Your browser doesn't support javascript.
loading
Breaking the intrinsic activity barriers of bilayer metal oxides for catalytic CO2 reduction.
Xu, Hangmin; Song, Hao; Bi, Chuanzhou; Zhou, Ganghua; Liu, Xiang; Zhong, Kang; Jiang, Weiyi; Yang, Jinman; Shen, Wenlong; Hao, Naiying; Zhu, Xianglin; Xu, Hui; Wang, Xiaozhi; Zhu, Xingwang.
Afiliação
  • Xu H; College of Environmental Science and Engineering, Institute of Technology for Carbon Neutralization, Yangzhou University, Yangzhou 225009, PR China.
  • Song H; College of Environmental Science and Engineering, Institute of Technology for Carbon Neutralization, Yangzhou University, Yangzhou 225009, PR China.
  • Bi C; College of Environmental Science and Engineering, Institute of Technology for Carbon Neutralization, Yangzhou University, Yangzhou 225009, PR China.
  • Zhou G; College of Environmental Science and Engineering, Institute of Technology for Carbon Neutralization, Yangzhou University, Yangzhou 225009, PR China.
  • Liu X; College of Environmental Science and Engineering, Institute of Technology for Carbon Neutralization, Yangzhou University, Yangzhou 225009, PR China.
  • Zhong K; School of the Environment and Safety Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China.
  • Jiang W; College of Environmental Science and Engineering, Institute of Technology for Carbon Neutralization, Yangzhou University, Yangzhou 225009, PR China.
  • Yang J; School of the Environment and Safety Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China.
  • Shen W; Jiangsu Vocational College of Electronics and Information, Huaian, Jiangsu 223003, PR China.
  • Hao N; Department of Materials Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, PR China.
  • Zhu X; School of the Environment and Safety Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China. Electronic address: zhuxianglin0374@163.com.
  • Xu H; School of the Environment and Safety Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China.
  • Wang X; College of Environmental Science and Engineering, Institute of Technology for Carbon Neutralization, Yangzhou University, Yangzhou 225009, PR China. Electronic address: xzwang@yzu.edu.cn.
  • Zhu X; College of Environmental Science and Engineering, Institute of Technology for Carbon Neutralization, Yangzhou University, Yangzhou 225009, PR China. Electronic address: zxw@yzu.edu.cn.
J Colloid Interface Sci ; 675: 419-428, 2024 Jun 27.
Article em En | MEDLINE | ID: mdl-38981251
ABSTRACT
The photocatalytic CO2 reduction reaction is severely limited by sluggish charge kinetics. To address this issue, a strategy utilizing non-metal-doped layered double hydroxide (LDH) has been developed to control the electronic structure of spindle-shaped nanoflowers, resulting in efficient photocatalytic CO2 reduction. The results demonstrate that the designed catalyst yields 263.16 µmol g-1 h-1 for the photoreduction of CO2 to CO. Furthermore, the in situ Fourier transform infrared spectrum (FT-IR) analysis demonstrate that the specific S-ligand (S-bridge) facilitates CO2 activation, ensuring the continuous production of *COOH. The hydrothermal-assisted ionic liquid method proposed in this study offers guidance for modifying catalysts.
Palavras-chave

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2024 Tipo de documento: Article

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2024 Tipo de documento: Article