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1.
Nat Commun ; 15(1): 4346, 2024 May 21.
Artigo em Inglês | MEDLINE | ID: mdl-38773182

RESUMO

Narrow bandwidths are a general bottleneck for applications relying on passive, linear, subwavelength resonators. In the past decades, several efforts have been devoted to overcoming this challenge, broadening the bandwidth of small resonators by the means of analog non-Foster matching networks for radiators, antennas and metamaterials. However, most non-Foster approaches present challenges in terms of tunability, stability and power limitations. Here, by tuning a subwavelength acoustic transducer with digital non-Foster-inspired electronics, we demonstrate five-fold bandwidth enhancement compared to conventional analog non-Foster matching. Long-distance transmission over airborne acoustic channels, with approximately three orders of magnitude increase in power level, validates the performance of the proposed approach. We also demonstrate convenient reconfigurability of our non-Foster-inspired electronics. This implementation provides a viable solution to enhance the bandwidth of sub-wavelength resonance-based systems, extendable to the electromagnetic domain, and enables the practical implementation of airborne and underwater acoustic radiators.

3.
Sci Adv ; 10(15): eadn6095, 2024 Apr 12.
Artigo em Inglês | MEDLINE | ID: mdl-38608013

RESUMO

Topological boundary modes in electronic and classical-wave systems exhibit fascinating properties. In photonics, topological nature of boundary modes can make them robust and endows them with an additional internal structure-pseudo-spins. Here, we introduce heterogeneous boundary modes, which are based on mixing two of the most widely used topological photonics platforms-the pseudo-spin-Hall-like and valley-Hall photonic topological insulators. We predict and confirm experimentally that transformation between the two, realized by altering the lattice geometry, enables a continuum of boundary states carrying both pseudo-spin and valley degrees of freedom (DoFs). When applied adiabatically, this leads to conversion between pseudo-spin and valley polarization. We show that such evolution gives rise to a geometrical phase associated with the synthetic gauge fields, which is confirmed via an Aharonov-Bohm type experiment on a silicon chip. Our results unveil a versatile approach to manipulating properties of topological photonic states and envision topological photonics as a powerful platform for devices based on synthetic DoFs.

4.
J Chem Phys ; 160(14)2024 Apr 14.
Artigo em Inglês | MEDLINE | ID: mdl-38619060

RESUMO

Heterogeneous photocatalysis is an important research problem relevant to a variety of sustainable energy technologies. However, obtaining high photocatalytic efficiency from visible light absorbing semiconductors is challenging due to a combination of weak absorption, transport losses, and low activity. Aspects of this problem have been addressed by multilayer approaches, which provide a general scheme for engineering surface reactivity and stability independent of electronic considerations. However, an analogous broad framework for optimizing light-matter interactions has not yet been demonstrated. Here, we establish a photonic approach using semiconductor metasurfaces that is highly effective in enhancing the photocatalytic activity of GaAs, a high-performance semiconductor with a near-infrared bandgap. Our engineered pillar arrays with heights of ∼150 nm exhibit Mie resonances near 700 nm that result in near-unity absorption and exhibit a field profile that maximizes charge carrier generation near the solid-liquid interface, enabling short transport distances. Our hybrid metasurface photoanodes facilitate oxygen evolution and exhibit enhanced incident photon-to-current efficiencies that are ∼22× larger than a corresponding thin film for resonant excitation and 3× larger for white light illumination. Key to these improvements is the preferential generation of photogenerated carriers near the semiconductor interface that results from the field enhancement profile of magnetic dipolar-type modes.

5.
Nat Commun ; 15(1): 2844, 2024 Apr 02.
Artigo em Inglês | MEDLINE | ID: mdl-38565570

RESUMO

Optical frequency combs, featuring evenly spaced spectral lines, have been extensively studied and applied to metrology, signal processing, and sensing. Recently, frequency comb generation has been also extended to MHz frequencies by harnessing nonlinearities in microelectromechanical membranes. However, the generation of frequency combs at radio frequencies (RF) has been less explored, together with their potential application in wireless technologies. In this work, we demonstrate an RF system able to wirelessly and passively generate frequency combs. This circuit, which we name quasi-harmonic tag (qHT), offers a battery-free solution for far-field ranging of unmanned vehicles (UVs) in GPS-denied settings, and it enables a strong immunity to multipath interference, providing better accuracy than other RF approaches to far-field ranging. Here, we discuss the principle of operation, design, implementation, and performance of qHTs used to remotely measure the azimuthal distance of a UV flying in an uncontrolled electromagnetic environment. We show that qHTs can wirelessly generate frequency combs with µWatt-levels of incident power by leveraging the nonlinear interaction between an RF parametric oscillator and a high quality factor piezoelectric microacoustic resonator. Our technique for frequency comb generation opens new avenues for a wide range of RF applications beyond ranging, including timing, computing and sensing.

6.
Light Sci Appl ; 13(1): 65, 2024 Mar 05.
Artigo em Inglês | MEDLINE | ID: mdl-38438358

RESUMO

Exceptional points (EPs), at which two or more eigenvalues and eigenstates of a resonant system coalesce, are associated with non-Hermitian Hamiltonians with gain and/or loss elements. Dynamic encircling of EPs has received significant interest in recent years, as it has been shown to lead to highly nontrivial phenomena, such as chiral transmission in which the final state of the system depends on the encircling handedness. Previously, chiral transmission for a pair of eigenmodes has been realized by establishing a closed dynamical trajectory in parity-time- (PT-) or anti-PT-symmetric systems. Although chiral transmission of symmetry-broken modes, more accessible in practical photonic integrated circuits, has been realized by establishing a closed trajectory encircling EPs in anti-PT-symmetric systems, the demonstrated transmission efficiency is very low due to path-dependent losses. Here, we demonstrate chiral dynamics in a coupled waveguide system that does not require a closed trajectory. Specifically, we explore an open trajectory linking two infinite points having the same asymptotic eigenmodes (not modes in PT- and anti-PT-symmetric systems), demonstrating that this platform enables high-efficiency chiral transmission, with each eigenmode localized in a single waveguide. This concept is experimentally implemented in a coupled silicon waveguide system at telecommunication wavelengths. Our work provides a new evolution strategy for chiral dynamics with superior performance, laying the foundation for the development of practical chiral-transmission devices.

7.
Nat Commun ; 15(1): 2237, 2024 Mar 12.
Artigo em Inglês | MEDLINE | ID: mdl-38472224

RESUMO

Signal processing is of critical importance for various science and technology fields. Analog optical processing can provide an effective solution to perform large-scale and real-time data processing, superior to its digital counterparts, which have the disadvantages of low operation speed and large energy consumption. As an important branch of modern optics, Fourier optics exhibits great potential for analog optical image processing, for instance for edge detection. While these operations have been commonly explored to manipulate the spatial content of an image, mathematical operations that act directly over the angular spectrum of an image have not been pursued. Here, we demonstrate manipulation of the angular spectrum of an image, and in particular its differentiation, using dielectric metasurfaces operating across the whole visible spectrum. We experimentally show that this technique can be used to enhance desired portions of the angular spectrum of an image. Our approach can be extended to develop more general angular spectrum analog meta-processors, and may open opportunities for optical analog data processing and biological imaging.

8.
Nat Commun ; 15(1): 2380, 2024 Mar 16.
Artigo em Inglês | MEDLINE | ID: mdl-38493161

RESUMO

As a fundamental property of light, polarization serves as an excellent information encoding carrier, playing significant roles in many optical applications, including liquid crystal displays, polarization imaging, optical computation and encryption. However, conventional polarization information encoding schemes based on Malus' law usually consider 1D polarization projections on a linear basis, implying that their encoding flexibility is largely limited. Here, we propose a Poincaré sphere (PS) trajectory encoding approach with metasurfaces that leverages a generalized form of Malus' law governing universal 2D projections between arbitrary elliptical polarization pairs spanning the entire PS. Arbitrary polarization encodings are realized by engineering PS trajectories governed by either arbitrary analytic functions or aligned modulation grids of interest, leading to versatile polarization image transformation functionalities, including histogram stretching, thresholding and image encryption within non-orthogonal PS loci. Our work significantly expands the encoding dimensionality of polarization information, unveiling new opportunities for metasurfaces in polarization optics for both quantum and classical regimes.

9.
ACS Photonics ; 11(3): 816-865, 2024 Mar 20.
Artigo em Inglês | MEDLINE | ID: mdl-38550347

RESUMO

Metasurfaces have recently risen to prominence in optical research, providing unique functionalities that can be used for imaging, beam forming, holography, polarimetry, and many more, while keeping device dimensions small. Despite the fact that a vast range of basic metasurface designs has already been thoroughly studied in the literature, the number of metasurface-related papers is still growing at a rapid pace, as metasurface research is now spreading to adjacent fields, including computational imaging, augmented and virtual reality, automotive, display, biosensing, nonlinear, quantum and topological optics, optical computing, and more. At the same time, the ability of metasurfaces to perform optical functions in much more compact optical systems has triggered strong and constantly growing interest from various industries that greatly benefit from the availability of miniaturized, highly functional, and efficient optical components that can be integrated in optoelectronic systems at low cost. This creates a truly unique opportunity for the field of metasurfaces to make both a scientific and an industrial impact. The goal of this Roadmap is to mark this "golden age" of metasurface research and define future directions to encourage scientists and engineers to drive research and development in the field of metasurfaces toward both scientific excellence and broad industrial adoption.

10.
Nat Commun ; 15(1): 2741, 2024 Mar 28.
Artigo em Inglês | MEDLINE | ID: mdl-38548757

RESUMO

Critical coupling in integrated photonic devices enables the efficient transfer of energy from a waveguide to a resonator, a key operation for many applications. This condition is achieved when the resonator loss rate is equal to the coupling rate to the bus waveguide. Carefully matching these quantities is challenging in practice, due to variations in the resonator properties resulting from fabrication and external conditions. Here, we demonstrate that efficient energy transfer to a non-critically coupled resonator can be achieved by tailoring the excitation signal in time. We rely on excitations oscillating at complex frequencies to load an otherwise overcoupled resonator, demonstrating that a virtual critical coupling condition is achieved if the imaginary part of the complex frequency equals the mismatch between loss and coupling rate. We probe a microring resonator with tailored pulses and observe a minimum intensity transmission T = 0.11 in contrast to a continuous-wave transmission T = 0.58 , corresponding to 8 times enhancement of intracavity intensity. Our technique opens opportunities for enhancing and controlling on-demand light-matter interactions for linear and nonlinear photonic platforms.

11.
Adv Mater ; : e2312421, 2024 Feb 22.
Artigo em Inglês | MEDLINE | ID: mdl-38386009

RESUMO

The discovery of higher-order topological insulator metamaterials, in analogy with their condensed-matter counterparts, has enabled various breakthroughs in photonics, mechanics, and acoustics. A common way of inducing higher-order topological wave phenomena is through pseudo-spins, which mimic the electron spins as a symmetry-breaking degree of freedom. Here we exploit degenerate orbitals in acoustic resonant cavities to demonstrate versatile, orbital-selective, higher-order topological corner states. Type-II corner states are theoretically investigated and experimentally demonstrated based on tailored orbital interactions, without the need for long-range hoppings that has so far served as a key ingredient for Type-II corner states in single-orbital systems. Due to the orthogonal nature of the degenerate p orbitals, we also introduce a universal strategy to realize orbital-dependent edge modes, featuring high-Q edge states identified in bulk bands. Our findings provide an understanding of the interplay between acoustic orbitals and topology, shedding light on orbital-related topological wave physics, as well as its applications for acoustic sensing and trapping. This article is protected by copyright. All rights reserved.

12.
Light Sci Appl ; 13(1): 28, 2024 Jan 24.
Artigo em Inglês | MEDLINE | ID: mdl-38263149

RESUMO

Diffractive nonlocal metasurfaces have recently opened a broad range of exciting developments in nanophotonics research and applications, leveraging spatially extended-yet locally patterned-resonant modes to control light with new degrees of freedom. While conventional grating responses are elegantly captured by temporal coupled mode theory, current approaches are not well equipped to capture the arbitrary spatial response observed in the nascent field of nonlocal metasurfaces. Here, we introduce spatio-temporal coupled mode theory (STCMT), capable of elegantly capturing the key features of the resonant response of wavefront-shaping nonlocal metasurfaces. This framework can quantitatively guide nonlocal metasurface design while maintaining compatibility with local metasurface frameworks, making it a powerful tool to rationally design and optimize a broad class of ultrathin optical components. We validate this STCMT framework against full-wave simulations of various nonlocal metasurfaces, demonstrating that this tool offers a powerful semi-analytical framework to understand and model the physics and functionality of these devices, without the need for computationally intense full-wave simulations. We also discuss how this model may shed physical insights into nonlocal phenomena in photonics and the functionality of the resulting devices. As a relevant example, we showcase STCMT's flexibility by applying it to study and rapidly prototype nonlocal metasurfaces that spatially shape thermal emission.

13.
Nat Commun ; 15(1): 931, 2024 Jan 31.
Artigo em Inglês | MEDLINE | ID: mdl-38296991
14.
Nat Commun ; 15(1): 946, 2024 Jan 31.
Artigo em Inglês | MEDLINE | ID: mdl-38297005

RESUMO

Parity-time (PT) symmetry has been unveiling new photonic regimes in non-Hermitian systems, with opportunities for lasing, sensing and enhanced light-matter interactions. The most exotic responses emerge at the exceptional point (EP) and in the broken PT-symmetry phase, yet in conventional PT-symmetric systems these regimes require large levels of gain and loss, posing remarkable challenges in practical settings. Floquet PT-symmetry, which may be realized by periodically flipping the effective gain/loss distribution in time, can relax these requirements and tailor the EP and PT-symmetry phases through the modulation period. Here, we explore Floquet PT-symmetry in an integrated photonic waveguide platform, in which the role of time is replaced by the propagation direction. We experimentally demonstrate spontaneous PT-symmetry breaking at small gain/loss levels and efficient control of amplification and suppression through the excitation ports. Our work introduces the advantages of Floquet PT-symmetry in a practical integrated photonic setting, enabling a powerful platform to observe PT-symmetric phenomena and leverage their extreme features, with applications in nanophotonics, coherent control of nanoscale light amplification and routing.

15.
Nat Commun ; 14(1): 8162, 2023 Dec 09.
Artigo em Inglês | MEDLINE | ID: mdl-38071337

RESUMO

Topological phases of matter have attracted significant attention in recent years, due to the unusual robustness of their response to defects and disorder. Various research efforts have been exploring classical and quantum topological wave phenomena in engineered materials, in which different degrees of freedom (DoFs) - for the most part based on broken crystal symmetries associated with pseudo-spins - induce synthetic gauge fields that support topological phases and unveil distinct forms of wave propagation. However, spin is not the only viable option to induce topological effects. Intrinsic orbital DoFs in spinless systems may offer a powerful alternative platform, mostly unexplored to date. Here we reveal orbital-selective wave-matter interactions in acoustic systems supporting multiple orbital DoFs, and report the experimental demonstration of disorder-immune orbital-induced topological edge states in a zigzag acoustic 1D spinless lattice. This work expands the study of topological phases based on orbitals, paving the way to explore other orbital-dependent phenomena in spinless systems.

16.
Nat Commun ; 14(1): 7078, 2023 Nov 04.
Artigo em Inglês | MEDLINE | ID: mdl-37925563

RESUMO

Optical metasurfaces performing analog image processing - such as spatial differentiation and edge detection - hold the potential to reduce processing times and power consumption, while avoiding bulky 4 F lens systems. However, current designs have been suffering from trade-offs between spatial resolution, throughput, polarization asymmetry, operational bandwidth, and isotropy. Here, we show that dispersion engineering provides an elegant way to design metasurfaces where all these critical metrics are simultaneously optimized. We experimentally demonstrate silicon metasurfaces performing isotropic and dual-polarization edge detection, with numerical apertures above 0.35 and spectral bandwidths of 35 nm around 1500 nm. Moreover, we introduce quantitative metrics to assess the efficiency of these devices. Thanks to the low loss nature and dual-polarization response, our metasurfaces feature large throughput efficiencies, approaching the theoretical maximum for a given NA. Our results pave the way for low-loss, high-efficiency and broadband optical computing and image processing with free-space metasurfaces.

17.
Nano Lett ; 23(23): 11252-11259, 2023 Dec 13.
Artigo em Inglês | MEDLINE | ID: mdl-37948605

RESUMO

Modulating anisotropic phonon polaritons (PhPs) can open new avenues in infrared nanophotonics. Promising PhP dispersion engineering through polariton hybridization has been demonstrated by coupling gated graphene to single-layer α-MoO3. However, the mechanism underlying the gate-dependent modulation of hybridization has remained elusive. Here, using IR nanospectroscopic imaging, we demonstrate active modulation of the optical response function, quantified in measurements of gate dependence of wavelength, amplitude, and dissipation rate of the hybrid plasmon-phonon polaritons (HPPPs) in both single-layer and twisted bilayer α-MoO3/graphene heterostructures. Intriguingly, while graphene doping leads to a monotonic increase in HPPP wavelength, amplitude and dissipation rate show transition from an initially anticorrelated decrease to a correlated increase. We attribute this behavior to the intricate interplay of gate-dependent components of the HPPP complex momentum. Our results provide the foundation for active polariton control of integrated α-MoO3 nanophotonics devices.

18.
Nano Lett ; 23(21): 9803-9810, 2023 Nov 08.
Artigo em Inglês | MEDLINE | ID: mdl-37879099

RESUMO

Two-dimensional exciton-polaritons in monolayer transition metal dichalcogenides (TMDs) exhibit practical advantages in valley coherence, optical nonlinearities, and even bosonic condensation owing to their light-emission capability. To achieve robust exciton-polariton emission, strong photon-exciton couplings are required at the TMD monolayer, which is challenging due to its atomic thickness. High-quality (Q) factor optical cavities with narrowband resonances are an effective approach but typically limited to a specific excitonic state of a certain TMD material. Herein, we achieve on-demand exciton-polariton emission from a wide range of TMDs at room temperature by hybridizing excitons with broadband Mie resonances spanning the whole visible spectrum. By confining broadband light at the TMD monolayer, our one type of Mie resonator on different TMDs enables enhanced light-matter interactions with multiple excitonic states simultaneously. We demonstrate multi-Rabi splittings and robust polaritonic photoluminescence in monolayer WSe2, WS2, and MoS2. The hybrid system also shows the potential to approach the ultrastrong coupling regime.

19.
Nature ; 620(7974): 533-537, 2023 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-37587298

RESUMO

Controlling quantum materials with light is of fundamental and technological importance. By utilizing the strong coupling of light and matter in optical cavities1-3, recent studies were able to modify some of their most defining features4-6. Here we study the magneto-optical properties of a van der Waals magnet that supports strong coupling of photons and excitons even in the absence of external cavity mirrors. In this material-the layered magnetic semiconductor CrSBr-emergent light-matter hybrids called polaritons are shown to substantially increase the spectral bandwidth of correlations between the magnetic, electronic and optical properties, enabling largely tunable optical responses to applied magnetic fields and magnons. Our results highlight the importance of exciton-photon self-hybridization in van der Waals magnets and motivate novel directions for the manipulation of quantum material properties by strong light-matter coupling.

20.
Sci Bull (Beijing) ; 68(19): 2164-2169, 2023 Oct 15.
Artigo em Inglês | MEDLINE | ID: mdl-37604721

RESUMO

Synthetic magnetism has been recently realized using spatiotemporal modulation patterns, producing non-reciprocal steering of charge-neutral particles such as photons and phonons. Here, we design and experimentally demonstrate a non-reciprocal acoustic system composed of three compact cavities interlinked with both dynamic and static couplings, in which phase-correlated modulations induce a synthetic magnetic flux that breaks time-reversal symmetry. Within the rotating wave approximation, the transport properties of the system are controlled to efficiently realize large non-reciprocal acoustic transport. By optimizing the coupling strengths and modulation phases, we achieve frequency-preserved unidirectional transport with 45-dB isolation ratio and 0.85 forward transmission. Our results open to the realization of acoustic non-reciprocal technologies with high efficiency and large isolation, and offer a route towards Floquet topological insulators for sound.

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