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1.
Phys Rev Lett ; 123(6): 067202, 2019 Aug 09.
Artigo em Inglês | MEDLINE | ID: mdl-31491175

RESUMO

We report a high-resolution terahertz spectroscopic study of quantum spin dynamics in the antiferromagnetic Heisenberg-Ising spin-chain compound BaCo_{2}V_{2}O_{8} as a function of temperature and longitudinal magnetic field. Confined spinon excitations are observed in an antiferromagnetic phase below T_{N}≃5.5 K. In a field-induced gapless phase above B_{c}=3.8 T, we identify many-body string excitations as well as low-energy fractional psinon or antipsinon excitations by comparing to Bethe ansatz calculations. In the vicinity of B_{c}, the high-energy string excitations are found to have a dominant contribution to the spin dynamics as compared with the fractional excitations.

2.
Phys Rev Lett ; 120(20): 207205, 2018 May 18.
Artigo em Inglês | MEDLINE | ID: mdl-29864334

RESUMO

We report on magnetization, sound-velocity, and magnetocaloric-effect measurements of the Ising-like spin-1/2 antiferromagnetic chain system BaCo_{2}V_{2}O_{8} as a function of temperature down to 1.3 K and an applied transverse magnetic field up to 60 T. While across the Néel temperature of T_{N}∼5 K anomalies in magnetization and sound velocity confirm the antiferromagnetic ordering transition, at the lowest temperature the field-dependent measurements reveal a sharp softening of sound velocity v(B) and a clear minimum of temperature T(B) at B_{⊥}^{c,3D}=21.4 T, indicating the suppression of the antiferromagnetic order. At higher fields, the T(B) curve shows a broad minimum at B_{⊥}^{c}=40 T, accompanied by a broad minimum in the sound velocity and a saturationlike magnetization. These features signal a quantum phase transition, which is further characterized by the divergent behavior of the Grüneisen parameter Γ_{B}∝(B-B_{⊥}^{c})^{-1}. By contrast, around the critical field, the Grüneisen parameter converges as temperature decreases, pointing to a quantum critical point of the one-dimensional transverse-field Ising model.

3.
Phys Rev Lett ; 111(18): 187202, 2013 Nov 01.
Artigo em Inglês | MEDLINE | ID: mdl-24237555

RESUMO

Comparing high-resolution specific heat and thermal expansion measurements to exact finite-size diagonalization, we demonstrate that Cs(2)CoCl(4) for a magnetic field along the crystallographic b axis realizes the spin-1/2 XXZ chain in a transverse field. Exploiting both thermal as well as virtual excitations of higher crystal-field states, we find that the spin chain is in the XY limit with an anisotropy J(z)/J[perpindicular] ≈ 0.12, substantially smaller than previously believed. A spin-flop Ising quantum phase transition occurs at a critical field of µ(0)H(b)(cr) ≈ 2 T before around 3.5 T the description in terms of an effective spin-1/2 chain becomes inapplicable.

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