Spectral splitting of the lasing emission of nitrogen ions pumped by 800-nm femtosecond laser pulses.

We report on a spectral splitting effect of the cavity-less lasing emission of nitrogen ions at 391.4 nm pumped by 800-nm femtosecond laser pulses. It was found that with the increase of the nitrogen gas pressure and pump pulse energy, both R and P branches experience spectral splitting. With an external injected seeding pulse, a similar split spectral line is observed for the amplified emission. In contrast, for the fluorescence radiation, no such spectral splitting phenomenon is observed with much more abundant R branch structures. Our theoretical model considers gas ionization by the pump pulse, the competition of excitation of all relevant electronic and vibrational states, and an amplification of the seeding pulse in the plasma with a population inversion. Our simulation reproduces this spectral splitting effect, which is attributed to the gain saturation resulting in the oscillation of the amplitude of the amplified signal.

Quantum and quasi-classical effects in the strong field ionization and subsequent excitation of nitrogen molecules.

The processes leading to the N2 + lasing are rather complex and even the population distribution after the pump laser excitation is unknown. In this paper, we study the population distribution at electronic and vibrational levels in N2 + driven by ultra-short laser pulse at the wavelengths of 800 nm and 400 nm by using the quantum-mechanical time-domain incoherent superposition model based on the time-dependent Schrödinger equation and the quasi-classical model assuming instantaneous ionization injection described by density matrix. It is shown that while both models provide qualitatively similar results, the quasi-classical instantaneous ionization injection model underestimates the population inversions corresponding to the optical transitions at 391 nm, 423 nm and 428 nm due to the assumption of quantum mixed states at the ionization time. A fast and accurate correction to this error is proposed. This work solidifies the theoretical models for population at vibrational states in N2 + and paves the way to uncover the mechanism of the N2 + lasing.

Time-resolved study of laser emission in nitrogen gas pumped by two near IR femtosecond laser pulses.

The time profile of a lasing signal at 391.4 nm emitted by a weakly ionized gas of nitrogen molecules at low pressure is measured under double excitation with intense femtosecond laser pulses at 800 nm. An abrupt decrease in emission occurs at the time of arrival of the second pulse. It is explained by a transfer of population from ground to first excited ionic level and by a disruption of coherence, terminating the conditions for lasing in a V-scheme without population inversion.

Quantum erasing of laser emission in N2.

Cavity-free lasing of N2+ induced by a femtosecond laser pulse at 800 nm is nearly totally suppressed by a delayed twin control pulse. We explain this surprising effect within the V-scheme of lasing without population inversion. A fast transfer of population between nitrogen ionic states X2Σg+ and A2Πu, induced by the second pulse, terminates the conditions for amplification in the system. The appearance of short lasing bursts at delays corresponding to revivals of rotational wave packets is explained along the same lines.

Mapping the Damping Dynamics of Mega-Ampere Electron Pulses Inside a Solid.

We report the lifetime of intense-laser (2×10^{19} W/cm^{2}) generated relativistic electron pulses in solids by measuring the time evolution of their Cherenkov emission. Using a picosecond resolution optical Kerr gating technique, we demonstrate that the electrons remain relativistic as long as 50 picoseconds-more than 1000 times longer than the incident light pulse. Numerical simulations of the propagation of relativistic electrons and the emitted Cherenkov radiation with Monte Carlo geant4 package reproduce the striking experimental findings.

Unexpected Sensitivity of Nitrogen Ions Superradiant Emission on Pump Laser Wavelength and Duration.

Nitrogen molecules in ambient air exposed to an intense near-infrared femtosecond laser pulse give rise to cavity-free superradiant emission at 391.4 and 427.8 nm. An unexpected pulse duration-dependent cyclic variation of the superradiance intensity is observed when the central wavelength of the femtosecond pump laser pulse is finely tuned between 780 and 820 nm, and no signal occurs at the resonant wavelength of 782.8 nm (2ω_{782.8 nm}=ω_{391.4 nm}). On the basis of a semiclassical recollision model, we show that an interference of dipolar moments of excited ions created by electron recollisions explains this behavior.

Recollision-Induced Superradiance of Ionized Nitrogen Molecules.

We propose a new mechanism to explain the origin of optical gain in the transitions between the excited and ground states of the ionized nitrogen molecule following irradiation of neutral nitrogen molecules with an intense ultrashort laser pulse. An efficient transfer of population to the excited state is achieved via field-induced multiple recollisions. We show that the proposed excitation mechanism must lead to a superradiant emission, a feature that we confirm experimentally.

Mechanism of Single-Cycle THz Pulse Generation and X-ray Emission: Water-Flow Irradiated by Two Ultra-Short Laser Pulses.

The interaction of two subsequent ultra-short sub-milli-Joule laser pulses with a thin water flow results in an emission of a strong single-cycle THz pulse associated with enhanced soft X-ray emission. In this paper, a chain of processes produced in this interaction is analyzed and compared with other THz generation studies. It is demonstrated that the enhanced THz and X-ray emissions are produced by an energetic electron beam accelerated in the interaction of a main laser pulse with liquid water ejected from the surface by the pre-pulse. This scheme thus provides an efficient laser energy conversion in a THz pulse, avoiding laser self-focusing and filamentation in air.

Modeling of electron nonlocal transport in plasmas using artificial neural networks.

This article presents the use of artificial neural networks (ANN) to predict nonlocal heat flux transport within hydrodynamic simulations. Several cases of laser driven ablation of a plastic target are considered. The database for the ANN training phase is built using the transport module of the hydrodynamic code CHIC. It covers a range of parameters characteristic of laser experiments in the context of high-energy-density physics. Results show that an ANN can efficiently replace a module of nonlocal transport in one- and two-dimensional hydrodynamic simulations, with an error less than 3% in a radius of 0.5µm and an average computation gain of a factor 433 in two dimensions.

High performance modelling of the transport of energetic particles for photon radiotherapy.

This work consists of the validation of a new Grid Based Boltzmann Solver (GBBS) conceived for the description of the transport and energy deposition by energetic particles for radiotherapy purposes. The entropic closure and a compact mathematical formulation allow our code (M1) to calculate the delivered dose with an accuracy comparable to the Monte-Carlo (MC) codes with a computational time that is reduced to the order of few minutes without any special processing power requirement. A validation protocol with heterogeneity inserts has been defined for different photon sources. The comparison with the MC calculated depth-dose curves and transverse profiles of the beam at different depths shows an excellent accuracy of the M1 model.

Strong enhancement of terahertz radiation from laser filaments in air by a static electric field.

We observe a 3 order of magnitude enhancement of the terahertz energy radiated by a femtosecond pulse undergoing filamentation in air in the presence of a static electric field. Measurements of terahertz pulse duration, spectrum, polarization, and radiation pattern elucidate the physical processes responsible for this radiation. A theoretical model explains the results and predicts another 3 orders of magnitude enhancement with a terawatt laser pulse.