Unidirectional Lasing from Mirror-Coupled Dielectric Lattices.

This paper reports how a hybrid system composed of transparent dielectric lattices over a metal mirror can produce high-quality lattice resonances for unidirectional lasing. The enhanced electromagnetic fields are concentrated in the cladding of the periodic dielectric structures and away from the metal. Based on a mirror-image model, we reveal that such high-quality lattice resonances are governed by bound states in the continuum resulting from destructive interference. Using hexagonal arrays of titanium dioxide nanoparticles on a silica-coated silver mirror, we observed lattice resonances with quality factors of up to 2750 in the visible regime. With the lattice resonances as optical feedback and dye solution as the gain medium, we demonstrated unidirectional lasing under optical pumping, where the array size was down to 100 µm × 100 µm. Our scheme can be extended to other spectral regimes to simultaneously achieve strongly enhanced surface fields and high quality factors.

Photochromic switching of narrow-band lattice resonances.

Narrow-band resonances supported by a variety of periodic metallic or dielectric nanostructures have great potential applications in light sources, optical sensors, and switches or modulators. Here we report the switching of narrow-band lattice resonances in a mirror-backed two-dimensional array of dielectric nanopillars. The nanopillar is composed of a silica core and photochromic coating. By exposure to ultraviolet light, the photochromic molecules can be turned into a state that is highly absorptive around the wavelength of the lattice resonance. Because the lattice resonance has enhanced the near-fields concentrated on the tops of dielectric nanopillars, the absorptive coating can destroy this resonance. The absorptive state of the photochromic molecules can be recovered to a transparent state by exposure to visible light. We fabricate the device and characterize the change of reflection spectra to demonstrate the reversible switching of lattice resonances by exposure to ultraviolet and visible light alternately. An all-optical control of the narrow-band photoluminescence is further demonstrated by combining a fluorescent dye with the photochromic molecules.

Lattice-Resonance Metalenses for Fully Reconfigurable Imaging.

This paper describes a reconfigurable metalens system that can image at visible wavelengths based on arrays of coupled plasmonic nanoparticles. These lenses manipulated the wavefront and focused light by exciting surface lattice resonances that were tuned by patterned polymer blocks on single-particle sites. Predictive design of the dielectric nanoblocks was performed using an evolutionary algorithm to create a range of three-dimensional focusing responses. For scalability, we demonstrated a simple technique for erasing and writing the polymer nanostructures on the metal nanoparticle arrays in a single step using solvent-assisted nanoscale embossing. This reconfigurable materials platform enables tunable focusing with diffraction-limited resolution and offers prospects for highly adaptive, compact imaging.

Unidirectional Enhanced Emission from 2D Monolayer Suspended by Dielectric Pillar Array.

Monolayers of transition metal dichalcogenides show great promise for optoelectronic devices as atomically thin semiconductors. Although dielectric or metal nanostructures have been extensively studied for tailoring and enhancing emission from monolayers, their applications are limited because of the mode concentrating inside the dielectric or the high optical losses in metals, together with the low quantum yield in monolayers. Here, we demonstrate that a metal-backed dielectric pillar array can suspend monolayers to increase the radiative recombination, and simultaneously, create strongly confined band-edge modes on surface directly accessible to monolayers. We observe unidirectional enhanced emission from WSe2 monolayers on polymer pillar array.

Surface mode with large field enhancement in dielectric-dimer-on-mirror structures.

Plasmonic nanostructures with accessible and strongly enhanced fields are useful for a variety of applications related to surface-enhanced light-matter interaction. We describe a method to migrate localized fields from a metal to dielectric surface. By arranging low-index contrast dielectric dimers on an optically thick metal film, a narrow-linewidth resonant mode is formed through diffraction coupling, with accessible enhancement away from a metal surface. The enhancement in the electric field intensity is over 2000 by dielectric dimers with a 100 nm gap and 720 nm period, and the resonant linewidth is about 0.35 nm around the wavelength of 725 nm. The dispersion of this periodic structure allows resonant enhancement of not only emission but also excitation. The design principle provides a means to tune the narrow-linewidth resonance over a wide wavelength range from ultraviolet to near-infrared.

Highly reproducible surface-enhanced Raman scattering substrate for detection of phenolic pollutants.

The ordering degree of nanostructures is the key to determining the uniformity of surface-enhanced Raman scattering (SERS). However, fabrication of large-area ordered nanostructures remains a challenge, especially with the ultrahigh-density (>1010 cm-2). Here, we report a fabrication of large-area ultrahigh-density ordered Ag@Al2O3/Ag core-shell nanosphere (NS) arrays with tunable nanostructures. The ultrahigh-density (2.8 × 1010 cm-2) ordered NS arrays over a large-area capability (diameter >4.0 cm) enable the uniform SERS signals with the relative standard deviation of less than 5%. The as-fabricated highly reproducible SERS substrate can be applied to detect trace phenolic pollutants in water. This work does not only provide a new route for synthesizing the ultrahigh-density ordered nanostructures, but also create a new class of SERS substrates with high sensitivity and excellent reproducibility.

Broadband metallic absorber on a non-planar substrate.

Absorbers for visible and near-infrared light are realized by depositing a thin iron layer on arrays of cones which are replicated from a porous template. The replicated conic structure itself is of several micrometers and ineffective at antireflection, but the subsequent deposition of iron on top generates nano-meter-size columnar structures, and thus broadband absorption enhancement is achieved.

Enhanced catalytic activity for methanol electro-oxidation of uniformly dispersed nickel oxide nanoparticles-carbon nanotube hybrid materials.

Highy crystalline NiO nanoparticles are uniformly grown on the walls of carbon nanotubes (CNTs) by atomic layer deposition (ALD) at moderate temperature.Their size and stoichiometry are controlled by the ALD process parameters. The obtained NiO/CNT hybrids exhibit excellent performance in the electro-oxidation of methanol.

Gain saturation in gain-guided slab waveguides with large-index antiguiding.

We investigate numerically and analytically the effects of gain saturation on the propagation of the fundamental mode in a gain-guided index-antiguided slab waveguide. The propagating mode adapts to gain saturation by becoming less confined, while at the same time its peak intensity increases more slowly. At steady state, both the mode shape and the power remain constant.

Design and experimental realization of a broadband transformation media field rotator at microwave frequencies.

We designed a metamaterial field rotator that can rotate electromagnetic wave fronts. Our starting point was the transformation-media concept. Effective medium theories and full simulations facilitated the actual design process. We created at a very simple structure comprising of an array of identical aluminum metal plates. We made and measured a sample and we experimentally demonstrated the field rotation effect as well as the broadband functionality at microwave frequencies.

Gain guiding in large-core Bragg fibers.

We theoretically analyze gain guiding in large-core Bragg fibers, to be used for large-mode-area laser amplifiers with single-transverse-mode operation. The signal is gain-guided in a low-index core, whereas the pump is guided by the photonic bandgap of the Bragg cladding to achieve good confinement. The high-index layers in the Bragg cladding are half-wave thick at the signal wavelength in order to eliminate Bragg reflection, reducing the Bragg fiber effectively to a step-index fiber for gain guiding.

Far-field image magnification for acoustic waves using anisotropic acoustic metamaterials.

A kind of two-dimensional acoustic metamaterial is designed so that it exhibits strong anisotropy along two orthogonal directions. Based on the rectangular equal frequency contour of this metamaterial, magnifying lenses for acoustic waves, analogous to electromagnetic hyperlenses demonstrated recently in the optical regime, can be realized. Such metamaterial may offer applications in imaging for systems that obey scalar wave equations.

Polarization beam splitters based on a two-dimensional photonic crystal of negative refraction.

A two-dimensional metallo-dielectric photonic crystal of negative refraction was designed for the application of polarization beam splitters. To match the refractive index of air, the effective refractive index of the designed photonic crystal is -1 for TE polarization and +1 for TM polarization. Two types of polarization beam splitter are presented.

Three-dimensional photonic crystal of negative refraction achieved by interference lithography.

A three-dimensional bicontinuous photonic crystal of a bcc lattice with all-angle negative refraction that can be achieved at optical frequencies by interference lithography is proposed. A numerical simulation of the focusing imaging of a slab of this crystal was performed to verify the property of all-angle negative refraction. The dependence of the negative-refraction frequency range on the threshold of photoresist development and on the dielectric constant is also discussed.

Two-stage design method for realization of photonic bandgap structures with desired symmetries by interference lithography.

Interference lithography for the fabrication of photonic crystals is considered. A two-stage design method for realization of photonic bandgap structures with desired symmetries is developed. An optimal photonic crystal with a large bandgap is searched by adjusting some parameters while keeping some basic symmetry of the unit cell unchanged. A nonlinear programming method is then used to find the optimal electric field vectors of the laser beams and realize the desired interference pattern. The present method is useful for a rational and systematical design of new photonic bandgap structures.

Subwavelength focusing and imaging by a multimode optical waveguide.

A simple subwavelength focusing system formed by a straight or bent multimode waveguide is investigated numerically. The simulation results indicate that an appropriately designed multimode waveguide can focus the outgoing waves of a point source and form an image with a full width at half-maximum of less than half a wavelength in the near-field area at the other side of the waveguide. The physical mechanism of the subwavelength focusing for this imaging system is explained.

General properties of N x M self-images in a strongly confined rectangular waveguide.

General properties of N x M self-images in a strongly confined rectangular waveguide are given. Analytical formulas are derived for the positions, amplitudes, and phases of the N x M images at the end of multimode interference section. The formulas are verified with numerical simulation of a three-dimensional semivectorial beam propagation method.