Unlocking the ultrafast potential of gold nanowires for mode-locking in the mid-infrared region.

ABSTRACT

In this Letter, we present the mode-locking operation of a 2.87 µm Ho3+/Pr3+ codoped fluoride fiber laser, helped by the ultrafast nonlinear optical absorption behavior of gold nanowires (GNWs). The mode locker is fabricated by depositing the GNW solution onto a silver mirror. It has a modulation depth of 14.2%, a saturation intensity of 26.2MW/cm2, and a non-saturation loss of 29.9% at 2.87 µm. With an increased pump power, the laser operates in Q-switched mode-locking, fundamental mode-locking, and harmonic mode-locking (HML) states. This represents the first, to our knowledge, mid-infrared mode-locked laser using gold nanomaterials. Additionally, the HML is also the first observation in a laser in this band using material saturable absorbers, implying the capability of GNWs for high repetition rate generation.