assunto principal: Água Potável / Chumbo Tipo de estudo: Diagnostic_studies Idioma: En Ano de publicação: 2018 Tipo de documento: Article

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Assunto principal: Água Potável / Chumbo Tipo de estudo: Diagnostic_studies Idioma: En Ano de publicação: 2018 Tipo de documento: Article