Control of Electron Wave Packets Close to the Continuum Threshold Using Near-Single-Cycle THz Waveforms.

The control of low-energy electrons by carrier-envelope-phase-stable near-single-cycle THz pulses is demonstrated. A femtosecond laser pulse is used to create a temporally localized wave packet through multiphoton absorption at a well defined phase of a synchronized THz field. By recording the photoelectron momentum distributions as a function of the time delay, we observe signatures of various regimes of dynamics, ranging from recollision-free acceleration to coherent electron-ion scattering induced by the THz field. The measurements are confirmed by three-dimensional time-dependent Schrödinger equation simulations. A classical trajectory model allows us to identify scattering phenomena analogous to strong-field photoelectron holography and high-order above-threshold ionization.

Magnetic-Field Effect in High-Order Above-Threshold Ionization.

We experimentally and theoretically investigate the influence of the magnetic component of an electromagnetic field on high-order above-threshold ionization of xenon atoms driven by ultrashort femtosecond laser pulses. The nondipole shift of the electron momentum distribution along the light-propagation direction for high energy electrons beyond the 2U_{p} classical cutoff is found to be vastly different from that below this cutoff, where U_{p} is the ponderomotive potential of the driving laser field. A local minimum structure in the momentum dependence of the nondipole shift above the cutoff is identified for the first time. With the help of classical and quantum-orbit analysis, we show that large-angle rescattering of the electrons strongly alters the partitioning of the photon momentum between electron and ion. The sensitivity of the observed nondipole shift to the electronic structure of the target atom is confirmed by three-dimensional time-dependent Schrödinger equation simulations for different model potentials. Our work paves the way toward understanding the physics of extreme light-matter interactions at long wavelengths and high electron kinetic energies.

Theory of Subcycle Linear Momentum Transfer in Strong-Field Tunneling Ionization.

Interaction of a strong laser pulse with matter transfers not only energy but also linear momentum of the photons. Recent experimental advances have made it possible to detect the small amount of linear momentum delivered to the photoelectrons in strong-field ionization of atoms. We present numerical simulations as well as an analytical description of the subcycle phase (or time) resolved momentum transfer to an atom accessible by an attoclock protocol. We show that the light-field-induced momentum transfer is remarkably sensitive to properties of the ultrashort laser pulse such as its carrier-envelope phase and ellipticity. Moreover, we show that the subcycle-resolved linear momentum transfer can provide novel insights into the interplay between nonadiabatic and nondipole effects in strong-field ionization. This work paves the way towards the investigation of the so-far unexplored time-resolved nondipole nonadiabatic tunneling dynamics.

Gouy's Phase Anomaly in Electron Waves Produced by Strong-Field Ionization.

Ionization of atoms by strong laser fields produces photoelectron momentum distributions that exhibit modulations due to the interference of outgoing electron trajectories. For a faithful modeling, it is essential to include previously overlooked phase shifts occurring when trajectories pass through focal points. Such phase shifts are known as Gouy's phase anomaly in optics or as Maslov phases in semiclassical theory. Because of Coulomb focusing in three dimensions, one out of two trajectories in photoelectron holography goes through a focal point as it crosses the symmetry axis in momentum space. In addition, there exist observable Maslov phases already in two dimensions. Clustering algorithms enable us to implement a semiclassical model with the correct preexponential factor that affects both the weight and the phase of each trajectory. We also derive a simple rule to relate two-dimensional and three-dimensional models for linear polarization. It explains the shifted interference fringes and weaker high-energy yield in three dimensions. The results are in excellent agreement with solutions of the time-dependent Schrödinger equation.

Attosecond-Scale Streaking Methods for Strong-Field Ionization by Tailored Fields.

Streaking with a weak probe field is applied to ionization in a two-dimensional strong field tailored to mimic linear polarization, but without disturbance by recollision or intracycle interference. This facilitates the observation of electron-momentum-resolved times of ionization with few-attosecond precision, as demonstrated by simulations for a model helium atom. Aligning the probe field along the ionizing field provides meaningful ionization times in agreement with the attoclock concept that ionization at maximum field corresponds to the peak of the momentum distribution, which is shifted due to the Coulomb force on the outgoing electron. In contrast, this attoclock shift is invisible in orthogonal streaking. Even without a probe field, streaking happens naturally along the laser propagation direction due to the laser magnetic field. As with an orthogonal probe field, the attoclock shift is not accessible by the magnetic-field scheme. For a polar molecule, the attoclock shift depends on orientation, but this does not imply an orientation dependence in ionization time.

Signatures of Electronic Structure in Bicircular High-Harmonic Spectroscopy.

High-harmonic spectroscopy driven by circularly polarized laser pulses and their counterrotating second harmonic is a new branch of attosecond science which currently lacks quantitative interpretations. We extend this technique to the midinfrared regime and record detailed high-harmonic spectra of several rare-gas atoms. These results are compared with the solution of the Schrödinger equation in three dimensions and calculations based on the strong-field approximation that incorporate accurate scattering-wave recombination matrix elements. A quantum-orbit analysis of these results provides a transparent interpretation of the measured intensity ratios of symmetry-allowed neighboring harmonics in terms of (i) a set of propensity rules related to the angular momentum of the atomic orbitals, (ii) atom-specific matrix elements related to their electronic structure, and (iii) the interference of the emissions associated with electrons in orbitals corotating or counterrotating with the laser fields. These results provide the foundation for a quantitative understanding of bicircular high-harmonic spectroscopy.