Electrotunable 180° achromatic linear polarization rotator based on a dual-frequency liquid crystal.

Linear polarization rotators have been widely used in optical systems. Commonly used polarization rotators are still beset by strong dispersion and thus restricted spectral bandwidth of operation. This leads to the development of achromatic or broadband alternatives, but most of them incorporate multiple waveplates for retardation compensation, which comes at the cost of increased complexity and reduced flexibility in operation and system design. Here, we demonstrate a single-element achromatic polarization rotator based on a thin film of dual-frequency chiral liquid crystal. The angle of polarization rotation is electrically tunable from 0° to 180° with low dispersion (±3°) in the entire visible spectrum, and a high degree of linear polarization (>95%) at the output.

Reconfiguration of three-dimensional liquid-crystalline photonic crystals by electrostriction.

Natural self-assembled three-dimensional photonic crystals such as blue-phase liquid crystals typically assume cubic lattice structures. Nonetheless, blue-phase liquid crystals with distinct crystal symmetries and thus band structures will be advantageous for optical applications. Here we use repetitive electrical pulses to reconfigure blue-phase liquid crystals into stable orthorhombic and tetragonal lattices. This approach, termed repetitively applied field, allows the system to relax between each pulse, gradually transforming the initial cubic lattice into various intermediate metastable states until a stable non-cubic crystal is achieved. We show that this technique is suitable for engineering non-cubic lattices with tailored photonic bandgaps, associated dispersion and band structure across the entire visible spectrum in blue-phase liquid crystals with distinct composition and initial crystal orientation. These field-free blue-phase liquid crystals exhibit large electro-optic responses and can be polymer-stabilized to have a wide operating temperature range and submillisecond response speed, which are promising properties for information display, electro-optics, nonlinear optics, microlasers and biosensing applications.

Optically rewritable dynamic phase grating based on blue-phase-templated azobenzene liquid crystal.

We propose an optically rewritable dynamic phase grating based on polymer-templated azo liquid crystal in a blue-phase structure. The grating consists of alternating blue-phase and light-induced isotropic-phase regions, patterned by ultraviolet illumination. In the field-off state, the grating is hidden (showing no diffraction), due to index matching between the two phases. An index change is induced in the blue-phase regions when an external voltage is applied, while the refractive index of the isotropic-phase regions remains the same. The resulting periodic index modulation causes the grating to diffract light. The diffraction efficiency is independent of incident polarization, and the electro-optic response is in the sub-millisecond scale. Enabled by the reversible photoisomerism of the azobenzene, we demonstrate optical-patterning, -erasure, and re-patterning of a single liquid-crystal cell into different grating geometries.

Optical control of the rotation of cholesteric liquid crystal gratings.

Two photoalignment-based methods to achieve orientational control of optical diffractions by cholesteric liquid crystal (CLC) fingerprint gratings are proposed and demonstrated. A trace of methyl red in the CLC host can effectively induce surface alignment upon linearly polarized green exposure and enable optically rewritable alignment. An effective rotation of the photo-aligned CLC grating is attained by changing the surface alignment axis. Using axially symmetric photoalignment, electrically tunable radial and concentric gratings are also realized. 1D grating diffraction is produced by operating off-axis and can be rotated by mechanically moving the axially symmetric grating. Such optical gratings have great potential for practical use in vibration detection, multi-directional optical modulations, and beam steering.

Selective variable optical attenuator for visible and mid-Infrared wavelengths.

This work demonstrates a variable optical attenuator (VOA) using dynamic scattering mode (DSM) in ion-doped liquid crystals with negative dielectric anisotropy. The mechanism of attenuation comes from optical scattering, which is generated by the electrically induced instability of undulation of LC textures. Electric fields are applied to switch the initial transparent state of the designed VOA to scattering states, varying the transmittance. The electric field also changes the size of the scattering domain from the LC texture and causes the designed device to exhibit an ultra-broadband selective operation in a visible to mid-IR spectral range. Furthermore, the VOA can selectively block one visible or mid-IR wavelength of light while letting other light pass. Such a VOA has many superior optical switching properties, such as high on/off contrast, insensitivity to polarization, and spectral selectivity; therefore, it has the potential to be used in practical optical systems.

All-optical control of polarization splitting with a dielectric-clad azobenzene liquid crystal.

We report the design, fabrication, and characterization of an optically switchable polarizing beam splitter with a prism/azobenzene liquid crystal/prism hybrid structure. The beam splitter can operate in the polarization-splitting mode and the non-splitting mode. The switching between the modes is realized by the photoisomerization-induced phase transitions in the azobenzene liquid crystal, featuring all-optical control, bistability, and fast response. Such an active polarization-handling element is highly desirable as it not only simplifies and compacts sophisticated optical systems but also increases the degree of freedom in optical circuit design.

Broadband mid-infrared polarization rotator based on optically addressable LCs.

This work proposes a mid-infrared polarization rotator that incorporates a twisted nematic liquid crystal (TNLC) cell with a photo-controllable alignment layer. The TNLC device with a sufficient phase retardation can act as an achromic polarization rotation device over a wide wavelengths range and thus can rotate the polarization of a mid-IR laser beam. The photo-alignment technique enables TNLCs with arbitrary twisting angles to be generated by the use of visible polarized addressing light to control the directors of the photo-alignment layer. Therefore, arbitrary rotation angles of the polarization axis of a linearly polarized mid-IR laser beam can be realized. Moreover, the rewritable property and reliability of this polarization rotator are experimentally verified. The flexibility of polarization control for broadband mid-IR opens up a large range of potential mid-IR applications.

Full-color reflectance-tunable filter based on liquid crystal cladded guided-mode resonant grating.

This work proposes a tunable reflective guided-mode resonant (GMR) filter that incorporates a 90° twisted nematic liquid crystal (TNLC). The GMR grating acts as an optical resonator that reflects strongly at the resonance wavelength and as an alignment layer for LC. The 90° TNLC functions as an achromic polarization rotator that alters the polarization of incident light. The resonance wavelength and reflectance of such a filter can be controlled by setting the angle of incidence and driving the 90° TNLC, respectively. The designed filter exhibits a very large spectral shift in resonance wavelength from 710 to 430 nm, which covers the entire visible spectrum. The transmittance can be tuned to within 10 V at various resonance wavelengths. The hybrid GMR - LC filter is compact, has a simple design, and is easy to fabricated. It can therefore be used in practical applications.

Highly sensitive optical temperature sensor based on a SiN micro-ring resonator with liquid crystal cladding.

This work develops a sensitivity-enhanced optical temperature sensor that is based on a silicon nitride (SiN) micro-ring resonator that incorporates nematic liquid crystal (NLC) cladding. As the ambient temperature changes, the refractive index of the NLCs, which have a large thermal-optical coefficient, dramatically varies. The change in the refractive index of the NLC cladding that is caused by the temperature shift can alter the effective refractive index of the micro-ring resonator and make the resonance wavelength very sensitive to the ambient temperature. The temperature-sensitivity of the device with 5CB cladding for TM-polarized light was measured to be as high as 1nm/°C between 25 and 33 °C and over 2nm/°C at temperatures close to clearing temperature of the 5CB cladding. The temperature-sensitivity of the proposed device is at least 55 times that of the micro-ring resonator with air cladding, whose temperature-dependent wavelength shift for TM-polarized light is 18pm/ °C.

Bistable light-driven π phase switching using a twisted nematic liquid crystal film.

A light-activated optical phase switch was developed, exploiting the conversion between left-handed and right-handed twisted nematic liquid crystals. Theoretical and experimental analyses revealed that the handedness inversion of the twisted nematic film altered the optical phase of the output waves by π. Herein, the competition between the helical twisting powers of the two reverse-handed chiral dopants determines the handedness of the twisted nematic film. The photo-responsibility and the bistability are attributed to the azobenzene chromophores in one of the chiral additives.

Electrically tunable high Q-factor micro-ring resonator based on blue phase liquid crystal cladding.

This work demonstrates an electrically tunable silicon nitride (SiN) micro-ring resonator with polymer-stabilized blue phase liquid crystals (PSBPLCs) cladding. An external vertical electric field is applied to modulate the refractive index of the PSBPLCs by exploiting its fast-response Kerr effect-induced birefringence. The consequent change in the refractive index of the cladding can vary the effective refractive index of the micro-ring resonator and shift the resonant wavelength. Crystalline structures of PSBPLCs with a scale of the order of hundreds of nanometers ensure that the resonator has a very low optical loss. The measured tuning range is 0.45 nm for TM polarized light under an applied voltage of 150V and the corresponding response time is in the sub-millisecond range with a Q-factor of greater than 20,000.

Multi-stable variable optical attenuator based on a liquid crystal gel-filled photonic crystal fiber.

This work demonstrates a multi-stable variable optical attenuator (VOA) that is fabricated by infiltrating a photonic crystal fiber (PCF) with a liquid crystal (LC) gel. Varying the cooling rate or biasing the electric field during gelation yields various degrees of scattering. Therefore, LC gel-filled PCFs with various transmittances can be realized. At a wavelength of 1550 nm, an attenuation rate of -33.4 dB/cm is obtained at a cooling rate of 30°C/min and a biasing voltage of 400 V during gelation. The proposed all-in-fiber VOA exhibits tunable attenuation and multiple stable states at room temperature.

Bistable cholesteric liquid crystal light shutter with multielectrode driving.

An electrically activated bistable light shutter that exploits polymer-stabilized cholesteric liquid crystal film was developed. Under double-sided three-terminal electrode driving, the device can be bistable and switched between focal conic and homeotropic textures with a uniform in-plane and vertical electrical field. The transparent state with a transmittance of 80% and the opaque/scattering state with a transmittance of 13% can be realized without any optical compensation film, and each can be simply switched to the other by applying a pulse voltage. Also, gray-scale selection can be performed by varying the applied voltage. The designed energy-saving bistable light shutter can be utilized to preserve privacy and control illumination and the flow of energy.

Directed crystalline symmetry transformation of blue-phase liquid crystals by reverse electrostriction.

Soft-matter-based photonic crystals like blue-phase liquid crystals (BPLC) have potential applications in wide-ranging photonic and bio-chemical systems. To date, however, there are limitations in the fabrication of large monocrystalline BPLCs. Traditional crystal-growth process involves the transition from a high-temperature disordered phase to an ordered (blue) phase and is generally slow (takes hours) with limited achievable lattice structures, and efforts to improve molecular alignment through post-crystallization field application typically prove ineffective. Here we report a systematic study on the molecular self-assembly dynamics of BPLC starting from a highly ordered phase in which all molecules are unidirectionally aligned by a strong electric field. We have discovered that, near the high-temperature end of the blue phase, if the applied field strength is then switched to an intermediate level or simply turned off, large-area monocrystalline BPLCs of various symmetries (tetragonal, orthorhombic, cubic) can be formed in minutes. Subsequent temperature tuning of the single crystal at a fixed applied field allows access to different lattice parameters and the formation of never-before-seen monoclinic structures. The formed crystals remain stable upon field removal. The diversity of stable monocrystalline BPLCs with widely tunable crystalline symmetries, band structures, and optical dispersions will significantly improve and expand their application potentials.

Optical bistability in a silicon nitride microring resonator with azo dye-doped liquid crystal as cladding material.

This investigation reports observations of optical bistability in a silicon nitride (SiN) micro-ring resonator with azo dye-doped liquid crystal cladding. The refractive index of the cladding can be changed by switching the liquid crystal between nematic (NLC) and photo-induced isotropic (PHI) states by. Both the NLC and the PHI states can be maintained for many hours, and can be rapidly switched from one state to the other by photo-induced isomerization using 532 nm and 408 nm addressing light, respectively. The proposed device exhibits optical bistable switching of the resonance wavelength without sustained use of a power source. It has a 1.9 nm maximum spectral shift with a Q-factor of over 10000. The hybrid SiN- LC micro-ring resonator possesses easy switching, long memory, and low power consumption. It therefore has the potential to be used in signal processing elements and switching elements in optically integrated circuits.

Polarization-independent bistable light valve in blue phase liquid crystal filled photonic crystal fiber.

This article demonstrates a bistable optical valve in a photonic liquid crystal fiber using the thermal hysteresis effect of the phase transition between the cholesteric phase and the blue phase (BP). The attenuation is due to various scattering losses in different phases. Both cholesteric and BPs can exist stably at room temperature (RT) and can also be switched to each other using temperature-control processes. The transmission spectrum and the intensity of the guided light can be controlled with various extents of scattering loss. For optical communications, this device can be manipulated over a loss difference of 10 dB at RT and insensitive to the polarization of light.

Wavelength tunable infrared light source based on semiconductor-integrated liquid crystal filter.

This work proposes an electrically tunable infrared light source based on a new compact structure, i.e., an AlGaInAs semiconductor multiple quantum well (MQW) integrated with a liquid crystal Fabry-Pérot filter. The AlGaInAs MQW is used as a luminance layer that emits broadband light. By sandwiching the AlGaInAs and LC material with two conducting mirrors, the active light source with an optical filter can be tuned with a wide wavelength range. The filter filled with nematic liquid crystal enables continuous tuning of emission along the extraordinary mode and provides a 58 nm tuning range with a bias of 14 V. The simulation results of wavelength and tunability are consistent with the experimental results. Cholesteric liquid crystal with a planar texture is also used to examine the properties of the tunable light source. Under an electric field, all the helical liquid crystal molecules tend to be aligned parallel to the field. The variation of the refractive index is normal to the substrate surface, and the polarization-independent tuning range is 41 nm. The wide tuning range and the polarization properties observed when NLC and CLC are respectively incorporated into the AlGaInAs based Fabry-Pérot cavity suggest that this integration scheme has potential for applying to optical communication system.

Random lasing in blue phase liquid crystals.

Random lasing actions have been observed in optically isotropic pure blue-phase and polymer-stabilized blue-phase liquid crystals containing laser dyes. Scattering, interferences and recurrent multiple scatterings arising from disordered platelet texture as well as index mismatch between polymer and mesogen in these materials provide the optical feedbacks for lasing action. In polymer stabilized blue-phase liquid crystals, coherent random lasing could occur in the ordered blue phase with an extended temperature interval as well as in the isotropic liquid state. The dependence of lasing wavelength range, mode characteristics, excitation threshold and other pertinent properties on temperature and detailed make-up of the crystals platelets were obtained. Specifically, lasing wavelengths and mode-stability were found to be determined by platelet size, which can be set by controlling the cooling rate; lasing thresholds and emission spectrum are highly dependent on, and therefore can be tuned by temperature.

Optically controllable bistable reflective liquid crystal display.

This Letter demonstrates a photo-addressable, bistable reflective liquid crystal display that is based on a dye-doped liquid crystal (DDLC). Bistable bright and dark states can be attained using the 45 deg twisted nematic (TN) and photo-induced isotropic states (PHI) of the DDLC, respectively. Both the 45 deg TN and PHI states can exist stably for tens of hours, and each can be rapidly switched to the other by the isomerization effect using UV and green light. A bistable reflective liquid crystal display is simply fabricated, easily operated, and rapidly switched. It therefore has the potential to be used in portable information systems.

Electrical control of shape of laser beam using axially symmetric liquid crystal cells.

This work demonstrates the electrical tuning of laser beam shape using an axially symmetric dye-dope liquid crystal (ASDDLC) device that is fabricated using a photo-alignment method. Various beam shapes can be obtained by linearly polarized Gaussian laser beams through an ASDDLC device under various applied voltages. The far-field intensity patterns generated by laser beams of selected shapes under various applied voltages are simulated, and the results are consistent with experiment. A rotatable petal-shaped beam is obtained by controlling the polarization of the output donut-shaped beam. The tenability of beam shape of light with a wavelength of 1064 nm, which is commonly used in biomedical applications, is also demonstrated.