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A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economy.
Shaw, Wendy J; Kidder, Michelle K; Bare, Simon R; Delferro, Massimiliano; Morris, James R; Toma, Francesca M; Senanayake, Sanjaya D; Autrey, Tom; Biddinger, Elizabeth J; Boettcher, Shannon; Bowden, Mark E; Britt, Phillip F; Brown, Robert C; Bullock, R Morris; Chen, Jingguang G; Daniel, Claus; Dorhout, Peter K; Efroymson, Rebecca A; Gaffney, Kelly J; Gagliardi, Laura; Harper, Aaron S; Heldebrant, David J; Luca, Oana R; Lyubovsky, Maxim; Male, Jonathan L; Miller, Daniel J; Prozorov, Tanya; Rallo, Robert; Rana, Rachita; Rioux, Robert M; Sadow, Aaron D; Schaidle, Joshua A; Schulte, Lisa A; Tarpeh, William A; Vlachos, Dionisios G; Vogt, Bryan D; Weber, Robert S; Yang, Jenny Y; Arenholz, Elke; Helms, Brett A; Huang, Wenyu; Jordahl, James L; Karakaya, Canan; Kian, Kourosh Cyrus; Kothandaraman, Jotheeswari; Lercher, Johannes; Liu, Ping; Malhotra, Deepika; Mueller, Karl T; O'Brien, Casey P.
Afiliação
  • Shaw WJ; Pacific Northwest National Laboratory, Richland, WA, USA. Wendy.shaw@pnnl.gov.
  • Kidder MK; Oak Ridge National Laboratory, Oak Ridge, TN, USA. kidderm@ornl.gov.
  • Bare SR; SLAC National Accelerator Laboratory, Menlo Park, CA, USA. srbare@slac.stanford.edu.
  • Delferro M; Argonne National Laboratory, Lemont, IL, USA. delferro@anl.gov.
  • Morris JR; Ames National Laboratory, Ames, IA, USA. morrisj@ameslab.gov.
  • Toma FM; Lawrence Berkeley National Laboratory, Berkeley, CA, USA. fmtoma@lbl.gov.
  • Senanayake SD; Institute of Functional Materials for Sustainability, Helmholtz Zentrum Hereon, Teltow, Brandenburg, Germany. fmtoma@lbl.gov.
  • Autrey T; Brookhaven National Laboratory, Upton, NY, USA. ssenanay@bnl.gov.
  • Biddinger EJ; Pacific Northwest National Laboratory, Richland, WA, USA.
  • Boettcher S; Department of Chemical Engineering, The City College of New York, New York, NY, USA.
  • Bowden ME; Lawrence Berkeley National Laboratory, Berkeley, CA, USA.
  • Britt PF; Department of Chemical & Biomolecular Engineering and Department of Chemistry, University of California, Berkeley, Berkeley, CA, USA.
  • Brown RC; Pacific Northwest National Laboratory, Richland, WA, USA.
  • Bullock RM; Oak Ridge National Laboratory, Oak Ridge, TN, USA.
  • Chen JG; Department of Mechanical Engineering, Iowa State University, Ames, IA, USA.
  • Daniel C; Pacific Northwest National Laboratory, Richland, WA, USA.
  • Dorhout PK; Brookhaven National Laboratory, Upton, NY, USA.
  • Efroymson RA; Department of Chemical Engineering, Columbia University, New York, NY, USA.
  • Gaffney KJ; Argonne National Laboratory, Lemont, IL, USA.
  • Gagliardi L; Vice President for Research, Iowa State University, Ames, IA, USA.
  • Harper AS; Oak Ridge National Laboratory, Oak Ridge, TN, USA.
  • Heldebrant DJ; SLAC National Accelerator Laboratory, Menlo Park, CA, USA.
  • Luca OR; Department of Chemistry, The University of Chicago, Chicago, IL, USA.
  • Lyubovsky M; Pacific Northwest National Laboratory, Richland, WA, USA.
  • Male JL; Pacific Northwest National Laboratory, Richland, WA, USA.
  • Miller DJ; Chemical Engineering and Bioengineering, Washington State University, Pullman, WA, USA.
  • Prozorov T; Department of Chemistry, University of Colorado Boulder, Boulder, CO, USA.
  • Rallo R; Booz Allen Hamilton, Washington DC, USA.
  • Rana R; Pacific Northwest National Laboratory, Richland, WA, USA.
  • Rioux RM; Biological Systems Engineering Department, Washington State University, Pullman, WA, USA.
  • Sadow AD; Lawrence Berkeley National Laboratory, Berkeley, CA, USA.
  • Schaidle JA; Ames National Laboratory, Ames, IA, USA.
  • Schulte LA; Pacific Northwest National Laboratory, Richland, WA, USA.
  • Tarpeh WA; Department of Chemical Engineering, University of California, Davis, CA, USA.
  • Vlachos DG; Department of Chemical Engineering, The Pennsylvania State University, University Park, PA, USA.
  • Vogt BD; Ames National Laboratory, Ames, IA, USA.
  • Weber RS; Department of Chemistry, Iowa State University, Ames, IA, USA.
  • Yang JY; National Renewable Energy Laboratory, Golden, CO, USA.
  • Arenholz E; Department of Natural Resource Ecology and Management, Iowa State University, Ames, IA, USA.
  • Helms BA; Department of Chemical Engineering, Stanford University, Stanford, CA, USA.
  • Huang W; Department of Chemical and Biomolecular Engineering, University of Delaware, Newark, DE, USA.
  • Jordahl JL; Department of Chemical Engineering, The Pennsylvania State University, University Park, PA, USA.
  • Karakaya C; Pacific Northwest National Laboratory, Richland, WA, USA.
  • Kian KC; Department of Chemistry, University of California Irvine, Irvine, CA, USA.
  • Kothandaraman J; Pacific Northwest National Laboratory, Richland, WA, USA.
  • Lercher J; Lawrence Berkeley National Laboratory, Berkeley, CA, USA.
  • Liu P; Ames National Laboratory, Ames, IA, USA.
  • Malhotra D; Department of Chemistry, Iowa State University, Ames, IA, USA.
  • Mueller KT; Department of Natural Resource Ecology and Management, Iowa State University, Ames, IA, USA.
  • O'Brien CP; Oak Ridge National Laboratory, Oak Ridge, TN, USA.
Nat Rev Chem ; 8(5): 376-400, 2024 May.
Article em En | MEDLINE | ID: mdl-38693313
ABSTRACT
Electrification to reduce or eliminate greenhouse gas emissions is essential to mitigate climate change. However, a substantial portion of our manufacturing and transportation infrastructure will be difficult to electrify and/or will continue to use carbon as a key component, including areas in aviation, heavy-duty and marine transportation, and the chemical industry. In this Roadmap, we explore how multidisciplinary approaches will enable us to close the carbon cycle and create a circular economy by defossilizing these difficult-to-electrify areas and those that will continue to need carbon. We discuss two approaches for this developing carbon alternatives and improving our ability to reuse carbon, enabled by separations. Furthermore, we posit that co-design and use-driven fundamental science are essential to reach aggressive greenhouse gas reduction targets.

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2024 Tipo de documento: Article

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2024 Tipo de documento: Article