RESUMEN
Resonance fluorescence of two-level quantum systems has emerged as a powerful tool in quantum information processing. Extension of this approach to higher-level systems provides new opportunities for quantum optics applications. Here we introduce an all-optical tuning functionality into a well-established resonance fluorescence coherent driving scheme. We accomplish this by resonant excitation of a three-level ladder system with two laser fields utilizing Autler-Townes and ac Stark effects. We propose theoretically and demonstrate experimentally the feasibility of this approach toward all-optical spectral tuning of quantum-dot-based single-photon sources and investigate photon indistinguishability and purity levels. Our tuning technique allows for fast optical control of the quantum emitter spectrum which paves the way toward temporal and spectral shaping of the single photons, formation of topological Floquet states, or generation of high-dimensional frequency-encoded quantum states of light.
RESUMEN
We present an open-system master equation study of the coherent and incoherent resonance fluorescence spectrum from a two-level quantum system under coherent pulsed excitation. Several pronounced features that differ from the fluorescence under a constant drive are highlighted, including a multi-peak structure and a pronounced off-resonant spectral asymmetry, in stark contrast to the conventional symmetrical Mollow triplet. We also study semiconductor quantum dot systems using a polaron master equation and show how the key features of dynamic resonance fluorescence change with electron-acoustic-phonon coupling.