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1.
Proc Natl Acad Sci U S A ; 118(8)2021 Feb 23.
Artículo en Inglés | MEDLINE | ID: mdl-33608457

RESUMEN

Nontrivial topology in condensed-matter systems enriches quantum states of matter to go beyond either the classification into metals and insulators in terms of conventional band theory or that of symmetry-broken phases by Landau's order parameter framework. So far, focus has been on weakly interacting systems, and little is known about the limit of strong electron correlations. Heavy fermion systems are a highly versatile platform to explore this regime. Here we report the discovery of a giant spontaneous Hall effect in the Kondo semimetal [Formula: see text] that is noncentrosymmetric but preserves time-reversal symmetry. We attribute this finding to Weyl nodes-singularities of the Berry curvature-that emerge in the immediate vicinity of the Fermi level due to the Kondo interaction. We stress that this phenomenon is distinct from the previously detected anomalous Hall effect in materials with broken time-reversal symmetry; instead, it manifests an extreme topological response that requires a beyond-perturbation-theory description of the previously proposed nonlinear Hall effect. The large magnitude of the effect in even tiny electric and zero magnetic fields as well as its robust bulk nature may aid the exploitation in topological quantum devices.

2.
Proc Natl Acad Sci U S A ; 116(36): 17701-17706, 2019 Sep 03.
Artículo en Inglés | MEDLINE | ID: mdl-31431528

RESUMEN

Complex and correlated quantum systems with promise for new functionality often involve entwined electronic degrees of freedom. In such materials, highly unusual properties emerge and could be the result of electron localization. Here, a cubic heavy fermion metal governed by spins and orbitals is chosen as a model system for this physics. Its properties are found to originate from surprisingly simple low-energy behavior, with 2 distinct localization transitions driven by a single degree of freedom at a time. This result is unexpected, but we are able to understand it by advancing the notion of sequential destruction of an SU(4) spin-orbital-coupled Kondo entanglement. Our results implicate electron localization as a unified framework for strongly correlated materials and suggest ways to exploit multiple degrees of freedom for quantum engineering.

3.
Crystals (Basel) ; 12(2): 251, 2022 Feb.
Artículo en Inglés | MEDLINE | ID: mdl-35910592

RESUMEN

Strange metal behavior refers to a linear temperature dependence of the electrical resistivity that is not due to electron-phonon scattering. It is seen in numerous strongly correlated electron systems, from the heavy fermion compounds, via transition metal oxides and iron pnictides, to magic angle twisted bi-layer graphene, frequently in connection with unconventional or "high temperature" superconductivity. To achieve a unified understanding of these phenomena across the different materials classes is a central open problem in condensed matter physics. Tests whether the linear-in-temperature law might be dictated by Planckian dissipation-scattering with the rate ∼ k B T / ℏ -are receiving considerable attention. Here we assess the situation for strange metal heavy fermion compounds. They allow to probe the regime of extreme correlation strength, with effective mass or Fermi velocity renormalizations in excess of three orders of magnitude. Adopting the same procedure as done in previous studies, i.e., assuming a simple Drude conductivity with the above scattering rate, we find that for these strongly renormalized quasiparticles, scattering is much weaker than Planckian, implying that the linear temperature dependence should be due to other effects. We discuss implications of this finding and point to directions for further work.

4.
Nat Commun ; 13(1): 5729, 2022 Sep 29.
Artículo en Inglés | MEDLINE | ID: mdl-36175415

RESUMEN

It is becoming increasingly clear that breakthrough in quantum applications necessitates materials innovation. In high demand are conductors with robust topological states that can be manipulated at will. This is what we demonstrate in the present work. We discover that the pronounced topological response of a strongly correlated "Weyl-Kondo" semimetal can be genuinely manipulated-and ultimately fully suppressed-by magnetic fields. We understand this behavior as a Zeeman-driven motion of Weyl nodes in momentum space, up to the point where the nodes meet and annihilate in a topological quantum phase transition. The topologically trivial but correlated background remains unaffected across this transition, as is shown by our investigations up to much larger fields. Our work lays the ground for systematic explorations of electronic topology, and boosts the prospect for topological quantum devices.

5.
Nat Commun ; 8: 14480, 2017 02 23.
Artículo en Inglés | MEDLINE | ID: mdl-28230099

RESUMEN

Superconductivity is a unique manifestation of quantum mechanics on a macroscopic scale, and one of the rare examples of many-body phenomena that can be explained by predictive, quantitative theories. The superconducting ground state is described as a condensate of Cooper pairs, and a major challenge has been to understand which mechanisms could lead to a bound state between two electrons, despite the large Coulomb repulsion. An even bigger challenge is to identify experimentally this pairing mechanism, notably in unconventional superconductors dominated by strong electronic correlations, like in high-Tc cuprates, iron pnictides or heavy-fermion compounds. Here we show that in the ferromagnetic superconductor UCoGe, the field dependence of the pairing strength influences dramatically its macroscopic properties like the superconducting upper critical field, in a way that can be quantitatively understood. This provides a simple demonstration of the dominant role of ferromagnetic spin fluctuations in the pairing mechanism.

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