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Self-oscillating polymeric refrigerator with high energy efficiency.
Han, Donglin; Zhang, Yingjing; Huang, Cenling; Zheng, Shanyu; Wu, Dongyuan; Li, Qiang; Du, Feihong; Duan, Hongxiao; Chen, Weilin; Shi, Junye; Chen, Jiangping; Liu, Gang; Chen, Xin; Qian, Xiaoshi.
Afiliação
  • Han D; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Zhang Y; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Huang C; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Zheng S; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Wu D; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Li Q; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Du F; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Duan H; School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Chen W; School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Shi J; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Chen J; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Liu G; School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Chen X; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China.
  • Qian X; State Key Laboratory of Mechanical System and Vibration, Interdisciplinary Research Center, Institute of Refrigeration and Cryogenics, and MOE Key Laboratory for Power Machinery and Engineering, School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai, China. xsqian@sjtu.edu.cn.
Nature ; 629(8014): 1041-1046, 2024 May.
Article em En | MEDLINE | ID: mdl-38720078
ABSTRACT
Electrocaloric1,2 and electrostrictive3,4 effects concurrently exist in dielectric materials. Combining these two effects could achieve the lightweight, compact localized thermal management that is promised by electrocaloric refrigeration5. Despite a handful of numerical models and schematic presentations6,7, current electrocaloric refrigerators still rely on external accessories to drive the working bodies8-10 and hence result in a low device-level cooling power density and coefficient of performance (COP). Here we report an electrocaloric thin-film device that uses the electro-thermomechanical synergy provided by polymeric ferroelectrics. Under one-time a.c. electric stimulation, the device is thermally and mechanically cycled by the working body itself, resulting in an external-driver-free, self-cycling, soft refrigerator. The prototype offers a directly measured cooling power density of 6.5 W g-1 and a peak COP exceeding 58 under a zero temperature span. Being merely a 30-µm-thick polymer film, the device achieved a COP close to 24 under a 4 K temperature span in an open ambient environment (32% thermodynamic efficiency). Compared with passive cooling, the thin-film refrigerator could immediately induce an additional 17.5 K temperature drop against an electronic chip. The soft, polymeric refrigerator can sense, actuate and pump heat to provide automatic localized thermal management.
Assuntos

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Assunto principal: Polímeros / Refrigeração / Termodinâmica Idioma: En Ano de publicação: 2024 Tipo de documento: Article

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Assunto principal: Polímeros / Refrigeração / Termodinâmica Idioma: En Ano de publicação: 2024 Tipo de documento: Article