Multipronged mapping to the dynamics of a barium atom deposited on argon clusters.

The dynamics of an electronically excited barium atom deposited at the surface of an Ar≈500 cluster was explored in a multipronged approach which associates information from frequency-resolved nanosecond experiments and information from femtosecond time-resolved experiments. In both types of experiments, the dynamics is monitored by photoelectron and photoion spectroscopy.

Synthesis and characterization of attosecond light vortices in the extreme ultraviolet.

Infrared and visible light beams carrying orbital angular momentum (OAM) are currently thoroughly studied for their extremely broad applicative prospects, among which are quantum information, micromachining and diagnostic tools. Here we extend these prospects, presenting a comprehensive study for the synthesis and full characterization of optical vortices carrying OAM in the extreme ultraviolet (XUV) domain. We confirm the upconversion rules of a femtosecond infrared helically phased beam into its high-order harmonics, showing that each harmonic order carries the total number of OAM units absorbed in the process up to very high orders (57). This allows us to synthesize and characterize helically shaped XUV trains of attosecond pulses. To demonstrate a typical use of these new XUV light beams, we show our ability to generate and control, through photoionization, attosecond electron beams carrying OAM. These breakthroughs pave the route for the study of a series of fundamental phenomena and the development of new ultrafast diagnosis tools using either photonic or electronic vortices.

Dual spectral-band interferometry for spatio-temporal characterization of high-power femtosecond lasers.

We present and demonstrate a technique called RED-SEA TADPOLE for the spatio-temporal characterization of high peak power femtosecond lasers. It retains the basic principle of an existing method, where a scanning monomode fiber is utilized in an interferometric scheme to measure the spectral amplitude and phase at all points across an ultrashort laser beam. We combine this approach with dual spectral-band interferometry, to correct for all phase errors occurring in this interferometer, thus allowing for the simultaneous measurement of the beam wavefront and pulse front in a collimated beam of large diameter. The generic phase correction procedure implemented here can also be extended to other fiber optic device applications sensitive to phase fluctuations.

Efficient broadband 400 nm noncollinear second-harmonic generation of chirped femtosecond laser pulses in BBO and LBO.

We report on 400 nm broadband type I frequency doubling in a noncollinear geometry with pulse-front-tilted and chirped femtosecond pulses (λ =800 nm; Fourier transform limited pulse duration, 45 fs). With moderate power densities (2 to 10 GW/cm2) thus avoiding higher-order nonlinear phenomena, the energy conversion efficiency was up to 65%. Second-harmonic pulses of Fourier transform limited pulse duration shorter than the fundamental wave were generated, exhibiting good beam quality and no pulse-front tilt. High energy (20 mJ/pulse) was produced in a 40 mm diameter and 6 mm thick LBO crystal. To the best of our knowledge, this is the first demonstration of this optical configuration with sub-100-fs pulses. Good agreement between experimental results and simulations is obtained.

Complete analog control of the carrier-envelope-phase of a high-power laser amplifier.

In this work we demonstrate the development of a complete analog feedback loop for the control of the carrier-envelope phase (CEP) of a high-average power (20 W) laser operating at 10 kHz repetition rate. The proposed method combines a detection scheme working on a single-shot basis at the full-repetition-rate of the laser system with a fast actuator based either on an acousto-optic or on an electro-optic crystal. The feedback loop is used to correct the CEP fluctuations introduced by the amplification process demonstrating a CEP residual noise of 320 mrad measured on a single-shot basis. The comparison with a feedback loop operating at a lower sampling rate indicates an improvement up to 45% in the residual noise. The measurement of the CEP drift for different integration times clearly evidences the importance of the single-shot characterization of the residual CEP drift. The demonstrated scheme could be efficiently applied for systems approaching the 100 kHz repetition rate regime.

Impact of wave front and coherence optimization in coherent diffractive imaging.

We present single shot nanoscale imaging using a table-top femtosecond soft X-ray laser harmonic source at a wavelength of 32 nm. We show that the phase retrieval process in coherent diffractive imaging critically depends on beam quality. Coherence and image fidelity are measured from single-shot coherent diffraction patterns of isolated nano-patterned slits. Impact of flux, wave front and coherence of the soft X-ray beam on the phase retrieval process and the image quality are discussed. After beam improvements, a final image reconstruction is presented with a spatial resolution of 78 nm (half period) in a single 20 fs laser harmonic shot.

Carrier-Envelope Phase stabilization of a 20 W, grating based, chirped-pulse amplified laser, using electro-optic effect in a LiNbO3 crystal.

Using an original CEP stabilization technique based on the linear electro-optical effect in a specific crystal, we achieved long term CEP stabilization of a 20 W, 1 kHz laser with residual noise as low as 440 mrad (rms). At 3 W, the CEP shot to shot noise is kept as low as 320 mrad (rms) over half an hour.

Attosecond emission from chromium plasma.

We present the first measurement of the attosecond emission generated from underdense plasma produced on a solid target. We generate high-order harmonics of a femtosecond Ti:sapphire laser focused in a weakly ionized underdense chromium plasma. Using the "Reconstruction of Attosecond Beating by Interference of Two-photon Transitions" (RABITT) technique, we show that the 11th to the 19th harmonic orders form in the time domain an attosecond pulse train with each pulse having 300 as duration, which is only 1.05 times the theoretical Fourier transform limit. Measurements reveal a very low positive group delay dispersion of 4200 as2. Beside its fundamental interest, high-order harmonic generation in plasma plumes could thus provide an intense source of attosecond pulses for applications.

Control of the attosecond synchronization of XUV radiation with phase-optimized mirrors.

We report on the advanced amplitude and phase control of attosecond radiation allowed by specifically-designed multilayer XUV mirrors. We first demonstrate that such mirrors can compensate for the intrinsic chirp of the attosecond emission over a large bandwidth of more than 20 eV. We then show that their combination with metallic foils introduces a third-order dispersion that is adjustable through the mirror's incidence angle. This results in a controllable beating allowing the radiation to be shaped from a single to a series of sub-100 as pulses.

Carrier-envelope phase control using linear electro-optic effect.

We present a new method to control the Carrier-Envelope Phase of ultra-short laser pulses by using the linear Electro-Optic Effect. Experimental demonstration is carried out on a Chirped Pulse Amplification based laser. Phase shifts greater than π radian can be obtained by applying moderate voltage on a LiNbO3 crystal with practically no changes to all other parameters of the pulse with the exception of its group delay. Time response of the Electro-Optic effect makes possible shaping at a high repetition rate or stabilization of the CEP of ultra short CPA laser systems.

Single-shot diffractive imaging with a table-top femtosecond soft x-ray laser-harmonics source.

Coherent x-ray diffractive imaging is a powerful method for studies on nonperiodic structures on the nanoscale. Access to femtosecond dynamics in major physical, chemical, and biological processes requires single-shot diffraction data. Up to now, this has been limited to intense coherent pulses from a free electron laser. Here we show that laser-driven ultrashort x-ray sources offer a comparatively inexpensive alternative. We present measurements of single-shot diffraction patterns from isolated nano-objects with a single 20 fs pulse from a table-top high-harmonic x-ray laser. Images were reconstructed with a resolution of 119 nm from the single shot and 62 nm from multiple shots.

High harmonic XUV spectral phase interferometry for direct electric-field reconstruction.

We demonstrate the first experimental complete temporal characterization of high-harmonic XUV pulses by spectral phase interferometry, with an all-optical setup. This method allows us to perform single-shot measurements of the harmonic temporal profile and phase, revealing a remarkable shot-to-shot stability. We characterize harmonics generated in argon by a 50 fs 800 nm laser pulse. The 11th harmonic is found to be 22 fs long with a negative chirp rate of -4.8 x 10(27) s(-2). This duration can be reduced to 13 fs by modulating the polarization of the generating laser. The technique is easy to implement and could be routinely used in femtosecond XUV pump-probe experiments with harmonics.

Complete characterization of a plasma mirror for the production of high-contrast ultraintense laser pulses.

Improving the temporal contrast of ultrashort and ultraintense laser pulses is a major technical issue for high-field experiments. This can be achieved using a so-called "plasma mirror." We present a detailed experimental and theoretical study of the plasma mirror that allows us to quantitatively assess the performances of this system. Our experimental results include time-resolved measurements of the plasma mirror reflectivity, and of the phase distortions it induces on the reflected beam. Using an antireflection coated plate as a target, an improvement of the contrast ratio by more than two orders of magnitude can be achieved with a single plasma mirror. We demonstrate that this system is very robust against changes in the pulse fluence and imperfections of the beam spatial profile, which is essential for applications.

Focused laser intensity measurement at 10(18) W/cm(2) and 1053 nm.

We present a simple experimental setup that makes possible the measurement of the beam section at focus under full-power conditions. We demonstrate that a 1.5-TW laser system can be focused down to a 13.5-microm-diameter spot using conventional lens focalization, thus achieving laser intensities of up to 10(18) W/cm(2).