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1.
Phys Rev Lett ; 131(15): 156705, 2023 Oct 13.
Artículo en Inglés | MEDLINE | ID: mdl-37897789

RESUMEN

Nonlinear interactions are crucial in science and engineering. Here, we investigate wave interactions in a highly nonlinear magnetic system driven by parametric pumping leading to Bose-Einstein condensation of spin-wave quanta-magnons. Using Brillouin light scattering spectroscopy in yttrium-iron garnet films, we found and identified a set of nonlinear processes resulting in off-resonant spin-wave excitations-virtual magnons. In particular, we discovered a dynamically strong, correlation-enhanced four-wave interaction process of the magnon condensate with pairs of parametric magnons having opposite wave vectors and fully correlated phases.

2.
Phys Rev Lett ; 121(7): 077203, 2018 Aug 17.
Artículo en Inglés | MEDLINE | ID: mdl-30169064

RESUMEN

Evolution of an overpopulated gas of magnons to a Bose-Einstein condensate and excitation of a magnon supercurrent, propelled by a phase gradient in the condensate wave function, can be observed at room temperature by means of the Brillouin light scattering spectroscopy in an yttrium iron garnet material. We study these phenomena in a wide range of external magnetic fields in order to understand their properties when externally pumped magnons are transferred towards the condensed state via two distinct channels: a multistage Kolmogorov-Zakharov cascade of the weak-wave turbulence or a one-step kinetic instability process. Our main result is that opening the kinetic instability channel leads to the formation of a much denser magnon condensate and to a stronger magnon supercurrent compared to the cascade mechanism alone.

3.
Phys Rev Lett ; 118(23): 237201, 2017 Jun 09.
Artículo en Inglés | MEDLINE | ID: mdl-28644646

RESUMEN

An ensemble of magnons, quanta of spin waves, can be prepared as a Bose gas of weakly interacting quasiparticles. Furthermore, the thermalization of the overpopulated magnon gas through magnon-magnon scattering processes, which conserve the number of particles, can lead to the formation of a Bose-Einstein condensate at the bottom of a spin-wave spectrum. However, magnon-phonon scattering can significantly modify this scenario and new quasiparticles are formed-magnetoelastic bosons. Our observations of a parametrically populated magnon gas in a single-crystal film of yttrium iron garnet by means of wave-vector-resolved Brillouin light scattering spectroscopy evidence a novel condensation phenomenon: A spontaneous accumulation of hybrid magnetoelastic bosonic quasiparticles at the intersection of the lowest magnon mode and a transversal acoustic wave.

4.
Npj Spintron ; 2(1): 29, 2024.
Artículo en Inglés | MEDLINE | ID: mdl-38966324

RESUMEN

Quantum magnonics investigates the quantum-mechanical properties of magnons, such as quantum coherence or entanglement for solid-state quantum information technologies at the nanoscale. The most promising material for quantum magnonics is the ferrimagnetic yttrium iron garnet (YIG), which hosts magnons with the longest lifetimes. YIG films of the highest quality are grown on a paramagnetic gadolinium gallium garnet (GGG) substrate. The literature has reported that ferromagnetic resonance (FMR) frequencies of YIG/GGG decrease at temperatures below 50 K despite the increase in YIG magnetization. We investigated a 97 nm-thick YIG film grown on 500 µm-thick GGG substrate through a series of experiments conducted at temperatures as low as 30 mK, and using both analytical and numerical methods. Our findings suggest that the primary factor contributing to the FMR frequency shift is the stray magnetic field created by the partially magnetized GGG substrate. This stray field is antiparallel to the applied external field and is highly inhomogeneous, reaching up to 40 mT in the center of the sample. At temperatures below 500 mK, the GGG field exhibits a saturation that cannot be described by the standard Brillouin function for a paramagnet. Including the calculated GGG field in the analysis of the FMR frequency versus temperature dependence allowed the determination of the cubic and uniaxial anisotropies. We find that the total crystallographic anisotropy increases more than three times with the decrease in temperature down to 2 K. Our findings enable accurate predictions of the YIG/GGG magnetic systems behavior at low and ultralow millikelvin temperatures, crucial for developing quantum magnonic devices.

5.
J Imaging ; 7(5)2021 Apr 29.
Artículo en Inglés | MEDLINE | ID: mdl-34460678

RESUMEN

Magnetic particles have been evaluated for their biomedical applications as a drug delivery system to treat asthma and other lung diseases. In this study, ferromagnetic barium hexaferrite (BaFe12O19) and iron oxide (Fe3O4) particles were suspended in water or glycerol, as glycerol can be 1000 times more viscous than water. The particle concentration was 2.50 mg/mL for BaFe12O19 particle clusters and 1.00 mg/mL for Fe3O4 particle clusters. The magnetic particle cluster cross-sectional area ranged from 15 to 1000 µµm2, and the particle cluster diameter ranged from 5 to 45 µµm. The magnetic particle clusters were exposed to oscillating or rotating magnetic fields and imaged with an optical microscope. The oscillation frequency of the applied magnetic fields, which was created by homemade wire spools inserted into an optical microscope, ranged from 10 to 180 Hz. The magnetic field magnitudes varied from 0.25 to 9 mT. The minimum magnetic field required for particle cluster rotation or oscillation in glycerol was experimentally measured at different frequencies. The results are in qualitative agreement with a simplified model for single-domain magnetic particles, with an average deviation from the model of 1.7 ± 1.3. The observed difference may be accounted for by the fact that our simplified model does not include effects on particle cluster motion caused by randomly oriented domains in multi-domain magnetic particle clusters, irregular particle cluster size, or magnetic anisotropy, among other effects.

6.
Nat Nanotechnol ; 15(6): 457-461, 2020 Jun.
Artículo en Inglés | MEDLINE | ID: mdl-32313217

RESUMEN

The fundamental phenomenon of Bose-Einstein condensation has been observed in different systems of real particles and quasiparticles. The condensation of real particles is achieved through a major reduction in temperature, while for quasiparticles, a mechanism of external injection of bosons by irradiation is required. Here, we present a new and universal approach to enable Bose-Einstein condensation of quasiparticles and to corroborate it experimentally by using magnons as the Bose-particle model system. The critical point to this approach is the introduction of a disequilibrium of magnons with the phonon bath. After heating to an elevated temperature, a sudden decrease in the temperature of the phonons, which is approximately instant on the time scales of the magnon system, results in a large excess of incoherent magnons. The consequent spectral redistribution of these magnons triggers the Bose-Einstein condensation.

7.
Nat Commun ; 10(1): 2460, 2019 06 05.
Artículo en Inglés | MEDLINE | ID: mdl-31165731

RESUMEN

A macroscopic collective motion of a Bose-Einstein condensate (BEC) is commonly associated with phenomena such as superconductivity and superfluidity, often generalised by the term supercurrent. Another type of motion of a quantum condensate is second sound-a wave of condensate's parameters. Recently, we reported on the decay of a BEC of magnons caused by a supercurrent outflow of the BEC from the locally heated area of a room temperature magnetic film. Here, we present the observation of a macroscopic BEC transport mechanism related to the excitation of second sound. The condensed magnons, being propelled out of the heated area, form compact humps of BEC density, which propagate many hundreds of micrometers in the form of distinct second sound-Bogoliubov waves. This discovery advances the physics of quasiparticles and allows for the application of related transport phenomena for low-loss data transfer in magnon spintronics devices.

8.
Nat Commun ; 5: 3452, 2014 Mar 11.
Artículo en Inglés | MEDLINE | ID: mdl-24613901

RESUMEN

Bose-Einstein condensation of quasi-particles such as excitons, polaritons, magnons and photons is a fascinating quantum mechanical phenomenon. Unlike the Bose-Einstein condensation of real particles (like atoms), these processes do not require low temperatures, since the high densities of low-energy quasi-particles needed for the condensate to form can be produced via external pumping. Here we demonstrate that such a pumping can create remarkably high effective temperatures in a narrow spectral region of the lowest energy states in a magnon gas, resulting in strikingly unexpected transitional dynamics of Bose-Einstein magnon condensate: the density of the condensate increases immediately after the external magnon flow is switched off and initially decreases if it is switched on again. This behaviour finds explanation in a nonlinear 'evaporative supercooling' mechanism that couples the low-energy magnons overheated by pumping with all the other thermal magnons, removing the excess heat, and allowing Bose-Einstein condensate formation.


Asunto(s)
Fenómenos Químicos , Gases/química , Calor , Transición de Fase , Algoritmos , Cinética , Modelos Teóricos , Fotones , Termodinámica
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