Evidence of 3D Topological-Domain Dynamics in KTN:Li Polarization-Supercrystal Formation.

We experimentally and theoretically investigate thermal domain evolution in near-transition KTN:Li. Results allow us to establish how polarization supercrystals form, a hidden 3D topological phase composed of hypervortex defects. These are the result of six converging polarization vortices, each associated to one orientation of the 3D broken inversion symmetry. We also identify rescaling soliton lattices and domain patterns that replicate on different scales. Findings shed light on volume domain self-organization into closed-flux patterns and open up new scenarios for topologically protected noise-resistant ferroelectric memory bits.

Intense Wave Formation from Multiple Soliton Fusion and the Role of Extra Dimensions.

We experimentally and numerically explore the role of dimensionality in multiple (three or more) soliton fusion supported by nonreciprocal energy exchange. Three-soliton fusion into an intense wave is found when an extra dimension, with no broken inversion symmetry, is involved. The phenomenon is observed for 2+1D spatial waves in photorefractive crystals, where solitons are supported by a spatially local saturated Kerr-like self-focusing and fusion is driven by the leading nonlocal correction, the spatial analog of the nonlinear Raman effect.

Electro-optic active Q-switched Tm:YLF laser based on polarization modulation.

An electro-optic active Q-switched Tm:YLF laser (1880 nm) employing a novel, to the best of our knowledge, switching scheme is presented. The switching is done by a potassium lithium tantalate niobate (KLTN) crystal operated slightly above the ferroelectric phase transition, cut in a trapezoidal shape for reducing acousto-optic oscillations. The novel switching scheme exploits the emission cross section difference between the π and σ polarizations in the Tm:YLF and overcomes the residual oscillation effects even at high repetition rates. The laser exhibited stable operation yielding pulses of 0.81 mJ and pulse duration of 30 ns at 5 kHz, and pulses of 1.25 mJ and pulse duration of 19 ns at 500 Hz.

Direct Observation of Fractal-Dimensional Percolation in the 3D Cluster Dynamics of a Ferroelectric Supercrystal.

We perform percolation analysis of crossed-polarizer transmission images in a biased nanodisordered bulk KTN:Li perovskite. Two distinct percolative transitions are identified at two electric field thresholds. The low-field transition involves a directional fractal chain of dimension D=1.65, while the high-field transition has a dimension D>2. Direct cluster imaging in the volume is achieved using high-resolution orthographic 3D projections based on giant refraction. Percolation is attributed to a full-3D domain reorientation that mediates the transition from a ferroelectric supercrystal state to a disordered domain mosaic.

Evidence of Chaotic Dynamics in Three-Soliton Collisions.

We observe chaotic optical wave dynamics characterized by erratic energy transfer and soliton annihilation and creation in the aftermath of a three-soliton collision in a photorefractive crystal. Irregular dynamics are found to be mediated by the nonlinear Raman effect, a coherent interaction that leads to nonreciprocal soliton energy exchange. Results extend the analogy between solitons and particles to the emergence of chaos in three-body physics and provide new insight into the origin of the irregular dynamics that accompany extreme and rogue waves.

Soliton Maxwell demons and long-tailed statistics in fluctuating optical fields.

We demonstrate experimentally in biased photorefractive crystals that collisions between random-amplitude optical spatial solitons produce long-tailed statistics from input Gaussian fluctuations. The effect is mediated by Raman nonlocal corrections to Kerr self-focusing that turn soliton-soliton interaction into a Maxwell demon for the output wave amplitude.

Fast electroholographic wavelength selective switching implemented in a slab waveguide.

We present wavelength selective switching with a rise time of 25 ns implemented in a slab waveguide constructed in a KLTN:Cu crystal. The waveguide was fabricated by implantations of alpha particles at 2.1 MeV which produced a 0.5 µm thick cladding layer with reduced refractive index at 4.5 µm underneath the crystal surface. This demonstrates the feasibility of implementing electroholography in waveguides maintaining the performance obtained in bulk crystals, providing in potential the basis for constructing integrated photonic circuits which incorporate interconnected electroholographic wavelength selective switches and electrical wavelength tuning devices for employing wavelength addressing routing schemes in computer networks, in particular for relieving the bandwidth bottlenecks in data center networks.

Electro-optical modulation with immunity to optical damage by bipolar operation in potassium lithium tantalate niobate.

A method for suppressing the formation of optical damage in quadratic electrooptic devices operated at short wavelengths is presented. Formation of optical damage is attributed to the generation of a trapped space charge induced by photoionization of impurity ions by the propagating beam. It is shown that in potassium lithium tantalate niobate where the electrooptic effect is quadratic, operating the electrooptic device by a bipolar driving voltage prevents the space charge from accumulating, which inhibits the formation of the optical damage. A 6 hours continuous operation of electrooptic modulator for a 30 W/cm(2) at λ = 445 nm input beam is demonstrated.

A sub wavelength localization scheme in optical imaging using conical diffraction.

In this paper we present a scheme for the acquisition of high temporal resolution images of single particles with enhanced lateral localization accuracy. The scheme, which is implementable as a part of the illumination system of a standard confocal microscope, is based on the generation of a vector beam that is manipulated by polarimetry techniques to create a set of illumination PSFs with different spatial profiles. The combination of data collected in different illumination states enables the extraction of spatial information obscured by diffraction in the standard imaging system. An implementation of the scheme based on the utilization of the unique phenomenon of conical diffraction is presented, and the basic strategy it provides for enhanced localization in the diffraction limited region is demonstrated.

Full C-band tunable laser based on electroholography.

A tunable laser that spans the entire C band is presented. The laser consists of an Er-doped fiber amplifier gain medium, a fiber ring resonator, and an electroholography-based tuning mechanism. The electrohologram used is in the g44 configuration where the Bragg condition can be electrically tuned for a specific wavelength. Two laser architectures are presented, one in which the diffracting beam and one in which the direct beam of the electrohologram is used as the laser output. Switching time between wavelengths is limited by the gain medium relaxation time, since the electrohologram switching time is less than 1 ns.

Anomalous Optical Properties of KTN:Li Ferroelectric Supercrystals.

We report a spectroscopic investigation of potassium-lithium-tantalate-niobate (KTN:Li) across its room-temperature ferroelectric phase transition, when the sample manifests a supercrystal phase. Reflection and transmission results indicate an unexpected temperature-dependent enhancement of average index of refraction from 450 nm to 1100 nm, with no appreciable accompanying increase in absorption. Second-harmonic generation and phase-contrast imaging indicate that the enhancement is correlated to ferroelectric domains and highly localized at the supercrystal lattice sites. Implementing a two-component effective medium model, the response of each lattice site is found to be compatible with giant broadband refraction.

Programming scale-free optics in disordered ferroelectrics.

Using the history dependence of a dipolar glass hosted in a compositionally disordered lithium-enriched potassium tantalate niobate (KTN:Li) crystal, we demonstrate scale-free optical propagation at tunable temperatures. The operating equilibration temperature is determined by previous crystal spiralling in the temperature/cooling-rate phase space.

The remote sensing of mental stress from the electromagnetic reflection coefficient of human skin in the sub-THz range.

Recent work has demonstrated that the reflection coefficient of human skin in the frequency range from 95 to 110 GHz (W band) mirrors the temporal relaxation of stress induced by physical exercise. In this work, we extend these findings to show that in the event of a subtle trigger to stress, such as mental activity, a similar picture of response emerges. Furthermore, the findings are extended to cover not only the W band (75-110 GHz), but also the frequency band from 110 to 170 GHz (D band). We demonstrate that mental stress, induced by the Stroop effect and recorded by the galvanic skin response (GSR), can be correlated to the reflection coefficient in the aforementioned frequency bands. Intriguingly, a light physical stress caused by repeated hand gripping clearly showed an elevated stress level in the GSR signal, but was largely unnoted in the reflection coefficient in the D band. The implication of this observation requires further validation.

Enhancing DNT Detection by a Bacterial Bioreporter: Directed Evolution of the Transcriptional Activator YhaJ.

Detection of buried landmines is a dangerous and complicated task that consumes large financial resources and poses significant risks to the personnel involved. A potential alternative to conventional detection methodologies is the use of microbial bioreporters, capable of emitting an optical signal upon exposure to explosives, thus revealing to a remote detector the location of buried explosive devices. We have previously reported the design, construction, and optimization of an Escherichia coli-based bioreporter for the detection of 2,4,6-trinitrotoluene (TNT) and its accompanying impurity 2,4-dinitrotoluene (DNT). Here we describe the further enhancement of this bioreporter by the directed evolution of YhaJ, the transcriptional activator of the yqjF gene promoter, the sensing element of the bioreporter's molecular circuit. This process resulted in a 37-fold reduction of the detection threshold, as well as significant enhancements to signal intensity and response time, rendering this sensor strain more suitable for detecting the minute concentrations of DNT in the soil above buried landmines. The capability of this enhanced bioreporter to detect DNT buried in sand is demonstrated.

Detection of buried explosives with immobilized bacterial bioreporters.

The unchecked dispersal of antipersonnel landmines since the late 19th century has resulted in large areas contaminated with these explosive devices, creating a substantial worldwide humanitarian safety risk. The main obstacle to safe and effective landmine removal is the identification of their exact location, an activity that currently requires entry of personnel into the minefields; to date, there is no commercialized technology for an efficient stand-off detection of buried landmines. In this article, we describe the optimization of a microbial sensor strain, genetically engineered for the remote detection of 2,4,6-trinitrotoloune (TNT)-based mines. This bioreporter, designed to bioluminescence in response to minute concentrations of either TNT or 2,4-dinitotoluene (DNT), was immobilized in hydrogel beads and optimized for dispersion over the minefield. Following modifications of the hydrogel matrix in which the sensor bacteria are encapsulated, as well as their genetic reporting elements, these sensor bacteria sensitively detected buried 2,4-dinitrotoluene in laboratory experiments. Encapsulated in 1.5 mm 2% alginate beads containing 1% polyacrylic acid, they also detected the location of a real metallic antipersonnel landmine under field conditions. To the best of our knowledge, this is the first report demonstrating the detection of a buried landmine with a luminescent microbial bioreporter.

Hyperbolic optics and superlensing in room-temperature KTN from self-induced k-space topological transitions.

A hyperbolic medium will transfer super-resolved optical waveforms with no distortion, support negative refraction, superlensing, and harbor nontrivial topological photonic phases. Evidence of hyperbolic effects is found in periodic and resonant systems for weakly diffracting beams, in metasurfaces, and even naturally in layered systems. At present, an actual hyperbolic propagation requires the use of metamaterials, a solution that is accompanied by constraints on wavelength, geometry, and considerable losses. We show how nonlinearity can transform a bulk KTN perovskite into a broadband 3D hyperbolic substance for visible light, manifesting negative refraction and superlensing at room-temperature. The phenomenon is a consequence of giant electro-optic response to the electric field generated by the thermal diffusion of photogenerated charges. Results open new scenarios in the exploration of enhanced light-matter interaction and in the design of broadband photonic devices.

An autonomous bioluminescent bacterial biosensor module for outdoor sensor networks, and its application for the detection of buried explosives.

We describe a miniaturized field-deployable biosensor module, designed to function as an element in a sensor network for standoff monitoring and mapping of environmental hazards. The module harbors live bacterial sensor cells, genetically engineered to emit a bioluminescent signal in the presence of preselected target materials, which act as its core sensing elements. The module, which detects and processes the biological signal, composes a digital record that describes its findings, and can be transmitted to a remote receiver. The module is an autonomous self-contained unit that can function either as a standalone sensor, or as a node in a sensor network. The biosensor module can potentially be used for detecting any target material to which the sensor cells were engineered to respond. The module described herein was constructed to detect the presence of buried landmines underneath its footprint. The demonstrated detection sensitivity was 0.25 mg 2,4-dinitrotoluene per Kg soil.

Genome-wide gene-deletion screening identifies mutations that significantly enhance explosives vapor detection by a microbial sensor.

Genetically engineered microbial biosensors, capable of detecting traces of explosives residues above buried military ordnance and emitting an optical signal in response, may potentially serve for the standoff detection of buried landmines. A promising candidate for such an application is a previously reported Escherichia coli-based reporter strain that employs the yqjF gene promoter as its sensing element; however, for this sensor to be able to detect actual landmines reliably, it was necessary for its detection sensitivity and signal intensity to be enhanced. In this study, a high-throughput approach was employed to screen the effects of individual gene deletions on yqjF activation by 2,4-dinitrotoluene (DNT). Several genes were identified, the deletion of which elicited a significant enhancement of yqjF induction by DNT. The most promising of these mutations were introduced into the sensor strain, individually or in pairs, yielding a considerable increase in signal intensity and a lowering of the detection threshold. A strain harboring two of the identified mutations, ygdD and eutE, appears to be the most sensitive microbial biosensor currently described for the detection of traces of landmine explosives.

A tunable channel waveguide array fabricated by the implantations of He+ ions in an electrooptical KLTN substrate.

An electrooptical channel waveguide array was constructed in potassium lithium tantalate niobate substrate by the implantation of He(+) ions at high energies. The array was fabricated by two successive implantation sessions at 1.6 MeV and 1.2 MeV through a comb-like stopping mask that limited the implanted ions to penetrate the substrate in 1 microm wide stripes periodically distributed at 3.5 microm intervals. This generated a grating of amorphized stripes with reduced refractive index. This was followed by a uniform implantation of He(+) ions at 1.8 MeV which created a bottom cladding layer below the array. Wave propagation in the array was studied by focusing a light beam at 636 nm into the central channel, and observing the wavefront it created at the output plane of the array. It was found that applying an electric field across the array strongly affects the coupling between adjacent channels and governs the width of the wavefront at the output plane.

The electromagnetic response of human skin in the millimetre and submillimetre wave range.

Recent studies of the minute morphology of the skin by optical coherence tomography revealed that the sweat ducts in human skin are helically shaped tubes, filled with a conductive aqueous solution. This, together with the fact that the dielectric permittivity of the dermis is higher than that of the epidermis, brings forward the supposition that as electromagnetic entities, the sweat ducts could be regarded as low Q helical antennas. The implications of this statement were further investigated by electromagnetic simulation and experiment of the in vivo reflectivity of the skin of subjects under varying physiological conditions (Feldman et al 2008 Phys. Rev. Lett. 100 128102). The simulation and experimental results are in a good agreement and both demonstrate that sweat ducts in the skin could indeed behave as low Q antennas. Thus, the skin spectral response in the sub-Terahertz region is governed by the level of activity of the perspiration system and shows the minimum of reflectivity at some frequencies in the frequency band of 75-110 GHz. It is also correlated to physiological stress as manifested by the pulse rate and the systolic blood pressure. As such, it has the potential to become the underlying principle for remote sensing of the physiological parameters and the mental state of the examined subject.