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J Am Chem Soc ; 144(44): 20288-20297, 2022 11 09.
Artículo en Inglés | MEDLINE | ID: mdl-36301712

RESUMEN

Delivering cargo molecules across the plasma membrane is critical for biomedical research, and the need to develop molecularly well-defined tags that enable cargo transportation is ever-increasing. We report here a hydrophilic endocytosis-promoting peptide (EPP6) rich in hydroxyl groups with no positive charge. EPP6 can transport a wide array of small-molecule cargos into a diverse panel of animal cells. Mechanistic studies revealed that it entered the cells through a caveolin- and dynamin-dependent endocytosis pathway, mediated by the surface receptor fibrinogen C domain-containing protein 1. After endocytosis, EPP6 trafficked through early and late endosomes within 30 min. Over time, EPP6 partitioned among cytosol, lysosomes, and some long-lived compartments. It also demonstrated prominent transcytosis abilities in both in vitro and in vivo models. Our study proves that positive charge is not an indispensable feature for hydrophilic cell-penetrating peptides and provides a new category of molecularly well-defined delivery tags for biomedical applications.


Asunto(s)
Péptidos de Penetración Celular , Endocitosis , Animales , Endosomas/metabolismo , Péptidos de Penetración Celular/metabolismo , Lisosomas/metabolismo , Interacciones Hidrofóbicas e Hidrofílicas
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