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Mass Production of Sulfur-Tuned Single-Atom Catalysts for Zn-Air Batteries.
Chen, Zehong; Peng, Xinwen; Chen, Zhongxin; Li, Tingzhen; Zou, Ren; Shi, Ge; Huang, Yongfa; Cui, Peng; Yu, Jian; Chen, Yuling; Chi, Xiao; Loh, Kian Ping; Liu, Zhaoqing; Li, Xuehui; Zhong, Linxin; Lu, Jun.
Afiliação
  • Chen Z; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Peng X; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Chen Z; School of Science and Engineering, The Chinese University of Hong Kong, Shenzhen, Guangdong, 518172, China.
  • Li T; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Zou R; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Shi G; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Huang Y; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Cui P; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Yu J; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Chen Y; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Chi X; Department of Chemistry and Centre for Advanced 2D Materials (CA2DM), National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
  • Loh KP; Department of Chemistry and Centre for Advanced 2D Materials (CA2DM), National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
  • Liu Z; School of Chemistry and Chemical Engineering/Guangzhou Key Laboratory for Clean Energy and Materials/Key Laboratory for Water Quality and Conservation of the Pearl River Delta, Ministry of Education, Guangzhou University, No. 230 Wai Huan Xi Road, Guangzhou, 510006, China.
  • Li X; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Zhong L; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, 510641, China.
  • Lu J; College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, Zhejiang, 310027, China.
Adv Mater ; 35(15): e2209948, 2023 Apr.
Article em En | MEDLINE | ID: mdl-36652951
ABSTRACT
Single-atom catalysts (SACs) show great potential for rechargeable Zn-air batteries (ZABs); however, scalable production of SACs from sustainable resources is difficult owing to poor control of the local coordination environment. Herein, lignosulfonate, a by-product of the papermaking industry, is utilized as a multifunctional bioligand for the mass production of SACs with highly active MN4 S sites (M represents Fe, Cu, and Co) via strong metalnitrogen/sulfur coordination. This effectively adjusts the charge distribution and promotes the catalytic performance, leading to highly durable and excellent performance in oxygen reduction and evolution reactions for ZABs. This study paves the way for the industrial production of cost-effective SACs in a sustainable manner.
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2023 Tipo de documento: Article
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2023 Tipo de documento: Article