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1.
ACS Omega ; 7(37): 33518-33529, 2022 Sep 20.
Artigo em Inglês | MEDLINE | ID: mdl-36157734

RESUMO

This work studied a multistage gasification system that is designed for producing a syngas with a low tar content. The proposed system is an atmospheric bubbling fluidized-bed gasifier and comprises mainly pyrolysis, combustion, and gasification zones. The numerical investigation is performed using Aspen Plus to study Prosopis Juliflora gasification. Chemical reactions as well as tar treatment in the process are investigated. Two different pyrolysis temperatures were considered: 500 and 600 °C, along with three different particle size ranges: 0.2-0.5, 0.5-1, and 1-2 mm. The effect of the air-to-biomass ratio, with values from 0.2 to 1.2, and the gasification reactor temperature, from 800 to 1000 °C, on the composition of product gas and tar species formation during the process (phenol, naphthalene, benzene, and toluene), its lower heating value (LHV), and cold gasification efficiency (CGE) were studied. Results showed that a pyrolysis temperature of 600 °C and a particle size range of 0.2-0.5 mm displayed less tar produced from both combustion and gasification zones and were associated with greater CO, H2, and CH4 yields, compared to the other pyrolysis parameters tested. Increasing the gasification temperature led to increasing the CO, H2, and tar yields and decreasing the CH4 yield and CGE. The maximum CGE combined with the minimum tar amount produced could be obtained with values of 800 °C and 1.2 for the gasification temperature and the air-to-biomass ratio, respectively. The numerical simulation results will be used to improve the performance of the proposed system.

2.
ACS Omega ; 6(51): 35607-35618, 2021 Dec 28.
Artigo em Inglês | MEDLINE | ID: mdl-34984292

RESUMO

In this work, mixed convection and entropy generation analyses in a partitioned porous cavity with double inner rotating cylinders are explored under magnetic field effects. A curved partition shape is considered with identical rotating cylinders and an inclined magnetic field, while the right vertical wall moves with a constant speed in the y-direction. Numerical simulations are performed by considering various values of Rayleigh number, Hartman number, Darcy number, inclination of the magnetic field, size of the curved partitions, and rotational speeds of the inner cylinders and their vertical locations with the cavity. Complicated flow field with multicellular structures are observed due to the complex interaction between the natural convection, moving wall, and rotational effects of inner cylinders. Improved heat-transfer performance is obtained with higher values of magnetic field inclination, higher values of permeability/porosity of the medium, and higher rotational speeds of the cylinders. Almost doubling of the average Nu number is obtained by decreasing the value of the Hartmann number from 25 to 0 or varying the magnetic field inclination from 90 to 0. When rotational effects of the cylinders are considered, average heat-transfer improvements by a factor of 5 and 5.9 are obtained for nondimensional rotational speeds of 5 and -5 in comparison with the case of motionless cylinders. An optimum length of the porous layer is achieved for which the best heat-transfer performance is achieved. As the curvature size of the partition is increased, better heat transfer of the hot wall is obtained and up to 138% enhancement is achieved. Significant increments of entropy generation are observed for left and right domains including the rotating cylinders. The magnetic field parameter also affects the entropy generation and contributions of different domains including the curved porous partition.

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