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We present a general framework for inverse design of nanopatterned surfaces that maximize spatially averaged surface-enhanced Raman (SERS) spectra from molecules distributed randomly throughout a material or fluid, building upon a recently proposed trace formulation for optimizing incoherent emission. This leads to radically different designs than optimizing SERS emission at a single known location, as we illustrate using several 2D design problems addressing effects of hot-spot density, angular selectivity, and nonlinear damage. We obtain optimized structures that perform about 4 × better than coating with optimized spheres or bowtie structures and about 20 × better when the nonlinear damage effects are included.
RESUMEN
The rates of optical processes, such as two-photon absorption and spontaneous photon emission, are strongly dependent on the environment in which they take place, easily varying by orders of magnitude between different settings. Using topology optimization, we design a set of compact wavelength-sized devices, to study the effect of optimizing geometries for enhancing processes that depend differently on the field in the device volume, characterized by different figures of merit. We find that significantly different field distributions lead to maximization of the different processes, and - by extension - that the optimal device geometry is highly dependent on the targeted process, with more than an order of magnitude performance difference between optimized devices. This demonstrates that a univeral measure of field confinement is meaningless when evaluting device performance, and stresses the importance of directly targeting the appropriate metric when designing photonic components for optimal performance.
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We show that topology optimization (TO) of metallic resonators can lead to â¼102 × improvement in surface-enhanced Raman scattering (SERS) efficiency compared to traditional resonant structures such as bowtie antennas. TO inverse design leads to surprising structures very different from conventional designs, which simultaneously optimize focusing of the incident wave and emission from the Raman dipole. We consider isolated metallic particles as well as more complicated configurations such as periodic surfaces or resonators coupled to dielectric waveguides, and the benefits of TO are even greater in the latter case. Our results are motivated by recent rigorous upper bounds to Raman scattering enhancement, and shed light on the extent to which these bounds are achievable.
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We demonstrate new axisymmetric inverse-design techniques that can solve problems radically different from traditional lenses, including reconfigurable lenses (that shift a multi-frequency focal spot in response to refractive-index changes) and widely separated multi-wavelength lenses (λ = 1â µm and 10â µm). We also present experimental validation for an axisymmetric inverse-designed monochrome lens in the near-infrared fabricated via two-photon polymerization. Axisymmetry allows fullwave Maxwell solvers to be scaled up to structures hundreds or even thousands of wavelengths in diameter before requiring domain-decomposition approximations, while multilayer topology optimization with â¼105 degrees of freedom can tackle challenging design problems even when restricted to axisymmetric structures.
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An acoustic topological insulator (TI) is synthesized using topology optimization, a free material inverse design method. The TI appears spontaneously from the optimization process without imposing explicit requirements on the existence of pseudospin-1/2 states at the TI interface edge, or the Chern number of the topological phases. The resulting TI is passive, consisting of acoustically hard members placed in an air background and has an operational bandwidth of ≈12.5% showing high transmission. Further analysis demonstrates confinement of more than 99% of the total field intensity in the TI within at most six lattice constants from the TI interface. The proposed design hereby outperforms a reference from recent literature regarding energy transmission, field confinement, and operational bandwidth.
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This paper describes a systematic design study of periodic gold-nanostrip arrays placed on a thin film aimed at enhancing the electric field inside the film when irradiated by light. Based on the study, a "selection rule" is proposed, which provides optimization-based design methods with an a priori choice between field-enhancement dominated by coupling to guided modes, by plasmonic near-field enhancement or by a mix hereof. An appropriate choice of wavelength and grating period is shown to selectively suppress or include waveguiding effects for the optimized designs. The validity of the selection rule is demonstrated through a numerical topology optimization study in which gold nanostrips are optimized for electric-field enhancement in an erbium-doped TiO2 thin film, targeting increased spectral upconversion in the erbium ions. The obtained designs exhibit waveguide excitation within the predicted intervals and, for light polarized perpendicularly to the strips, plasmonic response outside.
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The paper presents a topology optimization based method for designing acoustic focusing devices, capable of tailoring the sound emission pattern of one or several sources, across a chosen frequency band. The method is demonstrated numerically considering devices optimized for directional sound emission in two dimensions and is experimentally validated using three dimensional prints of the optimized designs. The emitted fields exhibit a level difference of at least 15 dB on axis relative to the off-axis directions, over frequency bands of approximately an octave. It is demonstrated to be possible to design focusing devices of dimensions comparable to the acoustic wavelength, a frequency range which is typically problematic, as well as devices operating at higher frequencies. The classical parabolic reflector is used as a benchmark. The devices designed using the proposed method are shown to outperform the latter in terms of directivity and maximum side-lobe level over nearly an octave band. A set of frequencies are considered simultaneously in the design formulation and performance robustness toward uniform spatial production errors in the designed devices is assured by including perturbations of the geometry in the design formulation.
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This paper presents the experimental validation of an acoustic cavity designed using topology optimization with the goal of minimizing the sound pressure locally for monochromatic excitation. The presented results show good agreement between simulations and measurements. The effect of damping, errors in the production of the cavity, and variations in operating frequency is discussed and the importance of taking these factors into account in the modeling process is highlighted.
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Compact visible wavelength achromats are essential for miniaturized and lightweight optics. However, fabrication of such achromats has proved to be exceptionally challenging. Here, using subsurface 3D printing inside mesoporous hosts we densely integrate aligned refractive and diffractive elements, forming thin high performance hybrid achromatic imaging micro-optics. Focusing efficiencies of 51-70% are achieved for 15µm thick, 90µm diameter, 0.3 numerical aperture microlenses. Chromatic focal length errors of less than 3% allow these microlenses to form high-quality images under broadband illumination (400-700 nm). Numerical apertures upwards of 0.47 are also achieved at the cost of some focusing efficiency, demonstrating the flexibility of this approach. Furthermore, larger area images are reconstructed from an array of hybrid achromatic microlenses, laying the groundwork for achromatic light-field imagers and displays. The presented approach precisely combines optical components within 3D space to achieve thin lens systems with high focusing efficiencies, high numerical apertures, and low chromatic focusing errors, providing a pathway towards achromatic micro-optical systems.