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Zirconium-Assisted Activation of Palladium To Boost Syngas Production by Methane Dry Reforming.
Köpfle, Norbert; Götsch, Thomas; Grünbacher, Matthias; Carbonio, Emilia A; Hävecker, Michael; Knop-Gericke, Axel; Schlicker, Lukas; Doran, Andrew; Kober, Delf; Gurlo, Aleksander; Penner, Simon; Klötzer, Bernhard.
Afiliação
  • Köpfle N; Institute of Physical Chemistry, University of Innsbruck, Innrain 52 c, 6020, Innsbruck, Austria.
  • Götsch T; Institute of Physical Chemistry, University of Innsbruck, Innrain 52 c, 6020, Innsbruck, Austria.
  • Grünbacher M; Institute of Physical Chemistry, University of Innsbruck, Innrain 52 c, 6020, Innsbruck, Austria.
  • Carbonio EA; Department of Inorganic Chemistry, Fritz-Haber-Institute of the Max-Planck-Society, Faradayweg 4-6, 14195, Berlin, Germany.
  • Hävecker M; Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, BESSY II, Albert-Einstein-Straße 15, 12489, Berlin, Germany.
  • Knop-Gericke A; Department of Inorganic Chemistry, Fritz-Haber-Institute of the Max-Planck-Society, Faradayweg 4-6, 14195, Berlin, Germany.
  • Schlicker L; Department of Inorganic Chemistry, Fritz-Haber-Institute of the Max-Planck-Society, Faradayweg 4-6, 14195, Berlin, Germany.
  • Doran A; Fachgebiet Keramische Werkstoffe, Institut für Werkstoffwissenschaften und -technologien, Technische Universität Berlin, Hardenbergstr. 40, 10623, Berlin, Germany.
  • Kober D; Advanced Light Source, Beamline 12.2.2., Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.
  • Gurlo A; Fachgebiet Keramische Werkstoffe, Institut für Werkstoffwissenschaften und -technologien, Technische Universität Berlin, Hardenbergstr. 40, 10623, Berlin, Germany.
  • Penner S; Fachgebiet Keramische Werkstoffe, Institut für Werkstoffwissenschaften und -technologien, Technische Universität Berlin, Hardenbergstr. 40, 10623, Berlin, Germany.
  • Klötzer B; Institute of Physical Chemistry, University of Innsbruck, Innrain 52 c, 6020, Innsbruck, Austria.
Angew Chem Int Ed Engl ; 57(44): 14613-14618, 2018 Oct 26.
Article em En | MEDLINE | ID: mdl-30179293
ABSTRACT
C-saturated Pd0 nanoparticles with an extended phase boundary to ZrO2 evolve from a Pd0 Zr0 precatalyst under CH4 dry reforming conditions. This highly active catalyst state fosters bifunctional action CO2 is efficiently activated at oxidic phase boundary sites and Pdx C provides fast supply of C-atoms toward the latter.
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2018 Tipo de documento: Article
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2018 Tipo de documento: Article